journal article·2025-12-03Open access

Circular Carbon Nanotube Production for Advanced Structural Fiber Applications

Xiao Sun, Di Chang, Varunkumar Thippanna, Xiaoli Li, Aidin Panahi, Huidong Dai, Hongyi Wang, Jianlin Li, Yunzheng Yang, Arunachalam Ramanathan, Wentao Liang, Yiannis Levendis, Kenan Song, Marilyn Minus

ACS Applied Materials & Interfaces· Volume 17· Issue 48

Abstract

Plastic waste accumulation remains a global challenge, with only a small fraction currently being recycled. Upcycling postconsumer plastics into value-added materials offers a sustainable solution for waste reduction and advanced manufacturing. In this study, we demonstrate a cost-effective method for synthesizing multiwalled carbon nanotubes (MWCNTs) from postconsumer plastics via catalytic chemical vapor deposition. The waste-derived MWCNTs were incorporated into polyacrylonitrile (PAN) through wet spinning to fabricate high-performance composite fibers. Compared to conventional PAN-based fibers that use commercially sourced CNTs, which often contain residual catalysts that weaken performance, the synthesized MWCNTs exhibit lower metal content and enhanced crystallinity (66%), reducing defects and improving composite integrity. The resulting PAN-MWCNT fibers achieved a Young's modulus of 13.4 GPa and tensile strength of 941 MPa. This work provides a dual benefit: mitigating plastic waste while producing high-value carbon nanomaterials, offering a sustainable route to manufacture lightweight, high-performance fibers applicable in aerospace, automotive, and energy sectors.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Fiber-reinforced polymer composites · Carbon Nanotubes in Composites · Natural Fiber Reinforced Composites

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Mechanical and Industrial Engineering, Northeastern University, 360 Huntington Avenue, Boston, Massachusetts 02115, United States

Mechanical Engineering, College of Engineering, University of Georgia, 302 E Campus Rd, Athens, Georgia 30602, United States

Chemical Engineering Department

Worcester Polytechnic Institute

Department of Chemistry and Chemical Biology

Northeastern University

Kennedy College of Sciences, University of Massachusetts Lowell, 220 Pawtucket Street, Lowell, Massachusetts 01854, United States

Kostas Advanced Nanocharacterization Facility (KANCF)

Mechanical Engineering, College of Engineering, University of Georgia (UGA), 302 E. Campus Rd., Athens, Georgia 30602, United States

Funding

Air Force Office of Scientific Research · Cannon

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