journal article·2015-09-23

Ultrathin Wrinkled N-Doped Carbon Nanotubes for Noble-Metal Loading and Oxygen Reduction Reaction

Jiehua Liu, Anli Shen, Xiangfeng Wei, Kuan Zhou, Wei Chen, Fang Chen, Jiaqi Xu, Shuangyin Wang, Liming Dai

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Abstract

We describe the fabrication of ultrathin wrinkled N-doped carbon nanotubes by an in situ solid-state method. The positions of Co catalyst were first labeled by good-dispersion and highly loaded Au and Pt, indicating the most of Co are unsealed. The resultant unique nanoarchitecture, which exhibits the features of carbon nanotube and graphene with a combined effect of 1D and 2D carbon-based nanostructures, exhibited a superior ORR activity to carbon nanotubes and graphene. Moreover, the novel catalysts showed a better durability and higher tolerance to methanol crossover and poisoning effects than those of Pt/C.
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Research context

OpenAlex topics: Electrocatalysts for Energy Conversion · Supercapacitor Materials and Fabrication · Advanced battery technologies research

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Future Energy Laboratory, School of Materials Science and Engineering, Hefei University of Technology, 193 Tunxi Road, Hefei, Anhui 230009, China

State Key Laboratory of Chem/Bio-Sensing and Chemometrics, College of Chemistry and Chemical Engineering, Hunan University, Changsha 410082 P.R. China

Department of Macromolecular Engineering, Case Western Reserve University, Cleveland, Ohio 44106, United States

Funding

National Natural Science Foundation of China · Ministry of Education of the People's Republic of China · Anhui Province

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