journal article·2024-10-25

Self-Powered Solar-Blind UV Photodetector Based on Core–Shell Heterojunction with Lu2O3 Nanolayer Modified β-Ga2O3 Microwire

Renjie Jin, Jinsong Liu, Shiwei Chen, Hongde Wang, Changsheng Niu, Xuehua Zhang, Chao Wu, Haizheng Hu, Kai Chen, Daoyou Guo, Shunli Wang

ACS Applied Nano Materials· Volume 7· Issue 20
Publisher page

Abstract

Solar-blind ultraviolet (UV) photodetectors play a critical role in ultraviolet communication and monitoring, effectively reducing false alarm rates and improving the accuracy of detection systems across various settings, which has garnered significant attention. Due to its exceptional solar-blind photon absorption coefficient, extremely stable structure, and ultrawide bandgap (4.5–4.9 eV), Ga 2 O 3 has recently been identified as a desirable material for solar-blind UV photodetectors. Heterojunctions can separate photogenerated electron–hole pairs and their absorption edges can be controlled by selecting semiconductors with appropriate bandgaps, making them an important technology for light detection. In this work, a self-powered solar-blind UV photodetector has been fabricated using a mechanically separated β-Ga 2 O 3 /Lu 2 O 3 core–shell microwire heterostructure. Our device demonstrates excellent solar-blind UV discriminability with self-powered photodetection, the device exhibits a responsivity of 38.8 mA/W, a detectivity of 1.22 × 10 12 Jones, a switching ratio of 1.43 × 10 3, and a decay rate under UV irradiation of 62 ms, benefiting from both photovoltaic and photoconductive effects. Due to the high dielectric constant of Lu 2 O 3 thin films at the nanoscale, enables more effective modulation of internal electric fields within heterojunction structures, thereby enhancing the response speed and sensitivity of photodetectors. The application of self-powered photodetectors in solar-blind communication systems has achieved promising results, which provides a viable strategy for Ga 2 O 3 -based high-performance self-powered photodetectors.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Ga2O3 and related materials · ZnO doping and properties · Advanced Photocatalysis Techniques

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Zhejiang Key Laboratory of Quantum State Control and Optical Field Manipulation & Department of Physics, Zhejiang Sci-Tech University, 310018 Hangzhou, China

Yiwu Huading Nylon Co., LTD., Yiwu 322000, China

Funding

Zhejiang Sci-Tech University · National Natural Science Foundation of China · Department of Education of Zhejiang Province · Natural Science Foundation of Zhejiang Province

References (46)

Show source-provided references
1. 10.1038/nphoton.2012.10810.1038/nphoton.2012.108 ↗
2. 10.1038/nature0881310.1038/nature08813 ↗
3. 10.1039/C8TC01122B10.1039/C8TC01122B ↗
4. 10.1039/C7TC03746E10.1039/C7TC03746E ↗
5. 10.1039/C7TC01741C10.1039/C7TC01741C ↗
6. 10.1021/acsanm.2c0549910.1021/acsanm.2c05499 ↗
7. 10.1016/j.pquantelec.2022.10039710.1016/j.pquantelec.2022.100397 ↗
8. 10.1002/adom.20200089310.1002/adom.202000893 ↗
9. 10.1063/1.490592910.1063/1.4905929 ↗
10. 10.1186/s43074-024-00120-z10.1186/s43074-024-00120-z ↗
11. 10.1364/OME.8.00078510.1364/OME.8.000785 ↗
12. 10.7567/JJAP.55.03550110.7567/JJAP.55.035501 ↗
13. 10.29026/oes.2023.23001010.29026/oes.2023.230010 ↗
14. 10.1016/j.mtphys.2020.10033510.1016/j.mtphys.2020.100335 ↗
15. 10.1021/acsami.8b0809510.1021/acsami.8b08095 ↗
16. 10.1039/D3TC03599A10.1039/D3TC03599A ↗
17. 10.1039/C9TC05159G10.1039/C9TC05159G ↗
18. 10.1021/acsphotonics.7b0148610.1021/acsphotonics.7b01486 ↗
19. 10.1016/j.mtphys.2023.10103410.1016/j.mtphys.2023.101034 ↗
20. 10.1039/c3tc30525b10.1039/c3tc30525b ↗
21. 10.1021/nn403751410.1021/nn4037514 ↗
22. 10.1039/C6TC00748A10.1039/C6TC00748A ↗
23. 10.1088/0957-4484/18/34/34530510.1088/0957-4484/18/34/345305 ↗
24. 10.1143/APEX.1.01120210.1143/APEX.1.011202 ↗
25. 10.1186/s43074-022-00054-410.1186/s43074-022-00054-4 ↗
26. 10.1002/adfm.20170026410.1002/adfm.201700264 ↗
27. 10.1016/j.solmat.2016.03.01510.1016/j.solmat.2016.03.015 ↗
28. 10.1063/1.499211410.1063/1.4992114 ↗
29. 10.1109/LED.2023.326275510.1109/LED.2023.3262755 ↗
30. 10.1134/S106378261005002710.1134/S1063782610050027 ↗
31. Wiktorczyk T. · Opt. Appl. · 2001 · 31 · 83
32. Fanciulli M. · 2007 · 106 · 1
33. 10.1103/PhysRevB.74.19512310.1103/PhysRevB.74.195123 ↗
34. 10.1016/j.ceramint.2021.04.28410.1016/j.ceramint.2021.04.284 ↗
35. 10.1016/j.ceramint.2021.07.00710.1016/j.ceramint.2021.07.007 ↗
36. 10.4236/ampc.2023.131101410.4236/ampc.2023.1311014 ↗
37. 10.1002/adma.20160404910.1002/adma.201604049 ↗
38. 10.1038/s41566-018-0288-z10.1038/s41566-018-0288-z ↗
39. 10.1038/nphoton.2007.14710.1038/nphoton.2007.147 ↗
40. 10.1021/acsphotonics.8b0017410.1021/acsphotonics.8b00174 ↗
41. 10.1016/j.apsusc.2020.14838010.1016/j.apsusc.2020.148380 ↗
42. 10.1016/j.jallcom.2019.15353210.1016/j.jallcom.2019.153532 ↗
43. 10.1021/acsami.6b1377110.1021/acsami.6b13771 ↗
44. 10.1063/5.004875210.1063/5.0048752 ↗
45. 10.1039/C8TC04258F10.1039/C8TC04258F ↗
46. 10.1002/adfm.20190093510.1002/adfm.201900935 ↗