DataVXACS Applied Nano MaterialsPaper
journal article·2020-12-24

Hierarchical Structures from Nanocrystalline Colloidal Precursors within Hybrid Perovskite Thin Films: Implications for Photovoltaics

Shambhavi Pratap, Johannes Schlipf, Lorenz Bießmann, Peter Müller-Buschbaum

ACS Applied Nano Materials· Volume 3· Issue 12
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Source abstract

Abstract

Originating from stochastic nanocrystalline colloidal precursors with differential chemical compositions, crystalline thin films exhibit hierarchical structures originating at the crystallographic level and scaling up to mesoscale structures, manifested within their nanocrystalline morphology and mesoscale topology. We interlink morphogenetic signatures within thin films to differential precursor chemistry and explain the cooperative impact of structure-defining inorganic and organic counterparts on perovskite hybrids. Understanding the effect of chemical species on the structural characteristics of thin films and leveraging complex assembly processes present facile routes to tuning multiscale morphologies in thin films, pertinent for engineering functional performance metrics within thin-film perovskite photovoltaics.
Source: openalex_inverted_index · Quality: baseline

Research context

NanomaterialsElectronic materials

OpenAlex topics: Perovskite Materials and Applications · Quantum Dots Synthesis And Properties · Chalcogenide Semiconductor Thin Films

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Physik-Department, Lehrstuhl für Funktionelle Materialien, Technische Universität München (TUM), James-Franck-Straße 1, 85748 Garching, Germany

Advanced Light Source, Lawrence Berkeley National Laboratory, 1 Cyclotron Road, Berkeley, California 94720, United States

Heinz Maier-Leibnitz Zentrum, Technische Universität München (TUM), Lichtenbergstraße 1, 85748 Garching, Germany

Funding

European Commission · Deutsche Forschungsgemeinschaft · Bayerisches Staatsministerium f?r Wissenschaft, Forschung und Kunst · TUM International Graduate School of Science and Engineering (IGSSE) · Centre for NanoScience (CeNS)

References (30)

Show source-provided references
1. 10.1021/ja809598r10.1021/ja809598r ↗
2. 10.1016/j.joule.2020.07.00410.1016/j.joule.2020.07.004 ↗
3. 10.1039/C7EE00757D10.1039/C7EE00757D ↗
4. Jean, J.; Brown, P. R. Emerging Photovoltaic Technologies; IOP Publishing, 2020; pp 2053–2563.10.1088/978-0-7503-2152-5 ↗
5. 10.1002/smtd.20170031010.1002/smtd.201700310 ↗
6. 10.1021/nl500390f10.1021/nl500390f ↗
7. 10.1002/adma.20130628110.1002/adma.201306281 ↗
8. 10.1021/acs.chemrev.6b0013610.1021/acs.chemrev.6b00136 ↗
9. 10.1039/C6EE00030D10.1039/C6EE00030D ↗
10. 10.1038/nenergy.2016.9310.1038/nenergy.2016.93 ↗
11. 10.1021/acs.jpclett.5b0184310.1021/acs.jpclett.5b01843 ↗
12. 10.1039/C8TA04120B10.1039/C8TA04120B ↗
13. 10.1021/acs.jpclett.0c0197510.1021/acs.jpclett.0c01975 ↗
14. 10.1038/nmat401410.1038/nmat4014 ↗
15. 10.1021/acs.jpcc.5b1146910.1021/acs.jpcc.5b11469 ↗
16. 10.1002/aenm.20170013110.1002/aenm.201700131 ↗
17. 10.1039/c3sm53214c10.1039/c3sm53214c ↗
18. 10.1038/s41578-019-0125-010.1038/s41578-019-0125-0 ↗
19. 10.1038/s41563-019-0379-310.1038/s41563-019-0379-3 ↗
20. 10.1039/C5SM01724F10.1039/C5SM01724F ↗
21. 10.1103/PhysRevLett.121.08550210.1103/PhysRevLett.121.085502 ↗
22. 10.1021/acs.chemrev.6b0019610.1021/acs.chemrev.6b00196 ↗
23. 10.1039/C8NR09853K10.1039/C8NR09853K ↗
24. 10.1021/acs.accounts.5b0044010.1021/acs.accounts.5b00440 ↗
25. 10.1039/C5TA09992G10.1039/C5TA09992G ↗
26. 10.1021/acsenergylett.8b0054410.1021/acsenergylett.8b00544 ↗
27. 10.1107/S010876731909844110.1107/S0108767319098441 ↗
28. 10.1016/j.prostr.2016.06.34810.1016/j.prostr.2016.06.348 ↗
29. 10.1039/C9CP01088B10.1039/C9CP01088B ↗
30. 10.1038/s41467-018-03757-010.1038/s41467-018-03757-0 ↗