journal article·2019-02-25

Lithium-Chemical Synthesis of Highly Conductive 3D Mesoporous Graphene for Highly Efficient New Generation Solar Cells

Wei Wei, Dario Stacchiola, Nusnin Akter, J. Anibal Boscoboinik, Yun Hang Hu

ACS Applied Energy Materials· Volume 2· Issue 2
Publisher page

Abstract

In this study, a highly conductive three-dimensional mesoporous graphene (3DMG), which was synthesized by our discovered reaction of lithium (Li) liquid and CO gas, was demonstrated as a promising electrode material for the hole transport material (HTM) free perovskite solar cell (PSC) and the dye-sensitized solar cell (DSSC), achieving high energy conversion efficiencies of 8.60% and 9.19%, respectively. The DSSC efficiency is higher than that (7.96%) of a DSSC with a standard Pt counter electrode. Furthermore, it was found that the electrical conductivity of 3DMG played a critical role in the PSC, but the DSSC performance was dependent on both its surface area and electrical conductivity. This would provide a novel approach to synthesize ideal electrode materials for energy devices.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Perovskite Materials and Applications · Advanced Photocatalysis Techniques · Conducting polymers and applications

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Materials Science and Engineering, Michigan Technological University, 1400 Townsend Dr., Houghton, Michigan 49931, United States

Center for Functional Nanomaterials, Brookhaven National Laboratory, Upton, New York 11973, United States

Department of Materials Science and Chemical Engineering, Stony Book University, Stony Brook, New York 11790, United States

Funding

Division of Civil, Mechanical and Manufacturing Innovation · Division of Chemical, Bioengineering, Environmental, and Transport Systems

References (51)

Show source-provided references
1. 10.1002/adma.20100106810.1002/adma.201001068 ↗
2. 10.1126/science.110289610.1126/science.1102896 ↗
3. 10.1038/nmat184910.1038/nmat1849 ↗
4. 10.1039/C5TA00252D10.1039/C5TA00252D ↗
5. 10.1021/nn100636810.1021/nn1006368 ↗
6. 10.1038/nature0771910.1038/nature07719 ↗
7. 10.1016/j.synthmet.2015.07.00510.1016/j.synthmet.2015.07.005 ↗
8. 10.1038/nnano.2008.36510.1038/nnano.2008.365 ↗
9. 10.1016/S1369-7021(09)70274-310.1016/S1369-7021(09)70274-3 ↗
10. 10.1039/C2CS35353A10.1039/C2CS35353A ↗
11. 10.1039/c3nr33700f10.1039/c3nr33700f ↗
12. 10.1002/adma.20150476010.1002/adma.201504760 ↗
13. 10.1021/acs.nanolett.6b0474210.1021/acs.nanolett.6b04742 ↗
14. 10.1039/C7TA01768E10.1039/C7TA01768E ↗
15. 10.1039/C4TA03909B10.1039/C4TA03909B ↗
16. 10.1039/C6TA04008J10.1039/C6TA04008J ↗
17. 10.1021/acs.iecr.6b0476810.1021/acs.iecr.6b04768 ↗
18. 10.1002/er.331210.1002/er.3312 ↗
19. 10.1021/acsami.8b0966110.1021/acsami.8b09661 ↗
20. 10.1038/353737a010.1038/353737a0 ↗
21. 10.1021/cr900356p10.1021/cr900356p ↗
22. 10.1038/nchem.186110.1038/nchem.1861 ↗
23. 10.1002/anie.20180133710.1002/anie.201801337 ↗
24. 10.1016/j.nanoen.2018.09.07010.1016/j.nanoen.2018.09.070 ↗
25. 10.1021/acsami.5b1109710.1021/acsami.5b11097 ↗
26. 10.1021/nn302944b10.1021/nn302944b ↗
27. 10.1021/ph500219r10.1021/ph500219r ↗
28. 10.1016/j.nanoen.2014.10.03310.1016/j.nanoen.2014.10.033 ↗
29. 10.1016/j.jcat.2016.11.03310.1016/j.jcat.2016.11.033 ↗
30. 10.1016/j.nanoen.2016.03.00310.1016/j.nanoen.2016.03.003 ↗
31. 10.1039/C6NR00401F10.1039/C6NR00401F ↗
32. 10.1039/C5NR06715D10.1039/C5NR06715D ↗
33. 10.1021/am508441810.1021/am5084418 ↗
34. 10.1002/er.317810.1002/er.3178 ↗
35. 10.1016/j.nanoen.2016.02.01010.1016/j.nanoen.2016.02.010 ↗
36. 10.1039/C5TA02946E10.1039/C5TA02946E ↗
37. 10.1039/9781782626855-0026810.1039/9781782626855-00268 ↗
38. 10.1039/C6TA04743B10.1039/C6TA04743B ↗
39. 10.1039/c3ta13002a10.1039/c3ta13002a ↗
40. 10.1039/c3ta10892a10.1039/c3ta10892a ↗
41. 10.1007/s11244-013-0218-810.1007/s11244-013-0218-8 ↗
42. 10.1002/anie.20140698210.1002/anie.201406982 ↗
43. 10.1002/anie.20140038810.1002/anie.201400388 ↗
44. 10.1002/adma.20150604910.1002/adma.201506049 ↗
45. 10.1038/nature1413310.1038/nature14133 ↗
46. 10.1126/science.aaa927210.1126/science.aaa9272 ↗
47. 10.1016/j.nanoen.2018.07.02810.1016/j.nanoen.2018.07.028 ↗
48. 10.1088/1361-6463/aa7cb010.1088/1361-6463/aa7cb0 ↗
49. 10.1126/science.125476310.1126/science.1254763 ↗
50. 10.1016/j.nanoen.2016.06.04710.1016/j.nanoen.2016.06.047 ↗
51. 10.1002/aenm.20150208710.1002/aenm.201502087 ↗