journal article·2024-03-08Open access

Advances in Perovskite Nanocrystals and Nanocomposites for Scintillation Applications

Abhinav Anand, Matteo L. Zaffalon, Andrea Erroi, Francesca Cova, Francesco Carulli, Sergio Brovelli

ACS Energy Letters· Volume 9· Issue 3

Abstract

In recent years, the field of radiation detection has witnessed a paradigm shift with the emergence of plastic scintillators incorporating perovskite nanocrystals (PNCs). This innovative class of scintillators not only capitalizes on the superior luminescent properties of PNCs but also harnesses the flexibility and processability of polymers. This review explores the intricate landscape of synthesizing and fabricating scintillating PNCs and nanocomposites, delving into the methods employed in their production. From solution-based methods to innovative solid-state approaches, the synthesis of PNCs for scintillators application is explored comprehensively. Furthermore, embedding strategies within polymeric matrices are scrutinized, shedding light on the various techniques utilized to achieve optimal dispersion and compatibility. The evaluation of the final nanocomposites is finally discussed, with a particular emphasis on their scintillating performance and radiation hardness. Through a meticulous exploration of synthesis methodologies, embedding techniques, and performance assessments, this Review aims to provide a multilayered understanding of the state-of-the-art in PNC-based nanoscintillators.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Perovskite Materials and Applications · Luminescence Properties of Advanced Materials · Radiation Detection and Scintillator Technologies

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Dipartimento di Scienza dei Materiali, Università degli Studi di Milano-Bicocca, via Roberto Cozzi 55, 20125 Milano, Italy

Department of Physics, School of Advanced Sciences, Vellore Institute of Technology, Vellore, Tamil Nadu 632007, India

Funding

HORIZON EUROPE European Innovation Council · Ministero dell'Universit? e della Ricerca

References (100+)

