journal article·2026-07-01

Geometry-Driven Performance Enhancement in h-BN/β-Ga 2 O 3 Heterostructures for Solar-Blind and Polarization-Sensitive Photodetection

Waqas Ahmad, Shrouq H. Aleithan, Muhammad Ajmal, Yury Yuryevich Illarionov

ACS Applied Materials & Interfaces· Volume 18· Issue 25
Publisher page

Abstract

Solar-blind ultraviolet photodetectors have attracted increasing interest, yet their performance is often limited by inefficient carrier collection and reliance on complex thin-film growth techniques. In this work, we investigate geometry-driven performance enhancement in h-BN/β-Ga 2 O 3 heterostructures fabricated using mechanically exfoliated β-Ga 2 O 3, offering a simple and cost-effective alternative to epitaxial approaches. The exfoliated β-Ga 2 O 3 devices exhibit a clear photoresponse over a broad spectral range from 200 to 405 nm. By systematically comparing vertical and lateral heterostructure architectures, we demonstrate that device geometry plays a decisive role in determining photodetection behavior. The vertical h-BN/β-Ga 2 O 3 photodetector device exhibits a markedly enhanced solar-blind response, achieving a high responsivity of 96.7 AW –1 and an external quantum efficiency of 52258% at 230 nm, which are substantially higher than those of the lateral heterostructure (5.0 AW –1 and 2317%) and the bare β-Ga 2 O 3 photodetector device (0.29 AW –1 and 135%). In addition, polarization-resolved measurements reveal an anisotropic photoresponse with a dichroic ratio of approximately 2.1 for the vertical configuration. Interfacial potential investigations confirm the presence of a built-in electric field that promotes efficient photocarrier separation. These results highlight geometry design as an effective strategy for realizing high-performance, solar-blind, and polarization-sensitive photodetection using straightforward exfoliation-based heterostructures.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Ga2O3 and related materials · Advanced Photocatalysis Techniques · Electronic and Structural Properties of Oxides

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Laboratory of 2D Optoelectronics and Nanoelectronics (L2DON), State Key Laboratory of Quantum Functional Materials, Department of Materials Science and Engineering, Southern University of Science and Technology, 1088 Xueyuan Blvd, Shenzhen 518055, China

Department of Physics, College of Science

King Faisal University

Interdisciplinary Research Center for Hydrogen Technologies and Carbon Management (IRC-HTCM)

King Fahd University of Petroleum & Minerals (KFUPM)

Funding

Basic and Applied Basic Research Foundation of Guangdong Province · Deanship of Scientific Research, King Faisal University · National Natural Science Foundation of China · Shenzhen Key Laboratory of Phononics and Intelligent Thermal Materials

References (61)

