journal article·2020-10-21Open access

Flexible and Green Electronics Manufactured by Origami Folding of Nanosilicate-Reinforced Cellulose Paper

Firoz Babu Kadumudi, Jon Trifol, Mohammadjavad Jahanshahi, Tiberiu-Gabriel Zsurzsan, Mehdi Mehrali, Eva Zeqiraj, Hossein Shaki, Morteza Alehosseini, Carsten Gundlach, Qiang Li, Mingdong Dong, Mohsen Akbari, Arnold Knott, Kristoffer Almdal, Alireza Dolatshahi-Pirouz

ACS Applied Materials & Interfaces· Volume 12· Issue 42

Abstract

Today’s consumer electronics are made from nonrenewable and toxic components. They are also rigid, bulky, and manufactured in an energy-inefficient manner via CO2-generating routes. Though petroleum-based polymers such as polyethylene terephthalate and polyethylene naphthalate can address the rigidity issue, they have a large carbon footprint and generate harmful waste. Scalable routes for manufacturing electronics that are both flexible and ecofriendly (Fleco) could address the challenges in the field. Ideally, such substrates must incorporate into electronics without compromising device performance. In this work, we demonstrate that a new type of wood-based [nanocellulose (NC)] material made via nanosilicate (NS) reinforcement can yield flexible electronics that can bend and roll without loss of electrical function. Specifically, the NSs interact electrostatically with NC to reinforce thermal and mechanical properties. For instance, films containing 34 wt % of NS displayed an increased young’s modulus (1.5 times), thermal stability (290 → 310 °C), and a low coefficient of thermal expansion (40 ppm/K). These films can also easily be separated and renewed into new devices through simple and low-energy processes. Moreover, we used very cheap and environmentally friendly NC from American Value Added Pulping (AVAP) technology, American Process, and therefore, the manufacturing cost of our NS-reinforced NC paper is much cheaper ($0.016 per dm–2) than that of conventional NC-based substrates. Looking forward, the methodology highlighted herein is highly attractive as it can unlock the secrets of Fleco electronics and transform otherwise bulky, rigid, and “difficult-to-process” rigid circuits into more aesthetic and flexible ones while simultaneously bringing relief to an already-overburdened ecosystem.
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Research context

OpenAlex topics: Advanced Cellulose Research Studies · Electrospun Nanofibers in Biomedical Applications · Advanced Sensor and Energy Harvesting Materials

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Health Technology, Technical University of Denmark (DTU), 2800 Kgs. Lyngby, Denmark

Danish Polymer Center, Department of Chemical Engineering, Technical University of Denmark (DTU), 2800 Kgs. Lyngby, Denmark

Student Research Committee, School of Medicine, Bam University of Medical Sciences, 4340847 Bam, Iran

Department of Marine Chemistry, Faculty of Marine Science, Chabahar Maritime University, 9971756499 Chabahar, Iran

Department of Electrical Engineering, Technical University of Denmark, 2800 Kgs. Lyngby, Denmark

Department of Health Technology, Institute of Biotherapeutic Engineering and Drug Targeting, Center for Intestinal Absorption and Transport of Biopharmaceuticals, Technical University of Denmark, 2800 Kgs. Lyngby, Denmark

Department of Mechanical Engineering, Technical University of Denmark, 2800 Kgs. Lyngby, Denmark

Department of Physics, DTU Physics, Technical University of Denmark, 2800 Kgs. Lyngby, Denmark

Biomedical Engineering Division, Faculty of Chemical Engineering, Tarbiat Modares University, P.O. Box, 14115-111 Tehran, Iran

Interdisciplinary Nanoscience Centre, Aarhus University, 8000 Aarhus, Denmark

School of Chemistry and Chemical Engineering, Shandong University, 250100 Jinan, China

Laboratory for Innovations in MicroEngineering (LiME), Department of Mechanical Engineering, University of Victoria, BC V8P 5C2 Victoria, Canada

Center for Advanced Materials and Related Technologies (CAMTEC), University of Victoria, BC V8P 5C2 Victoria, Canada

Department of Chemistry, Technical University of Denmark (DTU), 2800 Kgs. Lyngby, Denmark

Radboud Institute for Molecular Life Sciences, Department of Dentistry—Regenerative Biomaterials, Radboud University Medical Center, Philips van Leydenlaan 25, 6525EX Nijmegen, The Netherlands

Funding

Canadian Institutes of Health Research · Teknologi og Produktion, Det Frie Forskningsr?d · Villum Fonden · Nederlandse Organisatie voor Wetenschappelijk Onderzoek

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