journal article·2025-08-11

Ultrafast Laser Texturing of Ceramic Electrolytes toward Solid-State Battery Application

Shuo Yan, Deliang Guo, Elena A. Baranova, Ali Merati, Chae-Ho Yim, Yaser Abu-Lebdeh, Arnaud Weck

ACS Applied Energy Materials· Volume 8· Issue 15
Publisher page

Abstract

Solid-state batteries are expected to complement liquid-based lithium-ion batteries (LIBs) with improved safety and energy density. However, point-to-point interface contact between oxide-based ceramic solid-state electrolytes (SSEs) and electrodes impedes Li-ion transfer and degrades the battery performance. Herein, micropatterns with controllable geometries were created onto perovskite-type SSE surfaces via femtosecond ultrafast laser processing. Laser-textured SSEs with two-directional (2D) perpendicular grooves can achieve a significant reduction in interfacial resistance (<1 versus 3416.81 Ω cm –2 for bare sample) attributed to increased contact area and trapping of the liquid electrolyte. This work serves as a proof-of-concept for applying ultrafast laser processing toward solid-state battery applications.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Supercapacitor Materials and Fabrication · Advanced Battery Materials and Technologies · Silicone and Siloxane Chemistry

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Chemical and Biological Engineering, Center for Catalysis Research and Innovation (CCRI), Nexus for Quantum Technologies (NexQT)

University of Ottawa

Department of Mechanical Engineering, Center of Research in Photonics, Nexus for Quantum Technologies (NexQT)

Aerospace Research Center, National Research Council of Canada, 1200 Montreal Road, Ottawa, Ontario K1A 0R6, Canada

Clean Energy Innovation Research Center, National Research Council of Canada, 1200 Montreal Road, Ottawa, Ontario K1A 0R6, Canada

Funding

National Research Council Canada · Office of Energy Research and Development · Natural Sciences and Engineering Research Council of Canada

References (52)

Show source-provided references
1. 10.1016/j.energy.2020.11802510.1016/j.energy.2020.118025 ↗
2. 10.1016/j.rser.2022.11207710.1016/j.rser.2022.112077 ↗
3. 10.1016/j.est.2023.10715910.1016/j.est.2023.107159 ↗
4. 10.1007/s41918-018-0022-z10.1007/s41918-018-0022-z ↗
5. 10.1021/acsenergylett.0c0258410.1021/acsenergylett.0c02584 ↗
6. 10.1002/eem2.1245010.1002/eem2.12450 ↗
7. 10.1002/aenm.20190016110.1002/aenm.201900161 ↗
8. 10.1002/adma.20180056110.1002/adma.201800561 ↗
9. 10.1021/acsenergylett.1c0044510.1021/acsenergylett.1c00445 ↗
10. 10.1021/acsenergylett.2c0000310.1021/acsenergylett.2c00003 ↗
11. 10.1038/s41578-019-0165-510.1038/s41578-019-0165-5 ↗
12. 10.1038/s41586-023-05970-410.1038/s41586-023-05970-4 ↗
13. 10.1021/acs.chemrev.0c0010110.1021/acs.chemrev.0c00101 ↗
14. 10.1038/s41560-020-00759-510.1038/s41560-020-00759-5 ↗
15. 10.1038/s41563-019-0431-310.1038/s41563-019-0431-3 ↗
16. 10.3390/batteries704007510.3390/batteries7040075 ↗
17. 10.1002/adma.20220640210.1002/adma.202206402 ↗
18. 10.1021/acs.chemrev.9b0026810.1021/acs.chemrev.9b00268 ↗
19. 10.1021/acs.accounts.7b0046010.1021/acs.accounts.7b00460 ↗
20. 10.1016/j.ensm.2021.01.00210.1016/j.ensm.2021.01.002 ↗
21. 10.1039/D0EE01435D10.1039/D0EE01435D ↗
22. 10.1016/j.ensm.2023.03.00810.1016/j.ensm.2023.03.008 ↗
23. 10.1007/s11581-022-04870-310.1007/s11581-022-04870-3 ↗
24. 10.1126/sciadv.160165910.1126/sciadv.1601659 ↗
25. 10.1038/s41563-023-01627-910.1038/s41563-023-01627-9 ↗
26. 10.1021/acsami.9b1178010.1021/acsami.9b11780 ↗
27. 10.1021/acsami.3c0358310.1021/acsami.3c03583 ↗
28. 10.1016/j.ensm.2024.10341810.1016/j.ensm.2024.103418 ↗
29. 10.1039/D3TA01435E10.1039/D3TA01435E ↗
30. 10.1002/adma.20170713210.1002/adma.201707132 ↗
31. 10.1016/j.jpowsour.2011.07.00510.1016/j.jpowsour.2011.07.005 ↗
32. 10.1016/j.jpowsour.2010.11.13910.1016/j.jpowsour.2010.11.139 ↗
33. 10.1149/1.330845910.1149/1.3308459 ↗
34. 10.1021/acsmaterialslett.9b0018910.1021/acsmaterialslett.9b00189 ↗
35. 10.1016/j.jmapro.2023.09.07210.1016/j.jmapro.2023.09.072 ↗
36. 10.1016/j.matchemphys.2022.12626510.1016/j.matchemphys.2022.126265 ↗
37. 10.2351/7.000127410.2351/7.0001274 ↗
38. 10.1039/D1TA02991F10.1039/D1TA02991F ↗
39. 10.1002/adma.20210400910.1002/adma.202104009 ↗
40. 10.1021/acsenergylett.3c0104210.1021/acsenergylett.3c01042 ↗
41. 10.1002/smll.20150012710.1002/smll.201500127 ↗
42. 10.1002/sstr.20210001410.1002/sstr.202100014 ↗
43. 10.1016/j.jmapro.2024.11.05610.1016/j.jmapro.2024.11.056 ↗
44. 10.1016/j.jmatprotec.2023.11800110.1016/j.jmatprotec.2023.118001 ↗
45. 10.1016/j.jmatprotec.2019.03.03410.1016/j.jmatprotec.2019.03.034 ↗
46. 10.1016/j.ijhydene.2016.12.11210.1016/j.ijhydene.2016.12.112 ↗
47. 10.3390/cryst1307101610.3390/cryst13071016 ↗
48. 10.1021/acsami.3c0935810.1021/acsami.3c09358 ↗
49. 10.1002/admi.20130014310.1002/admi.201300143 ↗
50. 10.1002/adfm.20190914010.1002/adfm.201909140 ↗
51. 10.3389/fchem.2022.96627410.3389/fchem.2022.966274 ↗
52. 10.1038/nchem.247010.1038/nchem.2470 ↗