Overcoming efficiency and cost barriers for large-area quantum dot photovoltaics through stable ink engineering
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OpenAlex topics: Quantum Dots Synthesis And Properties · Nanowire Synthesis and Applications · Chalcogenide Semiconductor Thin Films
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References (74)
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1. Kagan, C. R., Lifshitz, E., Sargent, E. H. & Talapin, D. V. Building devices from colloidal quantum dots. Science 353, aac5523 (2016).10.1126/science.aac5523 ↗
2. García de Arquer, F. P. et al. Semiconductor quantum dots: technological progress and future challenges. Science 373, eaaz8541 (2021).10.1126/science.aaz8541 ↗
3. Boles, M. A., Ling, D., Hyeon, T. & Talapin, D. V. Erratum: the surface science of nanocrystals. Nat. Mater. 15, 364 (2016).10.1038/nmat4578 ↗
4. Liu, M. et al. Colloidal quantum dot electronics. Nat. Electron. 4, 548–558 (2021).10.1038/s41928-021-00632-7 ↗
5. Choi, M. J. et al. Tuning solute-redistribution dynamics for scalable fabrication of colloidal quantum-dot optoelectronics. Adv. Mater. 31, e1805886 (2019).10.1002/adma.201805886 ↗
6. Aqoma, H. & Jang, S.-Y. Solid-state-ligand-exchange free quantum dot ink-based solar cells with an efficiency of 10.9. Energy Environ. Sci. 11, 1603–1609 (2018).10.1039/C8EE00278A ↗
7. Wang, W. et al. Colloidal inorganic ligand-capped nanocrystals: fundamentals, status, and insights into advanced functional nanodevices. Chem. Rev. 122, 4091–4162 (2021).10.1021/acs.chemrev.1c00478 ↗
8. Pejovic, V. et al. Infrared colloidal quantum dot image sensors. IEEE Trans. Electron Devices 69, 2840–2850 (2022).10.1109/TED.2021.3133191 ↗
9. Frimova, A., Pekarovicova, A., Fleming, P. D. & Pekarovic, J. Ink stability during printing. TAGA J. 2, 122–131 (2005).
10. Liu, Y., Shi, G., Liu, Z. & Ma, W. Toward printable solar cells based on PbX colloidal quantum dot inks. Nanoscale Horiz. 6, 8–23 (2021).10.1039/D0NH00488J ↗
11. Xie, C. et al. Overcoming efficiency and stability limits in water-processing nanoparticular organic photovoltaics by minimizing microstructure defects. Nat. Commun. 9, 5335 (2018).10.1038/s41467-018-07807-5 ↗
12. YousefiAmin, A. et al. Fully printed infrared photodetectors from PbS nanocrystals with perovskite ligands. ACS Nano 13, 2389–2397 (2019).
13. Abelson, A. et al. Collective topo-epitaxy in the self-assembly of a 3D quantum dot superlattice. Nat. Mater. 19, 49–55 (2020).10.1038/s41563-019-0485-2 ↗
14. Yazdani, N. et al. Charge transport in semiconductors assembled from nanocrystal quantum dots. Nat. Commun. 11, 2852 (2020).10.1038/s41467-020-16560-7 ↗
15. Lan, X. et al. Quantum dot solids showing state-resolved band-like transport. Nat. Mater. 19, 323–329 (2020).10.1038/s41563-019-0582-2 ↗
16. Sun, B. et al. Ligand-assisted reconstruction of colloidal quantum dots decreases trap state density. Nano Lett. 20, 3694–3702 (2020).10.1021/acs.nanolett.0c00638 ↗
17. Hwang, G. W. et al. Identifying and eliminating emissive sub-bandgap states in thin films of PbS nanocrystals. Adv. Mater. 27, 4481–4486 (2015).10.1002/adma.201501156 ↗
18. Shi, G. et al. The effect of water on colloidal quantum dot solar cells. Nat. Commun. 12, 4381 (2021).10.1038/s41467-021-24614-7 ↗
19. Gilmore, R. H. et al. Epitaxial dimers and Auger-assisted detrapping in PbS quantum dot solids. Matter 1, 250–265 (2019).10.1016/j.matt.2019.05.015 ↗
