journal article·2022-06-29

High Spatial Resolution Thermal Mapping of Volatile Switching in NbOx-Based Memristor Using In Situ Scanning Thermal Microscopy

Sanjoy Kumar Nandi, Etienne Puyoo, Shimul Kanti Nath, David Albertini, Nicolas Baboux, Sujan Kumar Das, Thomas Ratcliff, Robert G. Elliman

ACS Applied Materials & Interfaces· Volume 14· Issue 25
Publisher page

Abstract

Temperature mapping by in situ thermoreflectance thermal imaging (TRTI) or midwave infrared spectroscopy has played an important role in understanding the origins of threshold switching and the effect of insulator–metal transitions in oxide-based memrsitive devices. In this study, we use scanning thermal microscopy (SThM) as an alternative thermal mapping technique that offers high spatial resolution imaging (∼100 nm) and is independent of material. Specifically, SThM is used to map the temperature distribution in NbOx-based cross-bar and nanovia devices with Pt top electrodes. The measurements on cross-bar devices reproduce the current redistribution and confinement processes previously observed by TRTI but without the need to coat the electrodes with a material of high thermo-reflectance coefficient (e.g., Au), while those on the nanovia devices highlight the spatial resolution of the technique. The measured temperature distributions are compared with those obtained from physics-based finite-element simulations and suggest that thermal boundary resistance plays an important role in heat transfer between the active device volume and the top electrode.
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Research context

OpenAlex topics: Advanced Memory and Neural Computing · Thermal properties of materials · Transition Metal Oxide Nanomaterials

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Affiliations

Department of Electronic Materials Engineering, Research School of Physics, Australian National University, Canberra, Australian Capital Territory 2601, Australia

Université Lyon, INSA Lyon, CNRS, Ecole Centrale de Lyon, Université Claude Bernard Lyon 1, CPE Lyon, INL, UMR5270, 69621 Villeurbanne, France

Department of Electrical, Electronic and Computer Engineering, The University of Western Australia, Crawley, Western Australia 6009, Australia

Department of Physics, Jahangirnagar University, Dhaka 1342, Bangladesh

Funding

Australian Research Council · Forrest Research Foundation · Lyon Institute of Nanotechnologies

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