journal article·2018-09

PEDOT:PSS Modification by blending graphene oxide to improve the efficiency of organic solar cells

Yishan Wang, Haowei Wang, Junfeng Xu, Bo He, Weile Li, Qi Wang, Shengyi Yang, Bingsuo Zou

Polymer Composites· Volume 39· Issue 9
Publisher page

Abstract

In this work, we present a simple method to modify poly(3,4‐ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS) by directly blending graphene oxide (GO) into PEDOT:PSS to form (PEDOT:PSS):GO nanocomposite and it shows an enhanced conductivity than that of pristine PEDOT:PSS due to the benzoid‐quinoid structure transition of PEDOT:PSS. By applying the obtained nanocomposite (PEDOT:PSS):GO film as the hole‐transporting layer (HTL) in organic solar cells (OSCs) ITO/HTL/active‐layer/Ca/Al, in which the active layer consists of poly(3‐hexylthiophene‐2,5‐diyl) (P3HT):[6,6]‐phenyl C61 butyric acid methyl ester (PC61BM) or P3HT:indene‐C60 bisadduct (ICBA), we found that the power conversion efficiency of these two OSCs with P3HT:PC61BM and P3HT:ICBA as the active layer reached to 3.96% and 5.89%, respectively, showing correspondingly enhancement of 14.78% and 9.89% as compared with those of the control devices in which PEDOT:PSS without any modification. Therefore, PEDOT:PSS modified with GO provides an easy way to fabricate stable OSCs with high performance and low cost. POLYM. COMPOS., 39:3066–3072, 2018. © 2017 Society of Plastics Engineers
Source: crossref · Quality: baseline

Research context

OpenAlex topics: Conducting polymers and applications · Organic Electronics and Photovoltaics · Advanced Sensor and Energy Harvesting Materials

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Beijing Key Lab of Nanophotonics and Ultrafine Optoelectronic Systems School of Physics, Beijing Institute of Technology Beijing 100081 People's Republic of China

Kunming Institute of Physics Kunming 650223 People's Republic of China

Beijing Key Lab of Nanophotonics and Ultrafine Optoelectronic Systems School of Materials Science and Engineering, Beijing Institute of Technology Beijing 100081 People's Republic of China

Beijing Key Lab of Nanophotonics and Ultrafine Optoelectronic Systems School of Optoelectronics, Beijing Institute of Technology Beijing 100081 People's Republic of China

State Key Lab of Transducer Technology, Chinese Academy of Sciences Beijing 100081 People's Republic of China

Funding

The Key Project of Chinese National Programs for Fundamental Research and Development · Project of State Key Laboratory of Transducer Technology · Project of the Key Laboratory of Photoelectronic Imaging Technology and System · Beijing Institute of Technology, Ministry of Education of China

References (34)

Show source-provided references
1. 10.1021/am505916q10.1021/am505916q ↗
2. Dou L. · Adv. Mater. · 2013 · 25 · 642
3. 10.1016/j.apsusc.2016.03.08010.1016/j.apsusc.2016.03.080 ↗
4. 10.1002/polb.2360510.1002/polb.23605 ↗
5. 10.1038/nphoton.2015.610.1038/nphoton.2015.6 ↗
6. 10.1002/adma.20110300610.1002/adma.201103006 ↗
7. 10.1039/c2ee02806a10.1039/c2ee02806a ↗
8. 10.12677/NAT.2013.3100110.12677/NAT.2013.31001 ↗
9. 10.1021/am900823b10.1021/am900823b ↗
10. 10.1016/j.orgel.2010.02.01410.1016/j.orgel.2010.02.014 ↗
11. 10.1143/JJAP.44.369510.1143/JJAP.44.3695 ↗
12. 10.1016/j.solmat.2009.10.00510.1016/j.solmat.2009.10.005 ↗
13. 10.1016/j.orgel.2014.08.00710.1016/j.orgel.2014.08.007 ↗
14. 10.1021/jp711838h10.1021/jp711838h ↗
15. 10.1039/c2cc33829g10.1039/c2cc33829g ↗
16. 10.1016/j.apsusc.2010.03.11810.1016/j.apsusc.2010.03.118 ↗
17. 10.1016/j.solmat.2010.08.00410.1016/j.solmat.2010.08.004 ↗
18. 10.1002/adma.20110477110.1002/adma.201104771 ↗
19. 10.1016/j.solmat.2012.09.00210.1016/j.solmat.2012.09.002 ↗
20. 10.1002/adma.20110220710.1002/adma.201102207 ↗
21. 10.1007/s10965-009-9360-110.1007/s10965-009-9360-1 ↗
22. 10.1016/S0379-6779(99)00271-410.1016/S0379-6779(99)00271-4 ↗
23. 10.1007/s11664-012-2162-y10.1007/s11664-012-2162-y ↗
24. 10.1002/polb.1065910.1002/polb.10659 ↗
25. 10.1016/j.carbon.2014.09.02310.1016/j.carbon.2014.09.023 ↗
26. 10.1021/ja01539a01710.1021/ja01539a017 ↗
27. 10.1002/adma.20080316010.1002/adma.200803160 ↗
28. 10.1016/j.polymer.2004.10.00110.1016/j.polymer.2004.10.001 ↗
29. 10.1002/adma.20080289310.1002/adma.200802893 ↗
30. 10.1039/C3TA13647G10.1039/C3TA13647G ↗
31. 10.1021/acs.jpcc.6b1054510.1021/acs.jpcc.6b10545 ↗
32. 10.1016/j.orgel.2016.10.01310.1016/j.orgel.2016.10.013 ↗
33. 10.1021/am506326y10.1021/am506326y ↗
34. 10.1021/am405148710.1021/am4051487 ↗