journal article·2026-03-25Open access

Stack-Engineered Mode Selection in PtMn/(Co/Pd) n Multilayers Enables Deterministic Analog Spin–Orbit Torque Synapses

Abhijeet Ranjan, Tamkeen Farooq, Chong-Chi Chi, Chao-Chin Wang, Yu-Lon Lin, Rudis Ismael Salinas Padilla, Ying-Hung Li, Yuan-Chieh Tseng, Chih-Hao Lee, Ming-Yen Lu, Rahul Mishra, Chih-Huang Lai

ACS Applied Materials & Interfaces· Volume 18· Issue 11

Abstract

High Resolution Image Download MS PowerPoint Slide Spin–orbit-torque (SOT) devices that support both binary and analog switching can bridge spintronic memory and neuromorphic computing, provided the switching mode can be deliberately assigned. Here, we demonstrate that in PtMn/(Co/Pd)n multilayers, the Co/Pd repeat number, n Co/Pd, serves as a material parameter that determines the reversal mechanism and switching mode. For n Co/Pd ≤ 7, magnetization reversal is governed by nucleation followed by domain-wall propagation, resulting in binary switching that can undergo a transition to analog behavior through electrical conditioning. For n Co/Pd ≥ 8, increased structural modulation in the as-deposited state suppresses domain-wall propagation and stabilizes nucleation-dominated analog switching without additional processing. Applying controlled current conditioning to these high-n Co/Pd stacks produces a hybrid state with smoother long-term potentiation and depression, an expanded number of intermediate states, and neuromorphic classification accuracy exceeding 97%. These results establish stack design and hybrid tuning as scalable strategies for energy-efficient analog SOT synapses in neuromorphic hardware.
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Research context

OpenAlex topics: Magnetic properties of thin films · Advanced Memory and Neural Computing · Ferroelectric and Negative Capacitance Devices

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Affiliations

Department of Materials Science and Engineering

National Tsing Hua University

Centre for Applied Research in Electronics

Indian Institute of Technology Delhi

Instrumentation Center

Department of Engineering and System Science

Department of Materials Science & Engineering

National Yang-Ming Chiao-Tung University

Institute of Space Systems Engineering

College of Semiconductor Research

Funding

National Science and Technology Council

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