journal article·2022-09-14Open access

Correlative Nanoscale Imaging of Strained hBN Spin Defects

David Curie, Jaron T. Krogel, Lukas Cavar, Abhishek Solanki, Pramey Upadhyaya, Tongcang Li, Yun-Yi Pai, Michael Chilcote, Vasudevan Iyer, Alexander Puretzky, Ilia Ivanov, Mao-Hua Du, Fernando Reboredo, Benjamin Lawrie

ACS Applied Materials & Interfaces· Volume 14· Issue 36

Abstract

Spin defects like the negatively charged boron vacancy color center (VB–) in hexagonal boron nitride (hBN) may enable new forms of quantum sensing with near-surface defects in layered van der Waals heterostructures. Here, the effect of strain on VB– color centers in hBN is revealed with correlative cathodoluminescence and photoluminescence microscopies. Strong localized enhancement and redshifting of the VB– luminescence is observed at creases, consistent with density functional theory calculations showing VB– migration toward regions with moderate uniaxial compressive strain. The ability to manipulate spin defects with highly localized strain is critical to the development of practical 2D quantum devices and quantum sensors.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Graphene research and applications · Diamond and Carbon-based Materials Research · Boron and Carbon Nanomaterials Research

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Physics and Astronomy, Vanderbilt University, Nashville, Tennessee 37235, United States

Materials Science and Technology Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, United States

Department of Physics, Indiana University, Bloomington, Indiana 47405, United States

Elmore Family School of Electrical and Computer Engineering, Purdue University, West Lafayette, Indiana 47907, United States

Department of Physics and Astronomy, Purdue University, West Lafayette, Indiana 47907, United States

Quantum Science Center, Oak Ridge, Tennessee 37831, United States

Center for Nanophase Materials Sciences, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, United States

Funding

U.S. Department of Defense · U.S. Department of Energy

References (54)

Show source-provided references
1. 10.1021/acsnano.6b0360210.1021/acsnano.6b03602 ↗
2. 10.1038/nphoton.2016.18610.1038/nphoton.2016.186 ↗
3. 10.1038/nnano.2015.24210.1038/nnano.2015.242 ↗
4. 10.1103/physrevb.94.12140510.1103/physrevb.94.121405 ↗
5. 10.1038/s41467-022-28169-z10.1038/s41467-022-28169-z ↗
6. 10.1103/physrevb.104.07541010.1103/physrevb.104.075410 ↗
7. 10.1126/sciadv.abf363010.1126/sciadv.abf3630 ↗
8. 10.1021/acs.nanolett.1c0436610.1021/acs.nanolett.1c04366 ↗
9. 10.1038/s41563-020-0619-610.1038/s41563-020-0619-6 ↗
10. 10.1021/acsphotonics.0c0061410.1021/acsphotonics.0c00614 ↗
11. 10.1038/s41467-022-30772-z10.1038/s41467-022-30772-z ↗
12. 10.1021/acs.nanolett.1c0461010.1021/acs.nanolett.1c04610 ↗
13. 10.1103/PhysRevLett.128.21640210.1103/PhysRevLett.128.216402 ↗
14. 10.1038/s41567-021-01338-510.1038/s41567-021-01338-5 ↗
15. 10.1103/physrevlett.102.19550510.1103/physrevlett.102.195505 ↗
16. Qiu, Z.; Vaklinova, K.; Huang, P.; Grzeszczyk, M.; Yang, H.; Watanabe, K.; Taniguchi, T.; Novoselov, K.; Lu, J.; Koperski, M. Atomic Structure of Carbon Centres in hBN: Towards Engineering of Single Photon Sources. 2021, arXiv:2110.07842 cond-mat.mtrl-sci Submitted on 15 Oct 2021.
17. 10.1038/nnano.2015.18810.1038/nnano.2015.188 ↗
18. 10.1364/optica.40618410.1364/optica.406184 ↗
19. 10.1103/physrevb.99.02010110.1103/physrevb.99.020101 ↗
20. 10.1021/acs.nanolett.1c0249510.1021/acs.nanolett.1c02495 ↗
21. 10.1021/acsphotonics.0c0184710.1021/acsphotonics.0c01847 ↗
22. 10.3390/nano1106137310.3390/nano11061373 ↗
23. 10.1021/acsphotonics.7b0144210.1021/acsphotonics.7b01442 ↗
24. 10.1103/physrevlett.128.16740110.1103/physrevlett.128.167401 ↗
25. 10.1021/acs.jpcc.1c0772910.1021/acs.jpcc.1c07729 ↗
26. 10.1038/s41534-020-00312-y10.1038/s41534-020-00312-y ↗
27. 10.1038/s41563-020-0616-910.1038/s41563-020-0616-9 ↗
28. 10.1016/j.nantod.2018.07.00110.1016/j.nantod.2018.07.001 ↗
29. 10.1002/adma.20190831610.1002/adma.201908316 ↗
30. 10.1364/optica.5.00112810.1364/optica.5.001128 ↗
31. 10.1021/acsami.0c0974010.1021/acsami.0c09740 ↗
32. 10.1021/acs.nanolett.6b0136810.1021/acs.nanolett.6b01368 ↗
33. 10.1103/physrevlett.114.19740110.1103/physrevlett.114.197401 ↗
34. 10.1021/acs.nanolett.9b0430410.1021/acs.nanolett.9b04304 ↗
35. 10.1109/tkde.2012.5110.1109/tkde.2012.51 ↗
36. 10.1088/0953-8984/21/39/39550210.1088/0953-8984/21/39/395502 ↗
37. 10.1103/physrevlett.77.386510.1103/physrevlett.77.3865 ↗
38. 10.1103/physrevlett.78.139610.1103/physrevlett.78.1396 ↗
39. 10.1016/j.commatsci.2013.08.05310.1016/j.commatsci.2013.08.053 ↗
40. 10.1063/5.006552410.1063/5.0065524 ↗
41. 10.1021/acs.analchem.9b0259310.1021/acs.analchem.9b02593 ↗
42. 10.1021/acsphotonics.1c0036410.1021/acsphotonics.1c00364 ↗
43. 10.1021/nl061081l10.1021/nl061081l ↗
44. 10.1103/physrevb.86.24540610.1103/physrevb.86.245406 ↗
45. 10.1155/2022/103694210.1155/2022/1036942 ↗
46. 10.1103/physrevb.97.06410110.1103/physrevb.97.064101 ↗
47. 10.1021/acsphotonics.9b0146310.1021/acsphotonics.9b01463 ↗
48. 10.1103/physrevb.97.08140410.1103/physrevb.97.081404 ↗
49. 10.1103/physrevb.75.09410410.1103/physrevb.75.094104 ↗
50. 10.1209/0295-5075/28/5/00710.1209/0295-5075/28/5/007 ↗
51. 10.1016/j.ssc.2005.02.00710.1016/j.ssc.2005.02.007 ↗
52. 10.1021/jp907850810.1021/jp9078508 ↗
53. 10.1038/s41524-020-0305-x10.1038/s41524-020-0305-x ↗
54. 10.1002/pssa.20056190210.1002/pssa.200561902 ↗