DataVXACS Applied Materials & InterfacesPaper
journal article·2017-02-01

CO2 Photoreduction by Formate Dehydrogenase and a Ru-Complex in a Nanoporous Glass Reactor

Tomoyasu Noji, Tetsuro Jin, Mamoru Nango, Nobuo Kamiya, Yutaka Amao

ACS Applied Materials & Interfaces· Volume 9· Issue 4
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Source abstract

Abstract

In this study, we demonstrated the conversion of CO 2 to formic acid under ambient conditions in a photoreduction nanoporous reactor using a photosensitizer, methyl viologen (MV 2+ ), and formate dehydrogenase (FDH). The overall efficiency of this reactor was 14 times higher than that of the equivalent solution. The accumulation rate of formic acid in the nanopores of 50 nm is 83 times faster than that in the equivalent solution. Thus, this CO 2 photoreduction nanoporous glass reactor will be useful as an artificial photosynthesis system that converts CO 2 to fuel.
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Research context

Ceramics & glassesNanomaterials

OpenAlex topics: CO2 Reduction Techniques and Catalysts · Advanced Photocatalysis Techniques · Electrocatalysts for Energy Conversion

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

The OCU Advanced Research Institute for Natural Science & Technology (OCARINA), Osaka City University, 3-3-138 Sugimoto, Sumiyoshi-ku, Osaka 558-8585, Japan

Inorganic Functional Materials Research Institute, National Institute of Advanced Industrial Science and Technology (AIST), 1-8-31, Midorigaoka, Ikeda, Osaka 563-8577, Japan

Monozukuri Research Center, Nagoya Institute of Technology, Gokiso-cho, Showa-ku, Nagoya 466-8555, Japan

Funding

Air Force Office of Scientific Research · Japan Society for the Promotion of Science · Takahashi Industrial and Economic Research Foundation · Japan Prize Foundation · Koyanagi Foundation · Iwatani Corporation

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