20. Kim, Y. et al. A facet-specific quantum dot passivation strategy for colloid management and efficient infrared photovoltaics. Adv. Mater. 31, e1805580 (2019).10.1002/adma.201805580 ↗
21. Vafaie, M. et al. Colloidal quantum dot photodetectors with 10-ns response time and 80% quantum efficiency at 1,550 nm. Matter 4, 1042–1053 (2021).10.1016/j.matt.2020.12.017 ↗
22. Wang, H. et al. PbS quantum dots ink with months-long shelf-lifetime enabling scalable and efficient short-wavelength infrared photodetectors. Adv. Mater. 36, e2311526 (2024).10.1002/adma.202311526 ↗
23. Sliz, R. et al. Stable colloidal quantum dot inks enable inkjet-printed high-sensitivity infrared photodetectors. ACS Nano 13, 11988–11995 (2019).10.1021/acsnano.9b06125 ↗
24. Bederak, D. et al. On the colloidal stability of PbS quantum dots capped with methylammonium lead iodide ligands. ACS Appl. Mater. Interfaces 12, 52959–52966 (2020).10.1021/acsami.0c16646 ↗
25. Sukharevska, N. et al. Scalable PbS quantum dot solar cell production by blade coating from stable inks. ACS Appl. Mater. Interfaces 13, 5195–5207 (2021).10.1021/acsami.0c18204 ↗
26. Yang, J. et al. Solvent engineering of colloidal quantum dot inks for scalable fabrication of photovoltaics. ACS Appl. Mater. Interfaces 13, 36992–37003 (2021).10.1021/acsami.1c06352 ↗
27. Zhao, X. et al. Stable PbS colloidal quantum dot inks enable blade-coating infrared solar cells. Front. Optoelectron. 16, 27 (2023).10.1007/s12200-023-00085-0 ↗
28. Goossens, V. M., Sukharevska, N. V., Dirin, D. N., Kovalenko, M. V. & Loi, M. A. Scalable fabrication of efficient p–n junction lead sulfide quantum dot solar cells. Cell Rep. Phys. Sci. 2, 100655 (2021).10.1016/j.xcrp.2021.100655 ↗
29. Ding, C. et al. Over 15% efficiency PbS quantum-dot solar cells by synergistic effects of three interface engineering: reducing nonradiative recombination and balancing charge carrier extraction. Adv. Energy Mater. 12, 2201676 (2022).10.1002/aenm.202201676 ↗
30. Jang, J. et al. All-solution-processed PbS quantum dot solar modules. Nanoscale 7, 8829–8834 (2015).10.1039/C5NR01508A ↗
31. Jean, J. et al. Synthesis cost dictates the commercial viability of lead sulfide and perovskite quantum dot photovoltaics. Energy Environ. Sci. 11, 2295–2305 (2018).10.1039/C8EE01348A ↗
32. Zhao, Q. et al. Colloidal quantum dot solar cells: progressive deposition techniques and future prospects on large-area fabrication. Adv. Mater. 34, 2107888 (2022).10.1002/adma.202107888 ↗
33. Wang, Y. et al. Room-temperature direct synthesis of semi-conductive PbS nanocrystal inks for optoelectronic applications. Nat. Commun. 10, 5136 (2019).10.1038/s41467-019-13158-6 ↗
34. Liu, Y. et al. PbSe quantum dot solar cells based on directly synthesized semiconductive inks. ACS Energy Lett. 5, 3797–3803 (2020).10.1021/acsenergylett.0c02011 ↗
35. Liu, Y. et al. Merging passivation in synthesis enabling the lowest open-circuit voltage loss for PbS quantum dot solar cells. Adv. Mater. 35, 2207293 (2022).10.1002/adma.202207293 ↗
36. Hu, L. et al. Optimizing surface chemistry of PbS colloidal quantum dot for highly efficient and stable solar cells via chemical binding. Adv. Sci. 8, 2003138 (2021).10.1002/advs.202003138 ↗
37. Zheng, S., Chen, J., Johansson, E. M. & Zhang, X. PbS colloidal quantum dot inks for infrared solar cells. iScience 23, 101753 (2020).10.1016/j.isci.2020.101753 ↗
