journal article·2016-12-14

Construction of a Unique Two-Dimensional Hierarchical Carbon Architecture for Superior Lithium-Ion Storage

Zhijie Wang, Xiaoliang Yu, Wenhui He, Yusuf Valentino Kaneti, Da Han, Qi Sun, Yan-Bing He, Bin Xiang

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Abstract

Two-dimensional nanocarbons are intriguing functional materials for energy storage. However, the serious aggregation problems hinder their wider applications. To address this issue, we developed a unique two-dimensional hierarchical carbon architecture (2D-HCA) with ultrasmall graphene-like carbon nanosheets uniformly grown on hexagonal carbon nanoplates. The obtained 2D-HCA shows an interconnected porous structure and abundant heteroelement doping. When employed as anode for lithium ion batteries, it exhibits a high discharge capacity of 748 m Ah g –1 even after 400 cycles at 2 A g –1 .
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Research context

OpenAlex topics: Advancements in Battery Materials · Supercapacitor Materials and Fabrication · Advanced Battery Materials and Technologies

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Materials Science & Engineering, CAS Key Lab of Materials for Energy Conversion, Synergetic Innovation Center of Quantum Information Quantum Physics, University of Science and Technology of China, Hefei, Anhui 230026, China

Engineering Laboratory for the Next Generation Power and Energy Storage Batteries, and Engineering Laboratory for Functionalized Carbon Materials, Graduate School at Shenzhen, Tsinghua University, Shenzhen 100084, China

Laboratory of Physics and Chemistry of Nano-Objects (LPCNO), Institut National des Sciences Appliquées de Toulouse (INSA), Paul Sabatier University-Toulouse III, Toulouse 31062, France

Funding

Ministry of Science and Technology of the People's Republic of China · Tsinghua University · Dongguan City · Guangdong Province · Shenzhen City

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