journal article·2023-07Open access

Sensitivity estimation of indium oxide thin film for gamma sensing

C. Aparna, Pramoda Kumara Shetty, M. G. Mahesha, I. Yashodhara, N. Karunakara

Journal of Materials Science· Volume 58· Issue 27

Abstract

Abstract This article aims to study the modification in the structural, optical and electrical properties of indium oxide thin film after gamma irradiation and estimation of sensitivity for gamma sensing applications. The thin film of indium oxide was deposited on a 450 °C preheated glass substrate using the spray pyrolysis technique. The deposited thin film of molar concentration 0.15 M and thickness of around 600 nm was irradiated with different gamma doses (100 Gy, 200 Gy, 300 Gy and 400 Gy). The optical properties of the irradiated film are studied using UV–Visible spectroscopy. Transmittance increased after irradiation up to 200 Gy and beyond that, it decreased. Indium oxide is an n-type semiconductor which exhibits both direct and indirect transitions. Both direct and indirect bandgap energy are calculated using Tauc’s plot. Extinction coefficient and refractive index variation with irradiation were also estimated. Photoluminescence study confirmed the gamma-induced defect formation and annihilation for an irradiation dose of 400 Gy and 200 Gy, respectively. Resistivity also decreased up to 200 Gy and beyond that, it increased. The sensitivity of the deposited film was estimated from the electrical measurements, and it lies between 10.7 and 53.4 mA/cm2/Gy. Graphical abstract
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Research context

OpenAlex topics: ZnO doping and properties · Semiconductor materials and devices · Ga2O3 and related materials

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References (48)

