journal article·2018-04Open access

Towards sensitive terahertz detection via thermoelectric manipulation using graphene transistors

Changlong Liu, Lei Du, Weiwei Tang, Dacheng Wei, Jinhua Li, Lin Wang, Gang Chen, Xiaoshuang Chen, Wei Lu

NPG Asia Materials· Volume 10· Issue 4

Abstract

Graphene has been highly sought after as a potential candidate for hot-electron terahertz (THz) detection benefiting from its strong photon absorption, fast carrier relaxation, and weak electron-phonon coupling. Nevertheless, to date, graphene-based thermoelectric THz photodetection is hindered by low responsivity owing to relatively low photoelectric efficiency. In this work, we provide a straightforward strategy for enhanced THz detection based on antenna-coupled CVD graphene transistors with the introduction of symmetric paired fingers. This design enables switchable photodetection modes by controlling the interaction between the THz field and free hot carriers in the graphene-channel through different contacting configurations. Hence a novel “bias-field effect” can be activated, which leads to a drastic enhancement in THz detection ability with maximum responsivity of up to 280 V/W at 0.12 THz relative to the antenna area and a Johnson-noise limited minimum noise-equivalent power (NEP) of 100 pW/Hz0.5 at room temperature. The mechanism responsible for the enhancement in the photoelectric gain is attributed to thermophotovoltaic instead of plasma self-mixing effects. Our results offer a promising alternative route toward scalable, wafer-level production of high-performance graphene detectors. Controlling how finger-like electrodes are positioned on graphene transistors makes it simpler to detect terahertz radiation for applications including medical diagnostics. When photons strike graphene sheets, multiple electrons with high kinetic energy are released. Changlong Liu at the Chinese Academy of Sciences, Shanghai, and coworkers have exploited these electrons to improve detection of terahertz light, which is useful for seeing features underneath human skin. The team’s device places single-layer graphene into a channel flanked by two microscale antennas, and then adds a pair of thin metal fingers on top of the 2D carbon film. By manipulating the separation of the finger contacts, the team unlocked an enhanced response to terahertz light at room temperature. Experiments and simulations revealed that temperature gradients between contact points generated a terahertz-sensitive photocurrent through conversion of heat into electricity. Graphene is very promising for THz application, especially in the fields desiring fast THz imaging, like security screening, communication, biomedical and pharmacy control. However, current graphene-based THz detectors are severely hindered by its poor switching behavior, and lack of internal gain to boost up the responsivity in the framework of plasma-wave self-mixing or thermoelectric detections. A proper means to selectively trigger the photoelectric conversion is highly desirable for practical applications. This work offers alternative way for room temperature THz detection via manipulating the hot carriers either electrically and electromagnetically. Internal photoelectric gain is achieved via the bias-field effect, which leads to the giant enhancement of graphene-based detector’s responsivity over 200 V/W. Furthermore, switching behavior between photoconductive and photovoltaic modes can be given rise in a single device, being promising for scalable THz imaging.
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Research context

OpenAlex topics: Thermal Radiation and Cooling Technologies · Plasmonic and Surface Plasmon Research · Topological Materials and Phenomena

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (38)

