Hybrid Metal–Organic Frameworks Encapsulated Hybrid Ni-Doped CdS Nanoparticles for Visible-Light-Driven CO₂ Reduction

Heng-Zhi Liu; Xiao Liu; Bo Li; Haiqiang Luo; Jian-Gong Ma; Peng Cheng

doi:10.1021/acsami.2c08776

journal article·2022-06-22

Hybrid Metal–Organic Frameworks Encapsulated Hybrid Ni-Doped CdS Nanoparticles for Visible-Light-Driven CO₂ Reduction

Heng-Zhi Liu, Xiao Liu, Bo Li, Haiqiang Luo, Jian-Gong Ma, Peng Cheng

ACS Applied Materials & Interfaces· Volume 14· Issue 24

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Abstract

The photocatalytic production of syngas from CO2 and water is an attractive and straightforward way for both solar energy storage and sustainable development. Here, we combined the hybrid shell of a bimetallic metal–organic framework (MOF) Zn/Co-zeolitic imidazolate framework (ZIF) and the hybrid photoactive center of Ni-doped CdS nanoparticles (Ni@CdS) to construct a new “2 + 2” photocatalysis system Ni@CdS⊂Zn/Co-ZIF through a facile self-assembly process, which exhibited a double-synergic effect for visible light harvesting and CO2 conversion, leading to one of the highest photocatalytic syngas production rates and excellent recyclability. The H2/CO of syngas ratios can be readily adjusted by controlling the ratio of Zn/Co in the hybrid MOF shell.

Source: openalex_inverted_index · Quality: baseline

Research context

Nanomaterials Catalysis & surfaces

OpenAlex topics: Advanced Photocatalysis Techniques · Metal-Organic Frameworks: Synthesis and Applications · CO2 Reduction Techniques and Catalysts

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Key Laboratory of Advanced Energy Materials Chemistry (MOE), Haihe Laboratory of Sustainable Chemical Transformations (Tianjin), Renewable Energy Conversion and Storage Center, College of Chemistry, Nankai University, Tianjin 300071, China

Funding

Central University Basic Research Fund of China · National Natural Science Foundation of China

References (68)

