journal article·2020-09-11

High-Performance Perovskite Single-Junction and Textured Perovskite/Silicon Tandem Solar Cells via Slot-Die-Coating

Anand S. Subbiah, Furkan H. Isikgor, Calvyn T. Howells, Michele De Bastiani, Jiang Liu, Erkan Aydin, Francesco Furlan, Thomas G. Allen, Fuzong Xu, Shynggys Zhumagali, Sjoerd Hoogland, Edward H. Sargent, Iain McCulloch, Stefaan De Wolf

ACS Energy Letters· Volume 5· Issue 9
Publisher page

Abstract

In this work, we report perovskite solar cells in the planar p–i–n configuration based on single-step, anti-solvent-free, low-temperature (70 °C) slot-die-coated methylammonium lead tri-iodide (MAPbI3). The devices are fabricated on hydrophobic poly(triarylamine) (PTAA) surfaces, using key strategies such as solvent engineering, enhanced ink–substrate dynamics, and surface passivation, enabling a power conversion efficiency (PCE) of 21.8%. We also adapted the technique to achieve the first slot-die-coated perovskite/silicon monolithic 2-terminal tandems, achieving a PCE of 23.8% utilizing a textured silicon bottom cell.
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Research context

OpenAlex topics: Perovskite Materials and Applications · Conducting polymers and applications · Organic Electronics and Photovoltaics

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

KAUST Solar Center (KSC), Division of Physical Sciences and Engineering (PSE), King Abdullah University of Science and Technology (KAUST), Thuwal 23955-6900, Saudi Arabia

QD Solar Inc., MaRS Center, 661 University Avenue, Toronto, Ontario M5G 1M1, Canada

Department of Electrical and Computer Engineering, University of Toronto, Toronto, Ontario M5S 1A4, Canada

Department of Chemistry, Chemistry Research Laboratory, University of Oxford, Oxford, OX1 3TA, United Kingdom

Funding

King Abdullah University of Science and Technology · QD Solar, Inc

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