journal article·2022-03-11Open access

Structural Reconstruction in Lead-Free Two-Dimensional Tin Iodide Perovskites Leading to High Quantum Yield Emission

Sushant Ghimire, Kevin Oldenburg, Stephan Bartling, Rostyslav Lesyuk, Christian Klinke

ACS Energy Letters· Volume 7· Issue 3

Abstract

We report a structural reconstruction-induced high photoluminescence quantum yield of 25% in colloidal two-dimensional tin iodide nanosheets that are synthesized by a hot-injection method. The as-synthesized red-colored nanosheets of octylammonium tin iodide perovskites at room temperature transform to white hexagonal nanosheets upon washing or exposure to light. This structural change increases the bandgap from 2.0 to 3.0 eV, inducing a large Stokes shift and a broadband emission. Further, a long photoluminescence lifetime of about 1 μs is measured for the nanosheets. Such long-lived broad and intense photoluminescence with a large Stokes shift is anticipated to originate from tin iodide clusters that are formed during the structural reconstruction. The stereoactive 5s2 lone pair of tin(II) ions perturbs the excited state geometry of the white hexagonal nanosheets and facilitates the formation of self-trapped excitons. Such broadband and intensely emitting metal halide nanosheets are promising for white light-emitting diodes.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Perovskite Materials and Applications · Quantum Dots Synthesis And Properties · 2D Materials and Applications

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Institute of Physics, University of Rostock, Albert-Einstein-Strasse 23, 18059 Rostock, Germany

Center for Interdisciplinary Electron Microscopy (ELMI-MV), Department “Life, Light & Matter”, University of Rostock, Albert-Einstein-Strasse 25, 18059 Rostock, Germany

Leibniz Institute for Catalysis (LIKAT), Albert-Einstein-Strasse 29a, 18059 Rostock, Germany

Department of Chemistry, Swansea University, Swansea SA2 8PP, United Kingdom

Funding

European Regional Development Fund · Deutsche Forschungsgemeinschaft · Alexander von Humboldt-Stiftung

References (69)

