journal article·2009-03Open access

Engineering the coupling between molecular spin qubits by coordination chemistry

Grigore A. Timco, Stefano Carretta, Filippo Troiani, Floriana Tuna, Robin J. Pritchard, Christopher A. Muryn, Eric J. L. McInnes, Alberto Ghirri, Andrea Candini, Paolo Santini, Giuseppe Amoretti, Marco Affronte, Richard E. P. Winpenny

Nature Nanotechnology· Volume 4· Issue 3

Abstract

The ability to assemble weakly interacting subsystems is a prerequisite for implementing quantum information processing and generating controlled entanglement. In recent years, molecular nanomagnets have been proposed as suitable candidates for qubit encoding and manipulation. In particular, antiferromagnetic Cr7Ni rings behave as effective spin-1/2 systems at low temperature and show long decoherence times. Here, we show that these rings can be chemically linked to each other and that the coupling between their spins can be tuned by choosing the linker. We also present calculations that demonstrate how realistic microwave pulse sequences could be used to generate maximally entangled states in such molecules.
Source: europepmc · Quality: candidate unverified · Source record ↗

Research context

OpenAlex topics: Magnetism in coordination complexes · Quantum and electron transport phenomena · Advanced NMR Techniques and Applications

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

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