journal article·2021-05-19Open access

Enhanced Spin-to-Charge Conversion Efficiency in Ultrathin Bi2Se3 Observed by Spintronic Terahertz Spectroscopy

Hanbum Park, Kwangsik Jeong, InHee Maeng, Kyung Ik Sim, Sachin Pathak, Jonghoon Kim, Seok-Bo Hong, Taek Sun Jung, Chul Kang, Jae Hoon Kim, Jongill Hong, Mann-Ho Cho

ACS Applied Materials & Interfaces· Volume 13· Issue 19

Abstract

Owing to their remarkable spin–charge conversion (SCC) efficiency, topological insulators (TIs) are the most attractive candidates for spin–orbit torque generators. The simple method of enhancing SCC efficiency is to reduce the thickness of TI films to minimize the trivial bulk contribution. However, when the thickness reaches the ultrathin regime, the SCC efficiency decreases owing to intersurface hybridization. To overcome these contrary effects, we induced dehybridization of the ultrathin TI film by breaking the inversion symmetry between surfaces. For the TI film grown on an oxygen-deficient transition-metal oxide, the unbonded transition-metal d-orbitals affected only the bottom surface, resulting in asymmetric surface band structures. Spintronic terahertz emission spectroscopy, an emerging tool for investigating the SCC characteristics, revealed that the resulting SCC efficiency in symmetry-broken ultrathin Bi2Se3 was enhanced by up to ∼2.4 times.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Topological Materials and Phenomena · Magnetic properties of thin films · Atomic and Subatomic Physics Research

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Physics, Yonsei University, Seoul 03722, Republic of Korea

Division of Physics and Semiconductor Science, Dongguk University, Seoul 04620, Republic of Korea

YUHS-KRIBB, Medical Convergence Research Institute, College of Medicine, Yonsei University, Seoul 03722, Republic of Korea

Center for Integrated Nanostructure Physics (CINAP), Institute for Basic Science (IBS), Suwon 16419, Republic of Korea

Department of Physics, School of Engineering, University of Petroleum and Energy Studies, Dehradun 248007, Uttarakhand, India

Department of Materials Science and Engineering, Yonsei University, Seoul 03722, Republic of Korea

Advanced Photonics Research Institute, Gwangju Institute of Science and Technology, Gwangju 61005, Republic of Korea

Funding

National Research Foundation of Korea

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