journal article·2025-05

Nanometre-resolution three-dimensional tomographic and vectorial near-field imaging in dielectric optical resonators

Bingbing Zhu, Qingnan Cai, Yaxin Liu, Sheng Zhang, Weifeng Liu, Qiong He, Lei Zhou, Zhensheng Tao

Nature Nanotechnology· Volume 20· Issue 5
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Abstract

All-dielectric optical nano-resonators have emerged as low-loss, versatile and highly adaptable components in nanophotonic structures for manipulating electromagnetic waves and enhancing light-matter interactions. However, achieving full three-dimensional characterization of near fields within dielectric nano-resonators poses great experimental challenges. Here we develop a technique to image near-field wave patterns inside dielectric optical nano-resonators using high-order sideband generation. By exploiting the phase sensitivity of various harmonic orders, which enables the detection of near-field distributions at distinct depths, we achieve three-dimensional tomographic and near-field imaging with a transverse resolution of ~920 nm and a longitudinal resolution of ~130 nm inside a micrometre-thick silicon anapole resonator. Our method offers high-contrast polarization sensitivity and phase-resolving capabilities, providing comprehensive vectorial near-field information and could be applied to diverse dielectric metamaterials.
Source: europepmc · Quality: candidate unverified · Source record ↗

Research context

OpenAlex topics: Plasmonic and Surface Plasmon Research · Photonic and Optical Devices · Near-Field Optical Microscopy

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (53)