Show source-provided references
1. 10.1021/ja809598r10.1021/ja809598r ↗
2. 10.1126/science.abh388410.1126/science.abh3884 ↗
3. 10.1038/s41467-021-25407-810.1038/s41467-021-25407-8 ↗
4. 10.1038/ncomms905610.1038/ncomms9056 ↗
5. 10.1038/ncomms640410.1038/ncomms6404 ↗
6. 10.1021/acs.chemrev.6b0013610.1021/acs.chemrev.6b00136 ↗
7. 10.1021/acsenergylett.8b0061510.1021/acsenergylett.8b00615 ↗
8. 10.1038/ncomms1521810.1038/ncomms15218 ↗
9. 10.1021/acs.jpclett.8b0040610.1021/acs.jpclett.8b00406 ↗
10. 10.1021/acsami.8b2221710.1021/acsami.8b22217 ↗
11. 10.1039/D1NR02769G10.1039/D1NR02769G ↗
12. 10.1021/acs.chemmater.0c0061310.1021/acs.chemmater.0c00613 ↗
13. 10.1002/anie.20140646610.1002/anie.201406466 ↗
14. 10.1016/j.joule.2018.11.02610.1016/j.joule.2018.11.026 ↗
15. 10.1021/acsmaterialslett.0c0012410.1021/acsmaterialslett.0c00124 ↗
16. 10.1021/acsenergylett.0c0005810.1021/acsenergylett.0c00058 ↗
17. 10.1002/adma.20210721110.1002/adma.202107211 ↗
18. 10.1021/acsnano.9b0897510.1021/acsnano.9b08975 ↗
19. 10.1126/science.aal421110.1126/science.aal4211 ↗
20. 10.1021/acs.chemrev.8b0047710.1021/acs.chemrev.8b00477 ↗
21. 10.1021/acs.jpclett.0c0035910.1021/acs.jpclett.0c00359 ↗
22. 10.1002/asia.20210107510.1002/asia.202101075 ↗
23. 10.1039/C7SC01590A10.1039/C7SC01590A ↗
24. 10.1021/acs.jpclett.1c0182810.1021/acs.jpclett.1c01828 ↗
25. 10.1021/acs.chemmater.7b0118410.1021/acs.chemmater.7b01184 ↗
26. 10.1021/acs.chemmater.0c0125410.1021/acs.chemmater.0c01254 ↗
27. 10.1039/C9SC00453J10.1039/C9SC00453J ↗
28. 10.1021/acsami.7b1286210.1021/acsami.7b12862 ↗
29. 10.1021/acsenergylett.8b0223910.1021/acsenergylett.8b02239 ↗
30. 10.1039/C9CC08216F10.1039/C9CC08216F ↗
31. 10.1021/acsenergylett.0c0104710.1021/acsenergylett.0c01047 ↗
32. 10.1021/acs.jpclett.0c0235510.1021/acs.jpclett.0c02355 ↗
33. 10.1021/acs.jpcc.0c0530110.1021/acs.jpcc.0c05301 ↗
34. 10.1021/acs.accounts.7b0043310.1021/acs.accounts.7b00433 ↗
35. 10.1016/j.joule.2020.12.00810.1016/j.joule.2020.12.008 ↗
36. 10.1021/jacs.8b0869110.1021/jacs.8b08691 ↗
37. 10.1002/adom.20210142310.1002/adom.202101423 ↗
38. 10.1103/PhysRevMaterials.3.03460410.1103/PhysRevMaterials.3.034604 ↗
39. 10.1021/jacs.9b0236510.1021/jacs.9b02365 ↗
40. 10.1021/acsmaterialslett.0c0021110.1021/acsmaterialslett.0c00211 ↗
41. 10.1038/s41467-020-20555-910.1038/s41467-020-20555-9 ↗
42. 10.1038/s41467-019-13910-y10.1038/s41467-019-13910-y ↗
43. 10.1021/jacs.5b1347010.1021/jacs.5b13470 ↗
44. 10.1002/asia.20180057310.1002/asia.201800573 ↗
45. 10.1021/acs.jpclett.1c0317010.1021/acs.jpclett.1c03170 ↗
46. 10.1021/acsomega.9b0220310.1021/acsomega.9b02203 ↗
47. 10.1021/acsnano.6b0386310.1021/acsnano.6b03863 ↗
48. 10.1021/acsnano.9b0190710.1021/acsnano.9b01907 ↗
49. 10.1039/C7NR09564C10.1039/C7NR09564C ↗
50. 10.1021/acsnano.6b0349610.1021/acsnano.6b03496 ↗
51. 10.1021/acs.nanolett.7b0327210.1021/acs.nanolett.7b03272 ↗
52. 10.1021/acs.langmuir.9b0212910.1021/acs.langmuir.9b02129 ↗
53. 10.1039/C9CP03080H10.1039/C9CP03080H ↗
54. 10.1021/acs.chemmater.9b0131810.1021/acs.chemmater.9b01318 ↗
55. 10.1007/s12200-020-1051-x10.1007/s12200-020-1051-x ↗
56. 10.1021/ja411045r10.1021/ja411045r ↗
57. 10.1038/s41467-021-22864-z10.1038/s41467-021-22864-z ↗
58. 10.1021/acs.chemrev.0c0100610.1021/acs.chemrev.0c01006 ↗
59. 10.1021/acsenergylett.1c0101510.1021/acsenergylett.1c01015 ↗
60. 10.1038/ncomms849710.1038/ncomms8497 ↗
61. 10.1021/acsami.0c0673710.1021/acsami.0c06737 ↗
62. 10.1103/PhysRevB.45.898910.1103/PhysRevB.45.8989 ↗
63. 10.1038/s41467-019-13773-310.1038/s41467-019-13773-3 ↗
64. 10.1016/j.jssc.2013.07.00810.1016/j.jssc.2013.07.008 ↗
65. 10.1038/369467a010.1038/369467a0 ↗
66. 10.1021/jacs.7b0181510.1021/jacs.7b01815 ↗
67. NIST X-ray Photoelectron Spectroscopy Database. NIST Standard Reference Database Number 20, National Institute of Standards and Technology: Gaithersburg MD, 2000: https://srdata.nist.gov/xps/ (retrieved 2022-02-02).
68. 10.1039/C6TC04864A10.1039/C6TC04864A ↗
69. 10.1021/acs.chemmater.6b0132910.1021/acs.chemmater.6b01329 ↗