journal article·2026-06-11Open access

High Thermal Conductivity Transfer-Printed Polycrystalline Diamond Membranes for Device- and Chip-Level Thermal Management

Husam Walwil, Chenyu Wang, Seokjun Kim, Xuanyu Zhou, Luke Suter, Matthias Muehle, Tae Kyoung Kim, Minji Kim, Jiun Oh, Joon Seop Kwak, Jung-Hun Seo, Sukwon Choi

Abstract

High Resolution Image Download MS PowerPoint Slide The thermal conductivity of polycrystalline diamond (PCD) thin films can vary by more than an order of magnitude due to differences in the microstructure. PCD films often undergo columnar growth where the grain size increases with the film thickness. Therefore, phonon-grain boundary scattering significantly impacts the thermal conductivity and interfacial thermal transport. In this work, to utilize PCD membranes (PCDm) as transfer-printed heat spreaders for high-power electronic devices and chiplets, a fabrication process was developed where the defective and low thermal conductivity nucleation region of the PCD film is removed to form a high-thermal-conductivity membrane. The temperature-dependent anisotropic thermal conductivity of a ∼2.4 μm-thick PCDm (with the nucleation region removed) and the thermal boundary conductance (TBC) across the PCDm/Si interface were characterized via time-domain thermoreflectance (TDTR). The measured out-of-plane ( κ out = 304 ± 82 W m −1 K −1 ) and in-plane thermal conductivities ( κ in = 136 ± 31 W m −1 K −1 ) of the nucleation region-free membrane are significantly higher than those ( κ out = 187 ± 41 and κ in = 103 ± 17 W m −1 K −1 ) for an as-grown ∼3.3 μm-thick PCDm that includes the nucleation region. The measured interfacial TBC at the PCDm/Si interface was determined to be 5.8 MW m -2 K −1, which is lower than typical values for PCD films directly grown on Si. Thermal modeling of a single-finger GaN high electron mobility transistor (HEMT) shows that a top-side integrated PCDm reduces the channel peak temperature by ∼10%. Simulation results suggest that the high-thermal-conductivity PCDm can serve as effective means for the cooling of high-power electronic devices and 3D-integrated circuits if the TBC is improved via optimization of the transfer-printing process.
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Research context

OpenAlex topics: Thermal properties of materials · Diamond and Carbon-based Materials Research · Carbon Nanotubes in Composites

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Mechanical Engineering

The Pennsylvania State University

Department of Materials Design and Innovation

University at Buffalo, The State University of New York

Fraunhofer USA Inc., Center Midwest

R&D center, Wavelord Inc

Department of Energy Engineering, Korea Institute of Energy Technology, 21, Kentech-gil, Naju-si, Jeollanam-do 58330, Republic of Korea

Funding

Army Research Office · Ministry of Trade, Industry and Energy · Fraunhofer Program Affiliate Cooperation for Knowledge Transfer (PACT) program · National Science Foundation (NSF)

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