journal article·2023-10-13

Room-Temperature NO2 Detection by MoS2–Nanoflake-Decorated AuPt/SnO2 Nanotubes

Weiqi Wang, Jiamu Cao, Rongji Zhang, Huaxin Xiu, Yufeng Zhang

ACS Applied Nano Materials· Volume 6· Issue 19
Publisher page

Abstract

Although SnO 2 nanomaterials have been leading components of semiconductor gas sensors, their long-standing challenges of high working temperatures limit their practical application for ultralow-power-consumption room-temperature sensing. In this study, Au and Pt bimetallic nanoparticles were used to fabricate a MoS 2 /AuPt/SnO 2 nanocomposite device by interfacially engineering a MoS 2 /SnO 2 nanostructure. Owing to the unique structure and electrical properties, the as-fabricated MoS 2 /AuPt/SnO 2 device exhibits a remarkable sensing response (2.22), short response time (20 s), and excellent baseline recovery (8 s) to 10 ppm NO 2 gas at 23 ± 2 °C. Meanwhile, the MoS 2 /AuPt/SnO 2 device possesses high sensitivity, a low detection limit (20 ppb), commendable reversibility, appreciable stability, and excellent selectivity against ammonia, carbon monoxide, ethanol, isopropanol, and acetone gases. The superior sensing characteristics of the MoS 2 /AuPt/SnO 2 nanocomposite device are attributed to the modulation effect of the Schottky junction and p–n heterojunction on the potential barrier, highly efficient interfacial electron transport, and edge-enriched structure, which provide abundant active adsorption sites. This work will advance the evolution of room-temperature gas-sensitive nanomaterials and render them promising for applications in ultralow power-integrated sensors.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Gas Sensing Nanomaterials and Sensors · Transition Metal Oxide Nanomaterials · Analytical Chemistry and Sensors

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

School of Astronautics, Harbin Institute of Technology, Harbin 150001, China

Optical Engineering, Harbin Institute of Technology, Harbin 150001, China

Key Laboratory of Micro-Systems and Micro-Structures Manufacturing, Ministry of Education, Harbin 150001, China

Funding

China Postdoctoral Science Foundation · Heilongjiang Provincial Postdoctoral Science Foundation · Fundamental Research Funds for the Central Universities · National Natural Science Foundation of China

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