Show source-provided references
1. Bradley W. G. · Proc. Am. Philos. Soc. · 2008 · 152 · 349
2. 10.1007/s13534-011-0019-610.1007/s13534-011-0019-6 ↗
3. 10.3390/app1115707310.3390/app11157073 ↗
4. 10.1016/j.nima.2008.03.01610.1016/j.nima.2008.03.016 ↗
5. 10.1038/s41467-022-32402-010.1038/s41467-022-32402-0 ↗
6. Faderl, N.Fast decay solid-state scintillators for high-speed x-ray imaging; SPIE, 2019; pp 54–71.10.1117/12.2532017 ↗
7. 10.3390/cryst1106066910.3390/cryst11060669 ↗
8. 10.1103/RevModPhys.75.124310.1103/RevModPhys.75.1243 ↗
9. Knoll G. F. · 2010
10. Birks J. B. · 2013 · 27
11. 10.1038/s41586-018-0451-110.1038/s41586-018-0451-1 ↗
12. 10.1038/nmat492710.1038/nmat4927 ↗
13. 10.1016/j.nima.2016.02.04510.1016/j.nima.2016.02.045 ↗
14. 10.1134/S106377961901002710.1134/S1063779619010027 ↗
15. 10.1038/s41565-020-0683-810.1038/s41565-020-0683-8 ↗
16. 10.1038/s41699-019-0120-810.1038/s41699-019-0120-8 ↗
17. 10.1088/1748-0221/11/10/P1001510.1088/1748-0221/11/10/P10015 ↗
18. 10.1021/ja036939c10.1021/ja036939c ↗
19. 10.1002/adfm.20150143910.1002/adfm.201501439 ↗
20. 10.1021/ja042801y10.1021/ja042801y ↗
21. 10.1002/chem.20060107210.1002/chem.200601072 ↗
22. 10.1021/ja00072a02510.1021/ja00072a025 ↗
23. 10.1021/ja970754m10.1021/ja970754m ↗
24. 10.1038/nature0396810.1038/nature03968 ↗
25. 10.1021/acs.nanolett.2c0297510.1021/acs.nanolett.2c02975 ↗
26. 10.1002/adom.20220041910.1002/adom.202200419 ↗
27. 10.1007/s12200-020-1003-510.1007/s12200-020-1003-5 ↗
28. 10.1002/adma.20180174310.1002/adma.201801743 ↗
29. 10.1021/acsami.9b0242510.1021/acsami.9b02425 ↗
30. 10.1039/D1TC01595H10.1039/D1TC01595H ↗
31. 10.1038/s43246-023-00348-510.1038/s43246-023-00348-5 ↗
32. 10.1021/nl504877910.1021/nl5048779 ↗
33. 10.1038/nphoton.2015.8210.1038/nphoton.2015.82 ↗
34. 10.1002/aelm.20180023710.1002/aelm.201800237 ↗
35. 10.1002/adma.20197021410.1002/adma.201970214 ↗
36. 10.1038/nature2403210.1038/nature24032 ↗
37. 10.1038/nphoton.2016.13910.1038/nphoton.2016.139 ↗
38. 10.1038/nphoton.2016.4110.1038/nphoton.2016.41 ↗
39. 10.1038/s41467-018-04073-310.1038/s41467-018-04073-3 ↗
40. 10.1002/advs.20200209810.1002/advs.202002098 ↗
41. 10.1021/acsenergylett.2c0003110.1021/acsenergylett.2c00031 ↗
42. 10.1039/C8EE03395A10.1039/C8EE03395A ↗
43. 10.1038/s41467-022-31569-w10.1038/s41467-022-31569-w ↗
44. 10.1016/j.trechm.2021.03.00510.1016/j.trechm.2021.03.005 ↗
45. 10.1021/acsnano.0c0890310.1021/acsnano.0c08903 ↗
46. 10.1002/aenm.20200134910.1002/aenm.202001349 ↗
47. 10.1038/nenergy.2016.19410.1038/nenergy.2016.194 ↗
48. 10.1016/j.jlumin.2019.11702310.1016/j.jlumin.2019.117023 ↗
49. 10.1021/acs.jpcc.1c0339210.1021/acs.jpcc.1c03392 ↗
50. 10.1002/cplu.20180001410.1002/cplu.201800014 ↗
51. 10.1126/science.abq361610.1126/science.abq3616 ↗
52. 10.1021/acs.chemrev.8b0064410.1021/acs.chemrev.8b00644 ↗
53. 10.1021/acs.accounts.0c0074110.1021/acs.accounts.0c00741 ↗
54. 10.1021/acs.accounts.3c0017410.1021/acs.accounts.3c00174 ↗
55. 10.1002/admi.20170166210.1002/admi.201701662 ↗
56. 10.1007/s10967-017-5562-x10.1007/s10967-017-5562-x ↗
57. 10.1021/acsnano.8b0948410.1021/acsnano.8b09484 ↗
58. 10.1007/s40820-019-0283-z10.1007/s40820-019-0283-z ↗
59. 10.1021/acsenergylett.1c0192310.1021/acsenergylett.1c01923 ↗
60. 10.1016/j.nima.2015.08.04110.1016/j.nima.2015.08.041 ↗
61. 10.1038/nphoton.2017.4310.1038/nphoton.2017.43 ↗
62. 10.1016/j.phpro.2017.09.01210.1016/j.phpro.2017.09.012 ↗
63. 10.1021/acsenergylett.3c0139610.1021/acsenergylett.3c01396 ↗
64. 10.1021/nl501627e10.1021/nl501627e ↗
65. 10.1038/nphoton.2014.5410.1038/nphoton.2014.54 ↗
66. 10.1038/nnano.2015.17810.1038/nnano.2015.178 ↗
67. 10.1021/acsenergylett.2c0007510.1021/acsenergylett.2c00075 ↗
68. 10.1021/acs.chemmater.8b0306610.1021/acs.chemmater.8b03066 ↗
69. 10.1021/acsenergylett.7b0070110.1021/acsenergylett.7b00701 ↗
70. 10.1021/jacs.6b0808510.1021/jacs.6b08085 ↗
71. 10.1021/acs.jpclett.9b0018210.1021/acs.jpclett.9b00182 ↗
72. 10.1021/acsenergylett.7b0017710.1021/acsenergylett.7b00177 ↗
73. 10.1002/adma.20170009510.1002/adma.201700095 ↗
74. 10.1021/acsenergylett.6b0074110.1021/acsenergylett.6b00741 ↗
75. 10.1021/acs.jpclett.0c0037210.1021/acs.jpclett.0c00372 ↗
76. 10.1021/acs.jpclett.9b0059910.1021/acs.jpclett.9b00599 ↗
77. 10.1002/anie.20191447310.1002/anie.201914473 ↗
78. 10.1021/acsomega.2c0171210.1021/acsomega.2c01712 ↗
79. 10.1002/adma.20170414910.1002/adma.201704149 ↗
80. 10.1021/jacs.9b0996910.1021/jacs.9b09969 ↗
81. 10.1021/acsnano.0c0638110.1021/acsnano.0c06381 ↗
82. 10.1021/acsnano.9b0611410.1021/acsnano.9b06114 ↗
83. 10.1039/D0NR00772B10.1039/D0NR00772B ↗
84. 10.1039/D1NR08120A10.1039/D1NR08120A ↗
85. 10.1002/adma.20210252910.1002/adma.202102529 ↗
86. 10.1002/adfm.20210233410.1002/adfm.202102334 ↗
87. 10.1002/adom.20200213010.1002/adom.202002130 ↗
88. 10.1016/j.apmt.2020.10091510.1016/j.apmt.2020.100915 ↗
89. 10.1038/s41467-018-03162-710.1038/s41467-018-03162-7 ↗
90. 10.1002/anie.20200695610.1002/anie.202006956 ↗
91. 10.1002/adom.20210129710.1002/adom.202101297 ↗
92. 10.1016/j.solener.2020.09.01810.1016/j.solener.2020.09.018 ↗
93. 10.1021/acsenergylett.2c0206210.1021/acsenergylett.2c02062 ↗
94. 10.1021/acsenergylett.3c0023410.1021/acsenergylett.3c00234 ↗
95. 10.1039/D0TA12365J10.1039/D0TA12365J ↗
96. 10.1038/s41566-022-01103-x10.1038/s41566-022-01103-x ↗
97. 10.1038/s41566-021-00766-210.1038/s41566-021-00766-2 ↗
98. 10.1021/acs.chemrev.8b0047710.1021/acs.chemrev.8b00477 ↗
99. 10.1038/nnano.2016.11010.1038/nnano.2016.110 ↗
100. 10.1002/adma.20167024210.1002/adma.201670242 ↗