DataVXACS Applied Energy MaterialsPaper
journal article·2024-12-23

Highly Efficient Blade-Coated 1.67 eV p-i-n Perovskite Solar Cells Enabled by a Hybrid Self-Assembled Monolayer and Surface Passivation

Zixuan Huang, Xin Ge, Zhen Liu, Biao Shi, Pengyang Wang, Ying Zhao, Xiaodan Zhang

ACS Applied Energy Materials· Volume 7· Issue 24
Publisher page
Source abstract

Abstract

Wide-band-gap perovskite solar cells (PSCs) are considered an important part of multijunction tandem solar cells and have attracted extensive research in related fields. For blade-coated inverted wide-band-gap PSCs, nonradiative recombination losses in the perovskite/charge transport layer interface are serious. The performance of blade-coated wide-band-gap perovskite solar cells has hindered the industrialization of tandem solar cells, especially for two-terminal perovskite/silicon tandem solar cells (TSCs). To reduce these losses as much as possible, the choice of hole transport layers and perovskite films post-treatment is extremely important. Herein, we used two strategies: a hybrid self-assembled monolayer as the hole transport layer and surface passivation post-treatment to obtain highly efficient and stable PSCs by the blade-coating method. The champion device demonstrated an efficiency of 21.30% for p-i-n PSCs, which is one of the highest efficiencies for band gaps above 1.67 eV among all of the scalable preparation methods employed.
Source: openalex_inverted_index · Quality: baseline

Research context

Electronic materials

OpenAlex topics: Perovskite Materials and Applications · Conducting polymers and applications · Chalcogenide Semiconductor Thin Films

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Institute of Photoelectronic Thin Film Devices and Technology, Renewable Energy Conversion and Storage Center, Solar Energy Research Center, Nankai University, Tianjin 300350, P. R. China

Key Laboratory of Photoelectronic Thin Film Devices and Technology of Tianjin, Tianjin 300350, P. R. China

Haihe Laboratory of Sustainable Chemical Transformations, Tianjin 300192, P. R. China

Engineering Research Center of Thin Film Photoelectronic Technology of Ministry of Education, Tianjin 300350, P. R. China

Collaborative Innovation Center of Chemical Science and Engineering (Tianjin), Tianjin 300072, P. R. China

Funding

Nankai University · National Key Research and Development Program of China · Major Science and Technology Projects in Yunnan Province · Hebei Provincial Key Research Projects · National Natural Science Foundation of China · Overseas Expertise Introduction Project for Discipline Innovation · Haihe Laboratory of Sustainable Chemical Transformations, Nankai University

References (33)

Show source-provided references
1. 10.1002/adma.20210654010.1002/adma.202106540 ↗
2. 10.1002/aenm.20220240410.1002/aenm.202202404 ↗
3. 10.1016/j.esci.2022.04.00110.1016/j.esci.2022.04.001 ↗
4. https://www.longi.com/cn/news/2024-snec-silicon-perovskite-tandem-solar-cells-new-world-efficiency/.
5. 10.1002/aesr.20200004610.1002/aesr.202000046 ↗
6. 10.1002/pip.369610.1002/pip.3696 ↗
7. 10.1002/adfm.20200862110.1002/adfm.202008621 ↗
8. 10.1039/C5MH00126A10.1039/C5MH00126A ↗
9. 10.1021/acsenergylett.7b0122110.1021/acsenergylett.7b01221 ↗
10. 10.1002/aenm.20220097510.1002/aenm.202200975 ↗
11. 10.1002/aenm.20230059510.1002/aenm.202300595 ↗
12. 10.1002/anie.20230026510.1002/anie.202300265 ↗
13. 10.1002/advs.20220030810.1002/advs.202200308 ↗
14. 10.1038/s41566-022-01033-810.1038/s41566-022-01033-8 ↗
15. 10.1038/s41467-023-36141-810.1038/s41467-023-36141-8 ↗
16. 10.1002/aenm.20200298910.1002/aenm.202002989 ↗
17. 10.1002/adma.20230441510.1002/adma.202304415 ↗
18. 10.1002/adfm.20230470810.1002/adfm.202304708 ↗
19. 10.1021/acsami.0c1810810.1021/acsami.0c18108 ↗
20. 10.1002/ange.20230739510.1002/ange.202307395 ↗
21. 10.1016/j.jechem.2024.01.06310.1016/j.jechem.2024.01.063 ↗
22. 10.1021/jacs.2c1330710.1021/jacs.2c13307 ↗
23. 10.1126/science.aap928210.1126/science.aap9282 ↗
24. 10.1002/aenm.20170339210.1002/aenm.201703392 ↗
25. 10.1063/1.496612710.1063/1.4966127 ↗
26. 10.1021/acsenergylett.9b0272010.1021/acsenergylett.9b02720 ↗
27. 10.1021/acsenergylett.0c0259910.1021/acsenergylett.0c02599 ↗
28. 10.1126/science.abn769610.1126/science.abn7696 ↗
29. 10.1021/acsenergylett.0c0129710.1021/acsenergylett.0c01297 ↗
30. 10.1021/acsenergylett.2c0150610.1021/acsenergylett.2c01506 ↗
31. 10.1002/adma.20220788310.1002/adma.202207883 ↗
32. 10.1021/acsaem.8b0032810.1021/acsaem.8b00328 ↗
33. 10.1021/acsami.1c0440710.1021/acsami.1c04407 ↗