Show source-provided references

1. 10.1038/nature1572510.1038/nature15725 ↗

2. 10.1039/C8CS00829A10.1039/C8CS00829A ↗

3. 10.1038/nmat483410.1038/nmat4834 ↗

4. 10.3389/fpubh.2020.0001410.3389/fpubh.2020.00014 ↗

5. 10.1016/j.ccr.2020.21326210.1016/j.ccr.2020.213262 ↗

6. 10.1002/anie.20200362310.1002/anie.202003623 ↗

7. 10.1016/j.apcatb.2021.11997610.1016/j.apcatb.2021.119976 ↗

8. 10.1002/anie.20211067010.1002/anie.202110670 ↗

9. 10.1016/j.apcatb.2020.11983410.1016/j.apcatb.2020.119834 ↗

10. 10.1039/C9NR10451H10.1039/C9NR10451H ↗

11. 10.1007/s12274-018-2240-410.1007/s12274-018-2240-4 ↗

12. 10.1002/anie.20201515910.1002/anie.202015159 ↗

13. 10.1021/acscatal.8b0079110.1021/acscatal.8b00791 ↗

14. 10.1038/s41563-019-0501-610.1038/s41563-019-0501-6 ↗

15. 10.1016/j.cej.2020.12836210.1016/j.cej.2020.128362 ↗

16. 10.1016/j.apcatb.2019.01.01410.1016/j.apcatb.2019.01.014 ↗

17. 10.1021/acsami.1c0825110.1021/acsami.1c08251 ↗

18. 10.1002/anie.20160642410.1002/anie.201606424 ↗

19. 10.1038/s41929-020-00510-z10.1038/s41929-020-00510-z ↗

20. 10.1039/D1TA04418D10.1039/D1TA04418D ↗

21. 10.1002/adfm.20200800810.1002/adfm.202008008 ↗

22. 10.1016/j.cej.2021.12934410.1016/j.cej.2021.129344 ↗

23. 10.1039/C8EE02538J10.1039/C8EE02538J ↗

24. 10.1038/s41560-018-0229-610.1038/s41560-018-0229-6 ↗

25. 10.1002/adma.20190070910.1002/adma.201900709 ↗

26. 10.1002/adma.20170462410.1002/adma.201704624 ↗

27. 10.1016/j.jcis.2021.07.15010.1016/j.jcis.2021.07.150 ↗

28. 10.1016/j.apsusc.2016.06.14810.1016/j.apsusc.2016.06.148 ↗

29. 10.1002/cssc.20180058310.1002/cssc.201800583 ↗

30. 10.1002/anie.20181055010.1002/anie.201810550 ↗

31. 10.1038/s41563-018-0033-510.1038/s41563-018-0033-5 ↗

32. 10.1002/anie.20180158810.1002/anie.201801588 ↗

33. 10.1021/acs.chemrev.9b0022310.1021/acs.chemrev.9b00223 ↗

34. 10.1002/smll.20180484910.1002/smll.201804849 ↗

35. 10.1016/j.chempr.2018.12.01110.1016/j.chempr.2018.12.011 ↗

36. 10.1021/acsami.1c0084410.1021/acsami.1c00844 ↗

37. 10.1021/acs.chemrev.9b0075710.1021/acs.chemrev.9b00757 ↗

38. 10.1002/ange.20211673610.1002/ange.202116736 ↗

39. 10.1002/aenm.20200305210.1002/aenm.202003052 ↗

40. 10.1002/adma.20170551210.1002/adma.201705512 ↗

41. 10.1039/C6CS00250A10.1039/C6CS00250A ↗

42. 10.1021/jacs.0c0590910.1021/jacs.0c05909 ↗

43. 10.1039/D1QI00543J10.1039/D1QI00543J ↗

44. 10.1002/anie.20201573510.1002/anie.202015735 ↗

45. 10.1021/jacs.0c0959910.1021/jacs.0c09599 ↗

46. 10.1021/jacs.0c0553010.1021/jacs.0c05530 ↗

47. 10.1038/s41586-020-2738-210.1038/s41586-020-2738-2 ↗

48. 10.1002/anie.20201106810.1002/anie.202011068 ↗

49. 10.1021/acsenergylett.8b0165810.1021/acsenergylett.8b01658 ↗

50. 10.1016/j.jcou.2019.07.01110.1016/j.jcou.2019.07.011 ↗

51. 10.1002/solr.20190044010.1002/solr.201900440 ↗

52. 10.1021/acsaem.0c0108310.1021/acsaem.0c01083 ↗

53. 10.1021/jacs.7b1158910.1021/jacs.7b11589 ↗

54. 10.1039/C6TA07860E10.1039/C6TA07860E ↗

55. 10.1039/C6TA04342A10.1039/C6TA04342A ↗

56. 10.1002/anie.20191360010.1002/anie.201913600 ↗

57. Frisch, M. J.; Trucks, G. W.; Schlegel, H. B.; Scuseria, G. E.; Robb, M. A.; Cheeseman, J. R.; Scalmani, G.; Barone, V.; Petersson, G. A.; Nakatsuji, H.; Li, X.; Caricato, M.; Marenich, A. V.; Bloino, J.; Janesko, B. G.; Gomperts, R.; Mennucci, B.; Hratchian, H. P.; Ortiz, J. V.; Izmaylov, A. F.; Sonnenberg, J. L.; Ding, F.; Lipparini, F.; Egidi, F.; Goings, J.; Peng, B.; Petrone, A.; Henderson, T.; Ranasinghe, D.; Zakrzewski, V. G.; Gao, J.; Rega, N.; Zheng, G.; Liang, W.; Hada, M.; Ehara, M.; Toyota, K.; Fukuda, R.; Hasegawa, J.; Ishida, M.; Nakajima, T.; Honda, Y.; Kitao, O.; Nakai, H.; Vreven, T.; Throssell, K.; Montgomery, J. A., Jr.; Peralta, J. E.; Ogliaro, F.; Bearpark, M. J.; Heyd, J. J.; Brothers, E. N.; Kudin, K. N.; Staroverov, V. N.; Keith, T. A.; Kobayashi, R.; Normand, J.; Raghavachari, K.; Rendell, A. P.; Burant, J. C.; Iyengar, S. S.; Tomasi, J.; Cossi, M.; Millam, J. M.; Klene, M.; Adamo, C.; Cammi, R.; Ochterski, J. W.; Martin, R. L.; Morokuma, K.; Farkas, O.; Foresman, J. B.; Fox, D. J. Gaussian 16, revision C.01, Wallingford, CT, 2016.

58. 10.1103/PhysRevA.38.309810.1103/PhysRevA.38.3098 ↗

59. 10.1007/BF0053348510.1007/BF00533485 ↗

60. 10.1063/1.44879910.1063/1.448799 ↗

61. 10.1016/j.jechem.2020.12.02510.1016/j.jechem.2020.12.025 ↗

62. 10.1039/C8TA00154E10.1039/C8TA00154E ↗

63. 10.1038/s41467-021-25007-610.1038/s41467-021-25007-6 ↗

64. 10.1016/j.carbon.2022.01.01910.1016/j.carbon.2022.01.019 ↗

65. 10.1016/j.cej.2021.13303910.1016/j.cej.2021.133039 ↗

66. 10.1002/smll.20200298810.1002/smll.202002988 ↗

67. 10.1016/j.apcatb.2014.07.02610.1016/j.apcatb.2014.07.026 ↗

68. 10.1016/j.jcat.2021.03.01810.1016/j.jcat.2021.03.018 ↗