38. Liu, M. et al. Hybrid organic–inorganic inks flatten the energy landscape in colloidal quantum dot solids. Nat. Mater. 16, 258–263 (2017).10.1038/nmat4800 ↗
39. Radicchi, E., Mosconi, E., Elisei, F., Nunzi, F. & De Angelis, F. Understanding the solution chemistry of lead halide perovskites precursors. ACS Appl. Energy Mater. 2, 3400–3409 (2019).10.1021/acsaem.9b00206 ↗
40. Dirin, D. N. et al. Lead halide perovskites and other metal halide complexes as inorganic capping ligands for colloidal nanocrystals. J. Am. Chem. Soc. 136, 6550–6553 (2014).10.1021/ja5006288 ↗
41. Sharenko, A., Mackeen, C., Jewell, L., Bridges, F. & Toney, M. F. Evolution of iodoplumbate complexes in methylammonium lead iodide perovskite precursor solutions. Chem. Mater. 29, 1315–1320 (2017).10.1021/acs.chemmater.6b04917 ↗
42. Sytnyk, M. et al. Quasi-epitaxial metal-halide perovskite ligand shells on PbS nanocrystals. ACS Nano 11, 1246–1256 (2017).10.1021/acsnano.6b04721 ↗
43. Manser, J. S., Saidaminov, M. I., Christians, J. A., Bakr, O. M. & Kamat, P. V. Making and breaking of lead halide perovskites. Acc. Chem. Res. 49, 330–338 (2016).10.1021/acs.accounts.5b00455 ↗
44. Hui, W. et al. Stabilizing black-phase formamidinium perovskite formation at room temperature and high humidity. Science 371, 1359–1364 (2021).10.1126/science.abf7652 ↗
45. Liu, M. et al. Lattice anchoring stabilizes solution-processed semiconductors. Nature 570, 96–101 (2019).10.1038/s41586-019-1239-7 ↗
46. Kim, J. et al. Unveiling the relationship between the perovskite precursor solution and the resulting device performance. J. Am. Chem. Soc. 142, 6251–6260 (2020).10.1021/jacs.0c00411 ↗
47. Salopek, B., Krasic, D. & Filipovic, S. Measurement and application of zeta-potential. Rudarsko-geolosko-naftni zbornik 4, 147 (1992).
48. Berne, B. J. & Pecora, R. Dynamic Light Scattering: With Applications to Chemistry, Biology, and Physics (Courier Corporation, 2000).
49. Zhang, H. et al. Stable colloids in molten inorganic salts. Nature 542, 328–331 (2017).10.1038/nature21041 ↗
50. Andersen, T. R. et al. Scalable, ambient atmosphere roll-to-roll manufacture of encapsulated large area, flexible organic tandem solar cell modules. Energy Environ. Sci. 7, 2925 (2014).10.1039/C4EE01223B ↗
51. Coropceanu, I. et al. Self-assembly of nanocrystals into strongly electronically coupled all-inorganic supercrystals. Science 375, 1422–1426 (2022).10.1126/science.abm6753 ↗
52. van Huis, M. A. et al. Low-temperature nanocrystal unification through rotations and relaxations probed by in situ transmission electron microscopy. Nano Lett. 8, 3959–3963 (2008).10.1021/nl8024467 ↗
53. Evers, W. H. et al. Low-dimensional semiconductor superlattices formed by geometric control over nanocrystal attachment. Nano Lett. 13, 2317–2323 (2013).10.1021/nl303322k ↗
54. More, S. A. et al. Investigating the effect of solvent vapours on crystallinity, phase, and optical, morphological and structural properties of organolead halide perovskite films. RSC Adv. 10, 39995–40004 (2020).10.1039/D0RA07926J ↗
55. Winslow, S. W., Liu, Y., Swan, J. W. & Tisdale, W. A. Quantification of a PbClx shell on the surface of PbS nanocrystals. ACS Mater. Lett. 1, 209–216 (2019).10.1021/acsmaterialslett.9b00200 ↗
56. Green, P. B., Li, Z. & Wilson, M. W. PbS nanocrystals made with excess PbCl2 have an intrinsic shell that reduces their stokes shift. J. Phys. Chem. Lett. 10, 5897–5901 (2019).10.1021/acs.jpclett.9b01841 ↗
