journal article·2026-04-15

Interfacial Coexistence of Superconductivity and Magnetism in NbN/Ti/MnBi 2 Te 4 Heterostructures

Yanjiang Wang, Peng Dong, Xiaohui Zeng, Chen Xu, Jianjun Xiao, Yang Zhao, Jinghui Wang, Yueshen Wu, Xiang Zhou, Yanfeng Guo, Yulin Chen, Thorsten Hesjedal, Jun Li

ACS Applied Materials & Interfaces· Volume 18· Issue 14
Publisher page

Abstract

Magnetic/superconducting heterostructures represent a frontier in condensed matter physics, offering pathways to realize unconventional pairing mechanisms such as topological superconductivity, spin-triplet pairing, and Majorana zero modes for fault-tolerant quantum computing. In this work, we integrate the magnetic van der Waals material MnBi 2 Te 4 (MBT) with a superconducting NbN thin film, achieving ultralow-disorder interfaces through Ti buffer layer engineering. Temperature- and field-dependent critical currents, extracted from differential resistance spectra, reveal robust coupling between the MnBi 2 Te 4 and the superconducting order of NbN, enabling proximity-induced superconductivity within MnBi 2 Te 4 . Notably, the proximity-induced critical currents remain invariant under in-plane field rotation, in contrast to the anisotropic response observed in pristine NbN. Moreover, the hysteretic behavior observed in the interfacial magnetoresistance curves confirms the proximity-induced spin polarization at the MBT interface, which is consistent with Andreev reflection results. These findings demonstrate a platform for fabricating high-quality heterointerfaces and enable targeted exploration of exotic quantum states.
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Research context

OpenAlex topics: Topological Materials and Phenomena · 2D Materials and Applications · Chemical and Physical Properties of Materials

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Affiliations

State Key Laboratory of Quantum Functional Materials

ShanghaiTech University

School of Physical Science and Technology

ShanghaiTech Laboratory for Topological Physics

Department of Physics, Clarendon Laboratory

University of Oxford

Funding

the National Natural Science Foundation of China

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