Show source-provided references
1. Ju, L. et al. Topological valley transport at bilayer graphene domain walls. Nature 520, 650–655 (2015).10.1038/nature14364 ↗
2. Sui, M. et al. Gate-tunable topological valley transport in bilayer graphene. Nat. Phys. 11, 1027–1031 (2015).10.1038/nphys3485 ↗
3. Giorgianni, F. et al. Strong nonlinear terahertz response induced by Dirac surface states in Bi2Se3 topological insulator. Nat. Commun. 7, 11421 (2016).10.1038/ncomms11421 ↗
4. Mak, K. F., McGill, K. L., Park, J. & McEuen, P. L. The valley Hall effect in MoS2 transistors. Science 344, 1489–1492 (2014).10.1126/science.1250140 ↗
5. Chen, S., Zheng, C., Fuhrer, M. S. & Yan, J. Helicity-resolved Raman scattering of MoS2, MoSe2, WS2, and WSe2 atomic layers. Nano Lett. 15, 2526–2532 (2015).10.1021/acs.nanolett.5b00092 ↗
6. Lu, J. M. et al. Evidence for two-dimensional lsing superconductivity in gated MoS2. Science 350, 1353–1357 (2015).10.1126/science.aab2277 ↗
7. Navarro-Moratalla, E. et al. Enhanced superconductivity in atomically thin TaS2. Nat. Commun. 7, 11043 (2016).10.1038/ncomms11043 ↗
8. Koppens, F. H. L. et al. Photodetectors based on graphene, other two-dimensional materials and hybrid systems. Nat. Nanotechnol. 9, 780–793 (2014).10.1038/nnano.2014.215 ↗
9. Grigorenko, A. N., Polini, M. & Novoselov, K. S. Grapheneplasmonics. Nat. Photonics 6, 749–758 (2012).10.1038/nphoton.2012.262 ↗
10. Lundeberg, M. B. et al. Tuning quantum nonlocal effects in grapheneplasmonics. Science 357, 187–191 (2017).10.1126/science.aan2735 ↗
11. Basov, D. N., Fogler, M. M. & García de Abajo, F. J. Polaritons in van der Waals materials. Science 354, 195 (2016).10.1126/science.aag1992 ↗
12. Choi, W. et al. High-detectivity multilayer MoS2 phototransistors with spectral response from ultraviolet to infrared. Adv. Mat. 24, 5832–5837 (2012).10.1002/adma.201201909 ↗
13. Jariwala, D. et al. Hybrid, gate-tunable, van der Waals p-n heterojunctions from pentacene and MoS2. Nano Lett. 16, 497–503 (2016).10.1021/acs.nanolett.5b04141 ↗
14. Buscema, M. et al. Photocurrent generation with two-dimensional van der Waals semiconductors. Chem. Soc. Rev. 44, 3691–3718 (2015).10.1039/C5CS00106D ↗
15. Freitag, M., Low, T., Xia, F. & Avouris, P. Photoconductivity of biased graphene. Nat. Photonics 7, 53–59 (2013).10.1038/nphoton.2012.314 ↗
16. Yao, Y. et al. High-responsivity mid-infrared graphene detectors with antenna-enhanced photocarrier generation and collection. Nano Lett. 14, 3749–3754 (2014).10.1021/nl500602n ↗
17. Yao, Y. et al. Wide wavelength tuning of optical antennas on graphene with nanosecond response time. Nano Lett. 14, 214–219 (2014).10.1021/nl403751p ↗
18. Tong, J., Muthee, M., Chen, S., Yngvesson, S. K. & Yan, J. Antenna enhanced graphene THz emitter and detector. Nano Lett. 15, 5295–5301 (2015).10.1021/acs.nanolett.5b01635 ↗
19. Ghahari, F. et al. Enhanced thermoelectric power in graphene: violation of the Mott relation by inelastic scattering. Phys. Rev. Lett. 116, 136802 (2016).10.1103/PhysRevLett.116.136802 ↗
20. Viti, L. et al. Heterostructured hBN-BP-hBN nanodetectors at terahertz frequencies. Adv. Mat. 28, 7390–7396 (2016).10.1002/adma.201601736 ↗
21. Viti, L. et al. Black phosphorus terahertz photodetectors. Adv. Mat. 27, 5567–5572 (2015).10.1002/adma.201502052 ↗
22. Vicarelli, L. et al. Graphene field-effect transistors as room-temperature terahertz detectors. Nat. Mater. 11, 865–871 (2012).10.1038/nmat3417 ↗
23. Otsuji, T. & Shur, M. S. Terahertz plasmonics: Good results and great expectations. IEEE Microw. Mag. 15, 43–50 (2014).10.1109/MMM.2014.2355712 ↗
24. Tomadin, A., Tredicucci, A., Pellegrini, V., Vitiello, M. S. & Polini, M. Photocurrent-based detection of terahertz radiation in graphene. Appl. Phys. Lett. 103, 211120 (2013).10.1063/1.4831682 ↗
25. Seo, M. A. et al. Terahertz field enhancement by a metallic nano slit operating beyond the skin-depth limit. Nat. Photonics 3, 152–156 (2009).10.1038/nphoton.2009.22 ↗
26. Viti, L. et al. Efficient terahertz detection in black-phosphorus nano-transistors with selective and controllable plasma-wave, bolometric and thermoelectric response. Sci. Rep. 6, 20474 (2016).10.1038/srep20474 ↗
27. Ghahari, F. et al. Enhanced thermoelectric power in graphene: violation of the Mott relation by inelastic scattering. Phys. Rev. Lett. 116, 136802 (2016).10.1103/PhysRevLett.116.136802 ↗
28. Song, J. C., Rudner, M. S., Marcus, C. M. & Levitov, L. S. Hot carrier transport and photocurrent response in graphene. Nano Lett. 11, 4688–4692 (2011).10.1021/nl202318u ↗
29. Yin, Y., Cheng, Z., Wang, L., Jin, K. & Wang, W. Graphene, a material for high temperature devices-intrinsic carrier density, carrier drift velocity, and lattice energy. Sci. Rep. 4, 5758 (2014).10.1038/srep05758 ↗
30. Zhou, H., Cai, Y., Zhang, G. & Zhang, Y. -W. Quantum thermal transport in stanene. Phys. Rev. B 94, 045423 (2016).10.1103/PhysRevB.94.045423 ↗
31. Cai, X. et al. Sensitive room-temperature terahertz detection via the photothermoelectric effect in graphene. Nat. Nanotechnol. 9, 814–819 (2014).10.1038/nnano.2014.182 ↗
32. Yan, J. et al. Dual-gated bilayer graphene hot-electron bolometer. Nat. Nanotechnol. 7, 472–478 (2012).10.1038/nnano.2012.88 ↗
33. Giovannetti, G. et al. Doping graphene with metal contacts. Phys. Rev. Lett. 101, 026803 (2008).10.1103/PhysRevLett.101.026803 ↗
34. Xia, F., Perebeinos, V., Lin, Y. -M., Wu, Y. & Avouris, P. The origins and limits of metal-graphene junction resistance. Nat. Nanotechnol. 6, 179–184 (2011).10.1038/nnano.2011.6 ↗
35. Sakowicz, M. et al. Terahertz responsivity of field effect transistors versus their static channel conductivity and loading effects. J. Appl. Phys. 110, 054512 (2011).10.1063/1.3632058 ↗
36. Qin, H. et al. Room-temperature, low-impedance and high-sensitivity terahertz direct detector based on bilayer graphene field-effect transistor. Carbon 116, 760–765 (2017).10.1016/j.carbon.2017.02.037 ↗
37. Romeo, L. et al. Nanowire-based field effect transistors for terahertz detection and imaging systems. Nanotechnology 24, 214005 (2013).10.1088/0957-4484/24/21/214005 ↗
38. Konstantatos, G. et al. Hybrid graphene-quantum dot phototransistors with ultrahigh gain. Nat. Nanotechnol. 7, 363–368 (2012).10.1038/nnano.2012.60 ↗