57. Zhang, Y. et al. Photoexcited carrier dynamics in colloidal quantum dot solar cells: insights into individual quantum dots, quantum dot solid films and devices. Chem. Soc. Rev. 49, 49–84 (2020).10.1039/C9CS00560A ↗
58. Fang, H. H. et al. Exciton recombination in formamidinium lead triiodide: nanocrystals versus thin films. Small 13, 1700673 (2017).10.1002/smll.201700673 ↗
59. Liu, J. et al. Visible and near-infrared, multiparametric, ultrasensitive nanothermometer based on dual-emission colloidal quantum dots. ACS Photon. 6, 2479–2486 (2019).10.1021/acsphotonics.9b00763 ↗
60. Papagiorgis, P., Stavrinadis, A., Othonos, A., Konstantatos, G. & Itskos, G. The influence of doping on the optoelectronic properties of PbS colloidal quantum dot solids. Sci. Rep. 6, 18735 (2016).10.1038/srep18735 ↗
61. Meng, X. et al. Perovskite bridging PbS quantum dot/polymer interface enables efficient solar cells. Nano Res. 15, 6121–6127 (2022).10.1007/s12274-022-4195-8 ↗
62. Kim, B., Baek, S. W., Kim, C., Kim, J. & Lee, J. Y. Mediating colloidal quantum dot/organic semiconductor interfaces for efficient hybrid solar cells. Adv. Energy Mater. 12, 2102689 (2022).10.1002/aenm.202102689 ↗
63. Shi, G. et al. Finely interpenetrating bulk heterojunction structure for lead sulfide colloidal quantum dot solar cells by convective assembly. ACS Energy Lett. 4, 960–967 (2019).10.1021/acsenergylett.9b00053 ↗
64. Qu, X. & Sun, X. Impedance spectroscopy for quantum dot light-emitting diodes. J. Semicond. 44, 091603 (2023).10.1088/1674-4926/44/9/091603 ↗
65. Karl, A., Osvet, A., Li, N. & Brabec, C. J. A general guideline for vertically resolved imaging of manufacturing defects in organic tandem solar cells. Adv. Mater. Interfaces 7, 2000336 (2020).10.1002/admi.202000336 ↗
66. VDMA. Photovoltaics Equipment, International Technology Roadmap for Photovoltaic Results 2023 (ITRPV, 2024).
67. Alberola-Borras, J. A. et al. Perovskite photovoltaic modules: life cycle assessment of pre-industrial production process. iScience 9, 542–551 (2018).10.1016/j.isci.2018.10.020 ↗
68. Tang, H. et al. Lead sulfide quantum dot photodetector with enhanced responsivity through a two-step ligand-exchange method. Appl. Nano Mater. 2, 6135–6143 (2019).10.1021/acsanm.9b00889 ↗
69. Wienhold, K. S. et al. Following in operando the structure evolution-induced degradation in printed organic solar cells with nonfullerene small molecule acceptor. Sol. RRL 4, 2000251 (2020).10.1002/solr.202000251 ↗
70. Chen, W. et al. Structure and charge carrier dynamics in colloidal PbS quantum dot solids. J. Phys. Chem. Lett. 10, 2058–2065 (2019).10.1021/acs.jpclett.9b00869 ↗
71. Kresse, G. & Hafner, J. Norm-conserving and ultrasoft pseudopotentials for first-row and transition elements. J. Phys. Condens. Matter 6, 8245 (1994).10.1088/0953-8984/6/40/015 ↗
72. Blochl, P. E., Jepsen, O. & Andersen, O. K. Improved tetrahedron method for Brillouin-zone integrations. Phys. Rev. B 49, 16223–16233 (1994).10.1103/PhysRevB.49.16223 ↗
73. Bende, D., Wagner, F. R., Sichevych, O. & Grin, Y. Chemical bonding analysis as a guide for the preparation of new compounds: the case of VIrGe and HfPtGe. Angew. Chem. Int. Ed. 56, 1313–1318 (2017).10.1002/anie.201610029 ↗
74. Lunardi, M. M., Alvarez-Gaitan, J., Chang, N. L. & Corkish, R. Life cycle assessment on PERC solar modules. Sol. Energy Mater. Sol. Cells 187, 154–159 (2018).10.1016/j.solmat.2018.08.004 ↗