Nanoparticle-Based Magnetorheological Elastomers with Enhanced Mechanical Deflection for Haptic Displays

Haptics allows tactile interactions between humans and digital interfaces. Magnetorheological elastomers (MREs) constitute a promising candidate material for creating the tactile interface of the future─one able to recreate 3D shapes that can be sensed with touch. Furthermore, an MRE formed by using nanoparticles, as opposed to previously used microparticles, is necessary to generate a variety of shapes involving sharp curvatures over small, micrometer-scale horizontal distances to pave the way for haptic displays with microtexture resolution. Here we fabricated both isotropic and anisotropic MREs with different concentrations (2-8 vol % nanoparticles) of soft, low-remanence ferromagnetic nanoparticles. When placed in a magnetic field gradient, isotropic MREs, nonintuitively, show higher deflection than anisotropic MREs, with the former achieving displacement on the order of a millimeter at just 100 mT. This enhanced performance in the isotropic case is explained based on the soft magnetic nature of the nanoparticles. We show that performance improves with magnetic content up to a composition of 6 vol %, where it plateaus. This behavior is attributed to the stiffness of the composite material increasing at a faster rate than the magnetization as the rigid magnetic nanoparticles are added to the elastomeric matrix. Moreover, 6 vol % microparticle-based isotropic and anisotropic MREs were fabricated and compared with the nanoparticle-based MREs. Anisotropic nanoparticle-based films show higher deflection when compared with their microparticle-based counterparts. The latter is only able to match the nanoparticle film deflection at higher applied fields of almost 300 mT. This performance difference between nanoparticle and microparticle-based films is attributed to the increased anisotropic film stiffness resulting from the larger micrometer-size particles. Finally, the optimally designed nanoparticle-based isotropic film was utilized to create a programmable and real-time reconfigurable braille-inspired interface.