Blatter Radical-Decorated Silica as a Prospective Adsorbent for Selective NO Capture from Air

Artem S. Poryvaev; Eva Gjuzi; Anastasiya A. Yazikova; Daniil M. Polyukhov; Yana N. Albrekht; Aleksandr A. Efremov; Nikita A. Kudriavykh; Vadim V. Yanshole; Frank Hoffmann; Michael Fröba; Matvey V. Fedin

doi:10.1021/acsami.2c19183

journal article·2023-02-01

Blatter Radical-Decorated Silica as a Prospective Adsorbent for Selective NO Capture from Air

Artem S. Poryvaev, Eva Gjuzi, Anastasiya A. Yazikova, Daniil M. Polyukhov, Yana N. Albrekht, Aleksandr A. Efremov, Nikita A. Kudriavykh, Vadim V. Yanshole, Frank Hoffmann, Michael Fröba, Matvey V. Fedin

ACS Applied Materials & Interfaces· Volume 15· Issue 4

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Source abstract

Abstract

Nitrogen oxides are adverse poisonous gases present in the atmosphere and having detrimental effects on the human health and environment. In this work, we propose a new type of mesoporous materials capable of capturing nitrogen monoxide (NO) from air. The designed material combines the robust Santa Barbara Amorphous-15 silica scaffold and ultrastable Blatter-type radicals acting as NO traps. Using in situ electron paramagnetic resonance spectroscopy, we demonstrate that NO capture from air is selective and reversible at practical conditions, thus making Blatter radical-decorated silica highly promising for environmental applications.

Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Mesoporous Materials and Catalysis · Catalytic Processes in Materials Science · Lanthanide and Transition Metal Complexes

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

International Tomography Center SB RAS, Institutskaya Street 3a, Novosibirsk, 630090, Russia

Institute of Inorganic and Applied Chemistry, University of Hamburg, Martin-Luther-King-Platz 6, 20146 Hamburg, Germany

Novosibirsk State University, Pirogova Street 2, 630090 Novosibirsk, Russia

Funding

Deutsche Forschungsgemeinschaft · Russian Foundation for Basic Research

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