Show source-provided references
1. O’Brien, S. & Pendry, J. B. Photonic band-gap effects and magnetic activity in dielectric composites. J. Phys. Condens. Matter 14, 4035–4044 (2002).10.1088/0953-8984/14/15/317 ↗
2. Koshelev, K. et al. Subwavelength dielectric resonators for nonlinear nanophotonics. Science 367, 288–292 (2020).10.1126/science.aaz3985 ↗
3. Kuznetsov, A. I., Miroshnichenko, A. E., Brongersma, M. L., Kivshar, Y. S. & Luk’yanchuk, B. Optically resonant dielectric nanostructures. Science 354, aag2472 (2016).10.1126/science.aag2472 ↗
4. Staude, I. & Schilling, J. Metamaterial-inspired silicon nanophotonics. Nat. Photon. 11, 274–284 (2017).10.1038/nphoton.2017.39 ↗
5. Gan, X. et al. High-contrast electrooptic modulation of a photonic crystal nanocavity by electrical gating of graphene. Nano Lett. 13, 691–696 (2013).10.1021/nl304357u ↗
6. Yang, Y., Kravchenko, I. I., Briggs, D. P. & Valentine, J. All-dielectric metasurface analogue of electromagnetically induced transparency. Nat. Commun. 5, 5753 (2014).10.1038/ncomms6753 ↗
7. Lin, D., Fan, P., Hasman, E. & Brongersma, M. L. Dielectric gradient metasurface optical elements. Science 345, 298–302 (2014).10.1126/science.1253213 ↗
8. Chen, Y. et al. Observation of intrinsic chiral bound states in the continuum. Nature 613, 474–478 (2023).10.1038/s41586-022-05467-6 ↗
9. Arbabi, A., Horie, Y., Bagheri, M. & Faraon, A. Dielectric metasurfaces for complete control of phase and polarization with subwavelength spatial resolution and high transmission. Nat. Nanotechnol. 10, 937–943 (2015).10.1038/nnano.2015.186 ↗
10. Koshelev, K. & Kivshar, Y. Dielectric resonant metaphotonics. ACS Photon. 8, 102–112 (2021).10.1021/acsphotonics.0c01315 ↗
11. Dorrah, A. H. & Capasso, F. Tunable structured light with flat optics. Science 376, eabi6860 (2022).10.1126/science.abi6860 ↗
12. Lin, R. J. et al. Achromatic metalens array for full-colour light-field imaging. Nat. Nanotechnol. 14, 227–231 (2019).10.1038/s41565-018-0347-0 ↗
13. West, P. R. et al. All-dielectric subwavelength metasurface focusing lens. Opt. Express 22, 26212 (2014).10.1364/OE.22.026212 ↗
14. Arbabi, A., Horie, Y., Ball, A. J., Bagheri, M. & Faraon, A. Subwavelength-thick lenses with high numerical apertures and large efficiency based on high-contrast transmitarrays. Nat. Commun. 6, 7069 (2015).10.1038/ncomms8069 ↗
15. Arbabi, A. & Faraon, A. Advances in optical metalenses. Nat. Photon. 17, 16–25 (2023).10.1038/s41566-022-01108-6 ↗
16. Kim, M., Lee, D., Yang, Y., Kim, Y. & Rho, J. Reaching the highest efficiency of spin Hall effect of light in the near-infrared using all-dielectric metasurfaces. Nat. Commun. 13, 2036 (2022).10.1038/s41467-022-29771-x ↗
17. Hentschel, M. et al. Dielectric Mie voids: confining light in air. Light Sci. Appl. 12, 3 (2023).10.1038/s41377-022-01015-z ↗
18. Rybin, M. V. et al. High-Q supercavity modes in subwavelength dielectric resonators. Phys. Rev. Lett. 119, 243901 (2017).10.1103/PhysRevLett.119.243901 ↗
19. Odit, M. et al. Observation of supercavity modes in subwavelength dielectric resonators. Adv. Mater. 33, 2003804 (2021).10.1002/adma.202003804 ↗
20. Zhao, Q., Zhou, J., Zhang, F. & Lippens, D. Mie resonance-based dielectric metamaterials. Mater. Today 12, 60–69 (2009).10.1016/S1369-7021(09)70318-9 ↗
21. Hillenbrand, R., Taubner, T. & Keilmann, F. Phonon-enhanced light–matter interaction at the nanometre scale. Nature 418, 159–162 (2002).10.1038/nature00899 ↗
22. Bek, A., Vogelgesang, R. & Kern, K. Apertureless scanning near field optical microscope with sub-10 nm resolution. Rev. Sci. Instrum. 77, 043703 (2006).10.1063/1.2190211 ↗
23. Ma, X. et al. 6 nm super-resolution optical transmission and scattering spectroscopic imaging of carbon nanotubes using a nanometer-scale white light source. Nat. Commun. 12, 6868 (2021).10.1038/s41467-021-27216-5 ↗
24. Moon, K. et al. Subsurface nanoimaging by THz pulse near-field microscopy. Nano Lett. 15, 549–552 (2015).10.1021/nl503998v ↗
25. Polman, A., Kociak, M. & García de Abajo, F. J. Electron-beam spectroscopy for nanophotonics. Nat. Mater. 18, 1158–1171 (2019).10.1038/s41563-019-0409-1 ↗
26. Nelayah, J. et al. Mapping surface plasmons on a single metallic nanoparticle. Nat. Phys. 3, 348–353 (2007).10.1038/nphys575 ↗
27. Vesseur, E. J. R., De Waele, R., Kuttge, M. & Polman, A. Direct observation of plasmonic modes in Au nanowires using high-resolution cathodoluminescence spectroscopy. Nano Lett. 7, 2843–2846 (2007).10.1021/nl071480w ↗
