journal article·2025-11-11

Impact of the Seed Layer on the Domain Switching and Electrical Properties of PbZr 0.52 Ti 0.48 O 3 Thin Films

Jinpeng Liu, Wenlong Lu, Junya Wang, Junsheng Yang, Huabin Yang, Hua Tan, Haibo Zhang

ACS Applied Electronic Materials· Volume 7· Issue 21
Publisher page

Abstract

Lead zirconate titanate (PZT) thin films are an important component for piezoelectric microelectromechanical systems (piezo-MEMS) and ferroelectric device applications. Three different seed layers, PbTiO 3 (PT), PbZrO 3 (PZ), and Pb 0.8 La 0.1 Ca 0.1 Ti 0.975 O 3 (PLCT), were applied to deposit PbZr 0.52 Ti 0.48 O 3 (PZT) films via the sol–gel method on Pt(111)/TiO 2 /SiO 2 /Si substrates. All films exhibited well-polycrystalline orientation. To demonstrate the differences of these films in device applications, the crystalline structure, surface morphology, piezoelectric, dielectric, and ferroelectric properties of these films were characterized. The results indicate reduced grain sizes in these films compared to pure PZT films. Under the action of the seed layers, the piezoelectric coefficients and domain switching behavior of these films were significantly improved. Furthermore, the PZT/PZ film exhibited an ultralow leakage current density (<10 –4 A/cm 2 ) and a loss tangent (<0.05) at ±350 kV/cm.
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Research context

OpenAlex topics: Ferroelectric and Piezoelectric Materials · Microwave Dielectric Ceramics Synthesis · Electronic and Structural Properties of Oxides

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

School of Mechanical Science & Engineering

Huazhong University of Science and Technology

School of Materials Science and Engineering, State Key Laboratory of Material Processing and Die & Mould Technology

Guangdong HUST Industrial Technology Research Institute

Guangdong Provincial Key Laboratory of Manufacturing Equipment Digitization

College of Mechanical Engineering

Wuhan Polytechnic University

School of Material Science and Engineering

Guilin University of Electronic Technology

Faculty of Chemical Engineering

Industrial University of Ho Chi Minh City

Huangpu Institute of Materials

Funding

Science and Technology Planning Project of Guangdong Province · Basic and Applied Basic Research Foundation of Guangdong Province · National Natural Science Foundation of China · Dongguan Key Research &Development Program, China · Innovation Project of Optics Valley Laboratory

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