All-Nanofibrous Ionic Capacitive Pressure Sensor for Wearable Applications

Currently, with the development of electronic skins (e-skins), wearable pressure sensors with low energy consumption and excellent wearability for long-term physiological signal monitoring are urgently desired but remain a challenge. Capacitive-type devices are desirable candidates for wearable applications, but traditional capacitive pressure sensors are limited by low capacitance and sensitivity. In this study, an all-nanofibrous ionic pressure sensor (IPS) is developed, and the formation of an electrical double layer at the electrode/electrolyte contact interface significantly enhances the capacitance and sensing properties. The IPS is fabricated by sandwiching a nanofibrous ionic gel sensing layer between two thermoplastic polyurethane nanofibrous membranes with graphene electrodes. The IPS has a high sensitivity of 217.5 kPa–1 in the pressure range of 0–5 kPa, which is much higher than that of conventional capacitive pressure sensors. Combined with the rapid response and recovery speed (30 and 60 ms), the IPS is suitable for real-time monitoring of multiple physiological signals. Moreover, the nanofiber network endows the IPS with excellent air permeability and heat dissipation, which guarantees comfort during long-term wearing. This work provides a viable strategy to improve the wearability of wearable sensors, which can promote healthcare and human–machine interaction applications.