journal article·2022-11-25

Ag-Doped CdSe Nanosheets as Photocatalysts for Uranium Reduction

Guo Li, Changxue Dong, Genshuai Sun, Mingzhe Li, Xin Cao, Li Zhou, Tao Chen, Fan Yang

ACS Applied Nano Materials· Volume 5· Issue 11
Publisher page

Abstract

Doping is a simple method to modulate the electronic configuration of semiconductor photocatalysts. This study regulated the energy band structure of CdSe nanosheets by Ag doping, which reduced the energy bandwidth of CdSe nanosheets by increasing the carrier density, thereby improving the efficiency of the photocatalytic reduction of uranium by CdSe nanosheets. A 96% removal of U(VI) was achieved by 3% Ag-CdSe nanosheets, which was 1.9 and 1.2 times higher than that of pristine CdSe nanosheets (50%), and 1% Ag-CdSe nanosheets (81%), respectively. Additionally, at pH = 4.0 and a solid–liquid ratio of 0.25, the reduction of uranium by 3% Ag-CdSe nanosheets (765 mg/g) was 2.2 times higher than that of pristine CdSe nanosheets (345.6 mg/g). This study provides a new idea for other efficient photocatalysts designed for uranium reduction.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Radioactive element chemistry and processing · Nuclear Materials and Properties · Advanced Photocatalysis Techniques

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang621010, PR China

School of Materials Science and Engineering, Sichuan University, Chengdu610000, PR China

State Key Laboratory of Environment-friendly Energy Materials, National Co-innovation Center for Nuclear Waste Disposal and Environmental Safety, Sichuan Institute of Military and Civilian Integration, Nuclear Waste and Environmental Safety Key Laboratory of Defense, School of Life Science and Engineering, Joint Laboratory for Extreme Conditions Matter Properties, Southwest University of Science and Technology, Mianyang621010, PR China

Funding

Department of Science and Technology of Sichuan Province · National Natural Science Foundation of China · State Key Laboratory of Environmental-friendly Energy Materials

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