Graphene Aerogel Broken to Fragments for a Piezoresistive Pressure Sensor with a Higher Sensitivity

The porous and elastic reduced graphene aerogel (rGA) is a promising active material for piezoresistive pressure sensors (PRSs) to realize an electronic skin. Due to the specific working mechanism and the limitation of the rGA's monolithic conductive network, the PRSs based on rGA suffer from a limited change of resistance with mechanical deformation, so they show poor sensitivity and cannot detect low pressures. Here we aim to improve the sensitivity of the PRS and make it suitable for a low-pressure system (0.5-8 kPa) through an effective method. The monolithic rGA is broken into small pieces by cutting (named as CGA). The sensitivity of the PRS based on CGA can be improved by 10 times that of the uncut rGA (named as UCGA). The resistance variation ratio of CGA (0.96) is 1.45 times of the resistance variation ratio of the UCGA (0.66). By using a package of elastic polypropylene thin films (PP), the cycle stability performance of CGA remains stable after 4200 cycles. The CGA can detect the pulse of a human being with sensitivity higher than the UCGA and the ordinary sensors. This method is simple, effective, and universal to improve the sensitivity of PRS based on porous and elastic materials.