journal article·2019-10-02

Broadband Nonlinear Optical Response of Single-Crystalline Bismuth Thin Film

Lin Du, Donglin Lu, Jie Li, Ke Yang, Lingling Yang, Bin Huang, Jun Yi, Qian Yi, Lili Miao, Xiang Qi, Chujun Zhao, Jianxin Zhong, Shuangchun Wen

ACS Applied Materials & Interfaces· Volume 11· Issue 39
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Abstract

Bismuth (Bi), a topological material, where many interesting condensed matter phenomena have been observed, possesses unique physical properties when its thickness is reduced to thin film. Here, we prepared the highly stable, single-crystalline, continuous Bi thin film via the vapor deposition (VD) method and found that the Bi thin film can exhibit broadband, ultrafast nonlinear optical response with low saturable intensity ranging from the near-infrared to mid-infrared spectral range under strong excitation. Moreover, we demonstrated that the Bi thin film was favorable to act as a nonlinear pulse modulator toward a high performance pulsed laser operating in optical communication and mid-infrared wavelengths. The experimental results highlight the prospects of Bi thin film as broadband pulsed modulators and may open new avenues toward advanced Bi-based broadband photonic devices.
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Research context

OpenAlex topics: Advanced Fiber Laser Technologies · Laser-Matter Interactions and Applications · Photorefractive and Nonlinear Optics

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Key Laboratory for Micro/Nano Optoelectronic Devices of Ministry of Education & Hunan Provincial Key Laboratory of Low-Dimensional Structural Physics and Devices, School of Physics and Electronics, Hunan University, Changsha 410082, China

Hunan Key Laboratory for Micro-Nano Energy Materials and Devices, Laboratory for Quantum Engineering and Micro-Nano Energy Technology, and School of Physics and Optoelectronics, Xiangtan University, Xiangtan 411105, China

Funding

Natural Science Foundation of?Hunan Province · National Natural Science Foundation of China · Science and Technology on Plasma Physics Laboratory, China Academy of Engineering Physics

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