28. Spektor, G. et al. Revealing the subfemtosecond dynamics of orbital angular momentum in nanoplasmonic vortices. Science 355, 1187–1191 (2017).10.1126/science.aaj1699 ↗
29. Dai, Y. et al. Plasmonic topological quasiparticle on the nanometre and femtosecond scales. Nature 588, 616–619 (2020).10.1038/s41586-020-3030-1 ↗
30. Piazza, L. et al. Simultaneous observation of the quantization and the interference pattern of a plasmonic near-field. Nat. Commun. 6, 6407 (2015).10.1038/ncomms7407 ↗
31. Barwick, B., Flannigan, D. J. & Zewail, A. H. Photon-induced near-field electron microscopy. Nature 462, 902–906 (2009).10.1038/nature08662 ↗
32. Harutyunyan, H., Palomba, S., Renger, J., Quidant, R. & Novotny, L. Nonlinear dark-field microscopy. Nano Lett. 10, 5076–5079 (2010).10.1021/nl1033304 ↗
33. Constant, T. J., Hornett, S. M., Chang, D. E. & Hendry, E. All-optical generation of surface plasmons in graphene. Nat. Phys. 12, 124–127 (2016).10.1038/nphys3545 ↗
34. Palomba, S., Danckwerts, M. & Novotny, L. Nonlinear plasmonics with gold nanoparticle antennas. J. Opt. A 11, 114030 (2009).10.1088/1464-4258/11/11/114030 ↗
35. Schlickriede, C. et al. Imaging through nonlinear metalens using second harmonic generation. Adv. Mater. 30, 1703843 (2018).10.1002/adma.201703843 ↗
36. Ali, R. F., Busche, J. A., Kamal, S., Masiello, D. J. & Gates, B. D. Near-field enhancement of optical second harmonic generation in hybrid gold–lithium niobate nanostructures. Light Sci. Appl. 12, 99 (2023).10.1038/s41377-023-01092-8 ↗
37. Metzger, B., Hentschel, M. & Giessen, H. Probing the near-field of second-harmonic light around plasmonic nanoantennas. Nano Lett. 17, 1931–1937 (2017).10.1021/acs.nanolett.6b05285 ↗
38. Grinblat, G., Li, Y., Nielsen, M. P., Oulton, R. F. & Maier, S. A. Efficient third harmonic generation and nonlinear subwavelength imaging at a higher-order anapole mode in a single germanium nanodisk. ACS Nano 11, 953–960 (2017).10.1021/acsnano.6b07568 ↗
39. Zheng, Z. et al. Third-harmonic generation and imaging with resonant Si membrane metasurface. Opto-Electron. Adv. 6, 220174 (2023).10.29026/oea.2023.220174 ↗
40. Frischwasser, K. et al. Real-time sub-wavelength imaging of surface waves with nonlinear near-field optical microscopy. Nat. Photon. 15, 442–448 (2021).10.1038/s41566-021-00782-2 ↗
41. Wang, Y., Lin, C.-Y., Nikolaenko, A., Raghunathan, V. & Potma, E. O. Four-wave mixing microscopy of nanostructures. Adv. Opt. Photon. 3, 1–52 (2011).10.1364/AOP.3.000001 ↗
42. Langer, F. et al. Lightwave-driven quasiparticle collisions on a subcycle timescale. Nature 533, 225–229 (2016).10.1038/nature17958 ↗
43. Zaks, B., Liu, R. B. & Sherwin, M. S. Experimental observation of electron-hole recollisions. Nature 483, 580–583 (2012).10.1038/nature10864 ↗
44. Liu, R.-B. & Zhu, B.-F. High-order THz-sideband generation in semiconductors. AIP Conf. Proc. 893, 1455–1456 (2007).10.1063/1.2730455 ↗
45. Miroshnichenko, A. E. et al. Nonradiating anapole modes in dielectric nanoparticles. Nat. Commun. 6, 8069 (2015).10.1038/ncomms9069 ↗
46. Wu, P. C. et al. Optical anapole metamaterial. ACS Nano 12, 1920–1927 (2018).10.1021/acsnano.7b08828 ↗
47. Papasimakis, N., Fedotov, V. A., Savinov, V., Raybould, T. A. & Zheludev, N. I. Electromagnetic toroidal excitations in matter and free space. Nat. Mater. 15, 263–271 (2016).10.1038/nmat4563 ↗
48. Liu, Y. et al. Dephasing of strong-field-driven excitonic autler-townes doublets revealed by time- and spectrum-resolved quantum-path interferometry. Phys. Rev. Lett. 133, 026901 (2024).10.1103/PhysRevLett.133.026901 ↗
49. Shanblatt, E. R. et al. Quantitative chemically specific coherent diffractive imaging of reactions at buried interfaces with few nanometer precision. Nano Lett. 16, 5444–5450 (2016).10.1021/acs.nanolett.6b01864 ↗
50. Dai, S. et al. Tunable phonon polaritons in atomically thin van der Waals crystals of boron nitride. Science 343, 1125–1129 (2014).10.1126/science.1246833 ↗
51. Ma, W. et al. Ghost hyperbolic surface polaritons in bulk anisotropic crystals. Nature 596, 362–366 (2021).10.1038/s41586-021-03755-1 ↗
52. Hafezi, M., Mittal, S., Fan, J., Migdall, A. & Taylor, J. M. Imaging topological edge states in silicon photonics. Nat. Photon. 7, 1001–1005 (2013).10.1038/nphoton.2013.274 ↗
53. Peng, S. et al. Probing the band structure of topological silicon photonic lattices in the visible spectrum. Phys. Rev. Lett. 122, 117401 (2019).10.1103/PhysRevLett.122.117401 ↗