DataVXACS Applied Materials & InterfacesPaper
journal article·2021-07-07

Development of Diketopyrrolopyrrole-Based Smart Inks by Substituting Ionic Pendants and Engineering Molecular Packing Structures

Seok-In Lim, Jahyeon Koo, Junhwa Jang, Mintaek Oh, Duy Thanh Tran, Sungjune Park, Yan Cao, Dae-Yoon Kim, Kwang-Un Jeong

ACS Applied Materials & Interfaces· Volume 13· Issue 26
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Source abstract

Abstract

A series of diketopyrrolopyrrole (DPP) luminogen amphiphiles were newly designed and synthesized by a single-step anionic exchange reaction for controlling the photoluminescence properties in both solution and solid states. Multicolor emission in response to thermal, mechanical, and chemical stimuli was successfully demonstrated by engineering well-defined supramolecular assemblies. Phase transformation from the metastable amorphous solid to the stable orthorhombic crystal of [DP-Im][Br] provided the reversibly patternable light emission. Self-organization into the smectic crystalline phase of [DP-Im][TFSI] allowed us to show the linearly polarized light emission. By simultaneously applying [DP-Im][Br] and [DP-Im][TFSI], we demonstrated the fabrication of smart sensors for packaging of food or vaccines that can detect thermal attacks.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Luminescence and Fluorescent Materials · Polydiacetylene-based materials and applications · Supramolecular Self-Assembly in Materials

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Polymer-Nano Science and Technology, Department of Nano Convergence Engineering, Jeonbuk National University, Jeonju 54896, Republic of Korea

Institute for Advanced Study, Shenzhen University, Guangdong 518060, China

Functional Composite Materials Research Center, Korea Institute of Science and Technology, Bongdong, Jeonbuk 55324, Republic of Korea

Funding

Korea Agency for Infrastructure Technology Advancement · Korea Government MSIT · Materials and Components Technology Development Program · Basic Research Laboratory Program · Mid-Career Researcher Program

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