journal article·2020-01-22

Specific Recognition of Uranyl Ion Employing a Functionalized Nanochannel Platform for Dealing with Radioactive Contamination

Linsen Yang, Yongchao Qian, Xiang-Yu Kong, Mengting Si, Yuanyuan Zhao, Bo Niu, Xiaolu Zhao, Yan Wei, Lei Jiang, Liping Wen

Publisher page

Abstract

Radioactive contamination is a highly concerning global environmental issue along with the development of the nuclear industry. On account of sophisticated operations and high cost of instrument detection methods, numerous efforts have been focused on rapid and simple detection of pollution elements and uranium is the most common one. It is an enormous challenge to push the limit of determination as low as possible while carrying out ultrasensitive detection. Here, we report an intelligent platform based on functionalized solid nanochannels to monitor ultratrace uranyl ions. The platform has a detection limit of 1 fM, which is far below the value that traditional instrumental methods can reach. What is more, the system also exhibits uranyl removal property. The mesenchymal stem cells cultivated in media containing uranyl can achieve excellent viability in the presence of the membranes. This work provides a new choice for handling global radioactive contamination of water.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Radioactive element chemistry and processing · Groundwater flow and contamination studies · Nanopore and Nanochannel Transport Studies

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Key Laboratory of Bio-inspired Materials and Interfacial Science, Technical Institute of Physics and Chemistry, Chinese Academy of Sciences, Beijing 100190, P. R. China

School of Future Technology, University of Chinese Academy of Sciences, Beijing 100049, P. R. China

Shanxi Key Laboratory of Macromolecular Science and Technology, School of Science, Northwestern Polytechnical University, Xi’an 710072, P. R. China

Beijing Laboratory of Biomedical Materials, Department of Geriatric Dentistry, Peking University School and Hospital of Stomatology, Beijing 100081, P. R. China

Funding

Ministry of Science and Technology of the People's Republic of China · Natural Science Foundation of Beijing Municipality · Beijing Municipal Science and Technology Commission · National Natural Science Foundation of China · Chinese Academy of Sciences

References (63)

Show source-provided references
1. 10.1080/01496395.2012.71259910.1080/01496395.2012.712599 ↗
2. 10.3390/ijerph701030310.3390/ijerph7010303 ↗
3. 10.1039/C4SC02022G10.1039/C4SC02022G ↗
4. 10.1021/es048344310.1021/es0483443 ↗
5. 10.1021/ac60138a00210.1021/ac60138a002 ↗
6. 10.1007/BF0124233110.1007/BF01242331 ↗
7. 10.1007/BF0278977110.1007/BF02789771 ↗
8. 10.1007/s10967-014-3306-810.1007/s10967-014-3306-8 ↗
9. 10.1016/j.talanta.2019.04.01810.1016/j.talanta.2019.04.018 ↗
10. 10.1021/acsami.6b1342710.1021/acsami.6b13427 ↗
11. 10.1039/C8EN01396A10.1039/C8EN01396A ↗
12. 10.1073/pnas.060787510410.1073/pnas.0607875104 ↗
13. 10.1007/s00604-019-3625-010.1007/s00604-019-3625-0 ↗
14. 10.1021/acs.est.6b0630510.1021/acs.est.6b06305 ↗
15. 10.1021/acs.est.8b0472810.1021/acs.est.8b04728 ↗
16. 10.1038/ncomms1536910.1038/ncomms15369 ↗
17. 10.1002/anie.20190971810.1002/anie.201909718 ↗
18. 10.1007/s00604-019-3426-510.1007/s00604-019-3426-5 ↗
19. 10.1002/anie.20110490410.1002/anie.201104904 ↗
20. 10.1021/acs.analchem.8b0516210.1021/acs.analchem.8b05162 ↗
21. 10.1002/anie.20180322910.1002/anie.201803229 ↗
22. 10.1039/C5CS00819K10.1039/C5CS00819K ↗
23. 10.1021/acs.analchem.9b0189610.1021/acs.analchem.9b01896 ↗
24. 10.1002/ange.20170869510.1002/ange.201708695 ↗
25. 10.1038/s41467-018-06873-z10.1038/s41467-018-06873-z ↗
26. 10.1126/sciadv.aao672410.1126/sciadv.aao6724 ↗
27. 10.1021/jacs.7b1313610.1021/jacs.7b13136 ↗
28. 10.1002/smll.20160035910.1002/smll.201600359 ↗
29. 10.1038/s41427-018-0079-510.1038/s41427-018-0079-5 ↗
30. 10.1039/C7CS00688H10.1039/C7CS00688H ↗
31. 10.1002/smll.20170225210.1002/smll.201702252 ↗
32. 10.1002/adfm.20110214610.1002/adfm.201102146 ↗
33. 10.1039/C5SC02191J10.1039/C5SC02191J ↗
34. 10.1021/jacs.5b1069210.1021/jacs.5b10692 ↗
35. 10.1038/s41467-017-00330-z10.1038/s41467-017-00330-z ↗
36. 10.1039/C5SC04726A10.1039/C5SC04726A ↗
37. 10.1021/acs.chemrev.7b0035510.1021/acs.chemrev.7b00355 ↗
38. 10.1021/jacs.5b0491110.1021/jacs.5b04911 ↗
39. Mercik S. · Acta Phys. Pol. B · 2001 · 32 · 1605
40. 10.1021/nn901402b10.1021/nn901402b ↗
41. 10.1021/acs.iecr.6b0500610.1021/acs.iecr.6b05006 ↗
42. 10.1038/nnano.2011.18910.1038/nnano.2011.189 ↗
43. 10.1021/nl070462b10.1021/nl070462b ↗
44. 10.1007/s10450-005-4816-z10.1007/s10450-005-4816-z ↗
45. 10.1134/S106193481401002X10.1134/S106193481401002X ↗
46. 10.1016/j.aca.2006.08.05210.1016/j.aca.2006.08.052 ↗
47. 10.1016/j.snb.2018.07.09310.1016/j.snb.2018.07.093 ↗
48. 10.1016/j.snb.2016.07.11910.1016/j.snb.2016.07.119 ↗
49. 10.1007/s00604-017-2397-710.1007/s00604-017-2397-7 ↗
50. 10.1016/j.bios.2016.05.00810.1016/j.bios.2016.05.008 ↗
51. 10.1016/j.snb.2015.04.08110.1016/j.snb.2015.04.081 ↗
52. 10.1021/ja803607z10.1021/ja803607z ↗
53. 10.1039/c2an00039c10.1039/c2an00039c ↗
54. 10.1016/j.aca.2016.12.02110.1016/j.aca.2016.12.021 ↗
55. 10.1007/s10967-018-5799-z10.1007/s10967-018-5799-z ↗
56. 10.1016/j.talanta.2018.08.01210.1016/j.talanta.2018.08.012 ↗
57. 10.1016/j.snb.2017.11.01810.1016/j.snb.2017.11.018 ↗
58. 10.1021/acs.analchem.6b0194310.1021/acs.analchem.6b01943 ↗
59. 10.1016/j.saa.2015.02.11310.1016/j.saa.2015.02.113 ↗
60. 10.1016/j.saa.2013.03.03610.1016/j.saa.2013.03.036 ↗
61. 10.1007/s11468-011-9292-610.1007/s11468-011-9292-6 ↗
62. 10.1081/SS-20004299710.1081/SS-200042997 ↗
63. 10.1021/je000013s10.1021/je000013s ↗