Show source-provided references
1. 10.1016/j.mtphys.2022.10088310.1016/j.mtphys.2022.100883 ↗
2. 10.1021/acsomega.4c0289710.1021/acsomega.4c02897 ↗
3. 10.1002/smll.20250820810.1002/smll.202508208 ↗
4. 10.1002/lpor.20240192610.1002/lpor.202401926 ↗
5. 10.1038/s41467-025-63302-810.1038/s41467-025-63302-8 ↗
6. 10.1002/adfm.20180600610.1002/adfm.201806006 ↗
7. 10.1016/j.jallcom.2019.15341910.1016/j.jallcom.2019.153419 ↗
8. 10.1021/acsphotonics.3c0128110.1021/acsphotonics.3c01281 ↗
9. 10.1002/lpor.20250226810.1002/lpor.202502268 ↗
10. 10.1002/adma.20240008910.1002/adma.202400089 ↗
11. 10.1038/s41377-021-00527-410.1038/s41377-021-00527-4 ↗
12. 10.1002/adom.20180058010.1002/adom.201800580 ↗
13. 10.1038/s41467-025-63683-w10.1038/s41467-025-63683-w ↗
14. 10.1002/adpr.20250000810.1002/adpr.202500008 ↗
15. 10.1016/j.apsusc.2025.16559910.1016/j.apsusc.2025.165599 ↗
16. 10.1016/j.jallcom.2024.17785110.1016/j.jallcom.2024.177851 ↗
17. 10.1109/JEDS.2025.359476710.1109/JEDS.2025.3594767 ↗
18. 10.1016/j.apsusc.2025.16236810.1016/j.apsusc.2025.162368 ↗
19. 10.1039/D4TC03641G10.1039/D4TC03641G ↗
20. 10.1016/j.nanoen.2025.11104710.1016/j.nanoen.2025.111047 ↗
21. 10.1109/TNS.2026.366650210.1109/TNS.2026.3666502 ↗
22. 10.1109/TGRS.2025.358636210.1109/TGRS.2025.3586362 ↗
23. 10.1002/adom.20250174710.1002/adom.202501747 ↗
24. 10.1002/smll.20240954410.1002/smll.202409544 ↗
25. 10.1002/adfm.20241072310.1002/adfm.202410723 ↗
26. 10.1063/1.173123710.1063/1.1731237 ↗
27. 10.35848/1882-0786/ad6b7310.35848/1882-0786/ad6b73 ↗
28. 10.1002/adfm.20100114010.1002/adfm.201001140 ↗
29. 10.1039/C8TC01122B10.1039/C8TC01122B ↗
30. 10.1021/acsami.4c1534510.1021/acsami.4c15345 ↗
31. 10.1016/j.jallcom.2024.17615610.1016/j.jallcom.2024.176156 ↗
32. 10.1021/acsami.4c0139610.1021/acsami.4c01396 ↗
33. 10.1002/lpor.20240081910.1002/lpor.202400819 ↗
34. 10.1021/acsami.7b0437410.1021/acsami.7b04374 ↗
35. 10.1016/j.mtphys.2024.10150610.1016/j.mtphys.2024.101506 ↗
36. 10.1016/j.optlastec.2025.11464410.1016/j.optlastec.2025.114644 ↗
37. 10.1016/j.apsusc.2022.15455910.1016/j.apsusc.2022.154559 ↗
38. 10.1109/JSTARS.2026.366571810.1109/JSTARS.2026.3665718 ↗
39. 10.1039/D5NR02661J10.1039/D5NR02661J ↗
40. 10.1016/j.mtener.2025.10190610.1016/j.mtener.2025.101906 ↗
41. 10.1021/acsami.5c1390310.1021/acsami.5c13903 ↗
42. 10.1016/j.optlastec.2025.11352510.1016/j.optlastec.2025.113525 ↗
43. 10.1039/D0MA00008F10.1039/D0MA00008F ↗
44. 10.1038/s41928-022-00911-x10.1038/s41928-022-00911-x ↗
45. 10.1063/1.500694110.1063/1.5006941 ↗
46. 10.1002/aelm.20240089810.1002/aelm.202400898 ↗
47. 10.1038/s43246-026-01114-z10.1038/s43246-026-01114-z ↗
48. 10.1002/adfm.20251689310.1002/adfm.202516893 ↗
49. 10.1038/s41467-023-37635-110.1038/s41467-023-37635-1 ↗
50. 10.1021/acsami.6c0372110.1021/acsami.6c03721 ↗
51. 10.1002/smll.20220764110.1002/smll.202207641 ↗
52. 10.1002/adma.20221211810.1002/adma.202212118 ↗
53. 10.1021/acsaelm.3c0006610.1021/acsaelm.3c00066 ↗
54. 10.1021/acsami.4c0180610.1021/acsami.4c01806 ↗
55. 10.1109/JEDS.2025.358330510.1109/JEDS.2025.3583305 ↗
56. 10.1021/acsami.4c0780210.1021/acsami.4c07802 ↗
57. 10.1021/acs.nanolett.4c0599710.1021/acs.nanolett.4c05997 ↗
58. 10.1039/C8TC04258F10.1039/C8TC04258F ↗
59. 10.1016/j.physb.2025.41765110.1016/j.physb.2025.417651 ↗
60. 10.1002/admi.20230037110.1002/admi.202300371 ↗
61. 10.1186/s11671-020-3271-910.1186/s11671-020-3271-9 ↗