Substrate-Independent Epitaxial Growth of the Metal–Organic Framework MOF-508a
Source abstract
Abstract
High Resolution Image Download MS PowerPoint Slide Plasmachemical deposition is a substrate-independent method for the conformal surface functionalization of solid substrates. Structurally well-defined pulsed plasma deposited poly(1-allylimidazole) layers provide surface imidazole linker groups for the directed liquid-phase epitaxial (layer-by-layer) growth of metal–organic frameworks (MOFs) at room temperature. For the case of microporous [Zn (benzene-1,4-dicarboxylate)-(4,4′-bipyridine) 0.5 ] (MOF-508), the MOF-508a polymorph containing two interpenetrating crystal lattice frameworks undergoes orientated Volmer–Weber growth and displays CO 2 gas capture behavior at atmospheric concentrations in proportion to the number of epitaxially grown MOF-508 layers.
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Research context
OpenAlex topics: Metal-Organic Frameworks: Synthesis and Applications · Enhanced Oil Recovery Techniques · Machine Learning in Materials Science
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
Affiliations
Department of Chemistry, Science Laboratories, Durham University, Durham DH1 3LE, U.K.
Department of Chemistry, Indian Institute of Technology Ropar, Punjab 140001, India
Funding
Engineering and Physical Sciences Research Council · Consejo Nacional de Ciencia y Tecnología
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