journal article·2025-09-24

Three-Dimensional Bubble Fluidics in Architected Porous Media

Jonathan T. Davis, Kansas Seung, Anna Guell Izard, Hawi B. Gemeda, Ariel Gluck, Thomas Moore, Nikola A. Dudukovic, Erika J. Fong, Joshua R. Deotte, Sarah E. Baker, Eric B. Duoss

ACS Applied Materials & Interfaces· Volume 17· Issue 38
Publisher page

Abstract

Gas bubble flows in porous media often exhibit complex and seemingly unpredictable behaviors that are difficult to control. This lack of control limits the ability to design effective devices which manage multiphase flows. We show how the design of 3D printed pores can deterministically control the flow path of an injected gas stream. Open cell structures can be designed to shape the gas/liquid interface with fidelity to control how the two phases are distributed throughout a porous material. The distributed gas volume is free to interact physically and chemically with the surrounding liquid phase, an effect we exploit to create a logical control gate to redirect flows within a lattice. This also allows us to design architectures for reactive capture and aerating bioreactors, resulting in patterned boundaries which can make more effective use of the liquid and gas reagents.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Fluid Dynamics and Mixing · Pickering emulsions and particle stabilization · Innovative Microfluidic and Catalytic Techniques Innovation

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Materials Engineering Division

Lawrence Livermore National Laboratory

Materials Science Division

Funding

Lawrence Livermore National Laboratory

References (61)

Show source-provided references
1. 10.1063/1.169530810.1063/1.1695308 ↗
2. 10.1016/j.nucengdes.2018.02.02410.1016/j.nucengdes.2018.02.024 ↗
3. 10.1016/j.cis.2020.10220810.1016/j.cis.2020.102208 ↗
4. 10.1126/science.110916410.1126/science.1109164 ↗
5. 10.1016/j.cell.2015.04.04410.1016/j.cell.2015.04.044 ↗
6. 10.1063/5.004989710.1063/5.0049897 ↗
7. 10.1021/acs.analchem.9b0142910.1021/acs.analchem.9b01429 ↗
8. 10.1038/s41586-021-03603-210.1038/s41586-021-03603-2 ↗
9. 10.1016/j.cej.2012.09.12110.1016/j.cej.2012.09.121 ↗
10. 10.1007/s10616-009-9189-910.1007/s10616-009-9189-9 ↗
11. 10.1002/aic.1573710.1002/aic.15737 ↗
12. 10.1007/s00253-011-3365-510.1007/s00253-011-3365-5 ↗
13. 10.1021/ie950366y10.1021/ie950366y ↗
14. 10.3390/fluids803009110.3390/fluids8030091 ↗
15. 10.1016/j.ijggc.2013.09.00810.1016/j.ijggc.2013.09.008 ↗
16. 10.1016/j.ijggc.2021.10353410.1016/j.ijggc.2021.103534 ↗
17. Schoenung, S. M.; Efroymson, R. A.; Langholtz, M. H. Considerations for the Design of a Gas Transport System for Co-location of Microalgae Cultivation with CO2 Sources; ORNL/TM-2019/1130: United States, 2019.10.2172/1507853 ↗
18. 10.3390/pr705031110.3390/pr7050311 ↗
19. 10.1039/D2EE03658D10.1039/D2EE03658D ↗
20. 10.1016/j.ces.2022.11832010.1016/j.ces.2022.118320 ↗
21. 10.1080/01496395.2018.154907810.1080/01496395.2018.1549078 ↗
22. 10.1016/j.ijggc.2012.03.00310.1016/j.ijggc.2012.03.003 ↗
23. 10.1038/438930a10.1038/438930a ↗
24. 10.1103/PhysRevLett.123.25450110.1103/PhysRevLett.123.254501 ↗
25. 10.1146/annurev-fluid-122414-03442510.1146/annurev-fluid-122414-034425 ↗
26. 10.1016/j.seppur.2019.11579110.1016/j.seppur.2019.115791 ↗
27. 10.1016/j.memsci.2022.12040310.1016/j.memsci.2022.120403 ↗
28. 10.1126/science.125229110.1126/science.1252291 ↗
29. 10.1016/j.applthermaleng.2022.11833910.1016/j.applthermaleng.2022.118339 ↗
30. 10.1002/adem.20200015810.1002/adem.202000158 ↗
31. 10.1021/acs.chemrev.0c0008410.1021/acs.chemrev.0c00084 ↗
32. 10.1016/j.biomaterials.2012.01.04810.1016/j.biomaterials.2012.01.048 ↗
33. 10.1002/bit.2495710.1002/bit.24957 ↗
34. 10.1002/adma.20240460610.1002/adma.202404606 ↗
35. 10.1021/jacsau.2c0043210.1021/jacsau.2c00432 ↗
36. 10.1016/j.ijmultiphaseflow.2012.01.00210.1016/j.ijmultiphaseflow.2012.01.002 ↗
37. 10.1039/b516975e10.1039/b516975e ↗
38. 10.1002/adma.20200553810.1002/adma.202005538 ↗
39. 10.1021/la803568a10.1021/la803568a ↗
40. 10.1016/j.jcis.2006.10.04210.1016/j.jcis.2006.10.042 ↗
41. 10.1016/j.jcis.2007.06.07010.1016/j.jcis.2007.06.070 ↗
42. 10.1103/PhysRevE.88.04301010.1103/PhysRevE.88.043010 ↗
43. 10.1002/2015GL06400710.1002/2015GL064007 ↗
44. 10.1103/PhysRevLett.120.02800510.1103/PhysRevLett.120.028005 ↗
45. 10.1073/pnas.202406911810.1073/pnas.2024069118 ↗
46. 10.1103/PhysRevLett.119.26450210.1103/PhysRevLett.119.264502 ↗
47. 10.1126/science.113690710.1126/science.1136907 ↗
48. 10.1002/adma.20170289410.1002/adma.201702894 ↗
49. 10.3390/membranes1207064210.3390/membranes12070642 ↗
50. 10.1039/C8LC00458G10.1039/C8LC00458G ↗
51. 10.1039/c2lc00033d10.1039/c2lc00033d ↗
52. 10.1126/sciadv.abm014410.1126/sciadv.abm0144 ↗
53. 10.1002/aic.1703110.1002/aic.17031 ↗
54. 10.1038/s41526-022-00246-z10.1038/s41526-022-00246-z ↗
55. 10.3389/frspt.2021.77969610.3389/frspt.2021.779696 ↗
56. 10.1016/j.cbpa.2007.05.03410.1016/j.cbpa.2007.05.034 ↗
57. 10.1042/BA2007017710.1042/BA20070177 ↗
58. 10.1002/btpr.179010.1002/btpr.1790 ↗
59. 10.1039/C9GC00920E10.1039/C9GC00920E ↗
60. 10.1126/sciadv.aau641910.1126/sciadv.aau6419 ↗
61. 10.1038/nmat469410.1038/nmat4694 ↗