journal article·2024-10-23

Ultralow Contact Thermal Resistance between Bismuth Selenide Nanoribbons Achieved by Current-Induced Annealing

Yucheng Xiong, Shouhang Li, Renzong Wang, Zhe Cheng, Juekuan Yang, Deyu Li, Xiangjun Liu, Dongyan Xu

ACS Applied Materials & Interfaces· Volume 16· Issue 42
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Abstract

Thermal resistance at interfaces/contacts stands as a persistent and increasingly critical issue, which hinders ultimate scaling and the performance of electronic devices. Compared to the extensive research on contact electrical resistance, contact thermal resistance and its mitigation strategies have received relatively less attention. Here, we report on an effective, in situ, and energy-efficient approach for enhancing thermal transport through the contact between semiconducting nanoribbons. By applying microampere-level electrical currents to the contact between Bi 2 Se 3 nanoribbons, we demonstrate that the contact thermal resistance between two nanoribbon segments is reduced dramatically by a factor of 4, rendering the total thermal resistance of two ribbon segments with a contact approximately the same as that of the corresponding single continuous nanoribbon of the same length. Analysis suggests that the ultralow contact thermal resistance is due to enhanced phonon transmission as a result of enhanced adhesion energy at the contact, with marginal contributions from direct electron–phonon coupling, even for ohmic contacts. Our work introduces a broadly applicable electrical treatment approach to various contacts between conducting and semiconducting materials, which has important implications for the design and operation of nanoelectronic devices and energy converters.
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Research context

OpenAlex topics: Thermal properties of materials · Advanced Thermoelectric Materials and Devices · Thermal Radiation and Cooling Technologies

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Institute of Micro/Nano Electromechanical System, College of Mechanical Engineering, Donghua University, Shanghai 201620, China

Department of Mechanical and Automation Engineering, The Chinese University of Hong Kong, Shatin, New Territories, Hong Kong Special Administrative Region, China

School of Integrated Circuit and Frontier Science Center for Nano-optoelectronics, Peking University, Beijing 100871, China

School of Mechanical Engineering and Jiangsu Key Laboratory for Design and Manufacture of Micro-Nano Biomedical Instruments, Southeast University, Nanjing 210096, China

Department of Mechanical Engineering, Vanderbilt University, Nashville, Tennessee 37235, United States

Funding

Natural Science Foundation of Shanghai Municipality · Science and Technology Commission of Shanghai Municipality · Fundamental Research Funds for the Central Universities · National Natural Science Foundation of China

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