journal article·2018-01-10

In Situ Characterization of Photothermal Nanoenergetic Combustion on a Plasmonic Microchip

Biyan Chen, Haisheng Zheng, Matthew Riehn, Sangho Bok, Keshab Gangopadhyay, Matthew R. Maschmann, Shubhra Gangopadhyay

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Abstract

Plasmonic gratings facilitate a robust in situ diagnostic platform for photothermal combustion of nanoenergetic composite thin films using an optical microscope and a high-speed camera. Aluminum nanoparticles (Al NPs) embedded in a fluoropolymer oxidizer are cast onto a plasmonic grating microchip and ignited using a low-power laser. The plasmonic grating enhances both spatial resolution and sufficient photothermal coupling to combust small Al NP clusters, initiating localized flames as small as 600 nm in size. Two-color pyrometry obtained from a high-speed color camera indicates an average flame temperature of 3900 K. Scattering measurements using polarized light microscopy enabled precise identification of individual Al NPs over a large field of view, leading to 3D reconstruction of combustion events.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: nanoparticles nucleation surface interactions · Plasmonic and Surface Plasmon Research · Thermal Radiation and Cooling Technologies

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Engineering and Technology, Southern Utah University, Cedar City, Utah 84720, United States

Funding

Army Research Office

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