Show source-provided references
1. Baydogan N, Ozdemir O, Cimenoglu H (2013) The improvement in the electrical properties of nanospherical ZnO:Al thin film exposed to irradiation using a Co-60 radioisotope. Radiat Phys Chem 89:20–2710.1016/j.radphyschem.2013.02.042 ↗
2. Sudha A, Sharma SL, Gupta AN (2019) Achieving sensitive and stable indium oxide thin films for gamma radiation monitoring. Sens Actuators A Phys 285:378–38510.1016/j.sna.2018.10.015 ↗
3. Yahia A, Attaf A, Saidi H, Dahnoun M, Khelifi C, Bouhdjer A, Saadi A, Ezzaouia H (2019) Structural, optical, morphological and electrical properties of indium oxide thin films prepared by sol gel spin coating process. Surf Interfaces 14:158–16510.1016/j.surfin.2018.12.012 ↗
4. Nefzi C, Souli M, Beji N, Mejri A, Kamoun-Turki N (2017) Enhancement by high gamma radiations of optical and electrical properties of indium oxide thin films for solar devices. J Mater Sci 52:336–34510.1007/s10853-016-0334-5 ↗
5. Narmada A, Kathirvel P, Lakshmi M, Saravanakumar S, Marnadu R, Chandrasekaran J (2020) Jet nebuliser spray pyrolysed indium oxide and nickel doped indium oxide thin films for photodiode application. Optik (Stuttg) 202:163701
6. Jung DS, Bin Park S, Kang YC (2010) Design of particles by spray pyrolysis and recent progress in its application. Korean J Chem Eng 27:1621–164510.1007/s11814-010-0402-5 ↗
7. Kaya S, Yıldız I, Lok R, Yılmaz E (2018) Co-60 gamma irradiation influences on physical, chemical and electrical characteristics of HfO2/Si thin films. Radiat Phys Chem 150:64–7010.1016/j.radphyschem.2018.04.023 ↗
8. Aparna C, Shetty PK, Mahesha MG (2022) Structural optimization of indium oxide thin film for gamma dosimetry applications. Mater Sci Semicond Process 150:106931
9. Sudha A, Sharma SL, Sharma SD (2017) Study of structural, optical and electrical properties of gamma irradiated In2O3 thin films for device applications. J Mater Sci Mater Electron 28:4619–462410.1007/s10854-016-6100-2 ↗
10. Sudha A, Maity TK, Sharma SL (2016) Effects of gamma irradiations on structural and electrical properties of indium oxide thin films prepared by thermal evaporation. Mater Lett 164:372–37510.1016/j.matlet.2015.11.003 ↗
11. Kaya S, Yilmaz E (2018) Modifications of structural, chemical, and electrical characteristics of Er2O3/Si interface under Co-60 gamma irradiation. Nucl Instrum Methods Phys Res Sect B Beam Interact with Mater Atoms 418:74–7910.1016/j.nimb.2018.01.010 ↗
12. Nefzi C, Beji N, Souli M, Mejri A, Alleg S, Kamoun-Turki N (2019) Effect of gamma-irradiation on optical, structural and electrical properties of In2O3: F thin films for photocatalysis application. Opt Laser Technol 112:85–9210.1016/j.optlastec.2018.11.010 ↗
13. Dey PC, Sarkar S, Das R (2020) X-ray diffraction study of the elastic properties of jagged spherical CdS nanocrystals. Mater Sci Pol 38:271–27810.2478/msp-2020-0032 ↗
14. Gurer U, Yilmaz O, Karacali H, Kaya S, Yilmaz E (2020) Co-60 gamma radiation influences on the electrochemical, physical and electrical characteristics rare-earth dysprosium oxide (Dy2O3). Radiat Phys Chem 171:10868410.1016/j.radphyschem.2020.108684 ↗
15. Souli M, Reghima M, Secu M, Bartha C, Enculescu M, Mejri A, Kamoun-Turki N, Badica P (2019) Physical properties investigation of samarium doped calcium sulfate thin films under high gamma irradiations for space photovoltaic and dosimetric applications. Superlattices Microstruct 126:103–11910.1016/j.spmi.2018.12.021 ↗
16. Nefzi C, Souli M, Beji N, Mejri A, Kamoun-Turki N (2019) Improvement of structural, optical and electrical properties of iron doped indium oxide thin films by high gamma radiations for photocatalysis applications. Mater Sci Semicond Process 90:32–4010.1016/j.mssp.2018.09.022 ↗
17. Arshak K, Korostynska O (2006) Response of metal oxide thin film structures to radiation. Mater Sci Eng B Solid-State Mater Adv Technol 133:1–710.1016/j.mseb.2006.06.012 ↗
18. Arshak K, Korostynska O, Henry J (2005) Structural modifications in thin films caused by gamma radiation. Mater Sci Forum 480–481:13–2010.4028/www.scientific.net/MSF.480-481.13 ↗
19. Abhirami KM, Sathyamoorthy R, Asokan K (2013) Structural, optical and electrical properties of gamma irradiated SnO thin films. Radiat Phys Chem 91:35–3910.1016/j.radphyschem.2013.05.030 ↗
20. Beji N, Souli M, Azzaza S, Alleg S, Kamoun Turki N (2016) Study on the zinc doping and annealing effects of sprayed In2O3 thin films. J Mater Sci Mater Electron 5:4849–486010.1007/s10854-016-4367-y ↗
21. Saeed F, Farooq A, Ali A, Mehmood S, Cepek C, Bhardwaj S, Ul-Hamid A, Bhatti AS (2020) Anomalous optical behavior in pyramid-like indium oxide (In2O3) nanostructures. Mater Sci Eng B Solid-State Mater Adv Technol 262:11478110.1016/j.mseb.2020.114781 ↗
22. Dasari SG, Nagaraju P, Yelsani V, Tirumala S, Ramana Reddy MV (2021) Nanostructured indium oxide thin films as a room temperature toluene sensor. ACS Omega 6:17442–1745410.1021/acsomega.1c01831 ↗
23. Hazem R, Izerrouken M, Cheraitia A, Djehlane A (2019) Raman study of ion beam irradiation damage on nanostructured TiO 2 thin film. Nucl Instru Methods Phys Res Sect B Beam Interact with Mater Atoms 444:62–6710.1016/j.nimb.2019.02.011 ↗
24. Choudhary R, Chauhan RP (2016) Gamma irradiation induced modifications in spin coated CdSe thin films. J Mater Sci Mater Electron 27:11674–1168110.1007/s10854-016-5303-x ↗
25. Ramaiah KS, Raja VS, Bhatnagar AK, Juang FS, Chang SJ, Su YK (2000) Effect of annealing and γ-irradiation on the properties of CuInSe2 thin films. Mater Lett 45:251–26110.1016/S0167-577X(00)00114-2 ↗
26. Sarker P, Sen SK, Mia MNH et al (2021) Effect of gamma irradiation on structural, morphological and optical properties of thermal spray pyrolysis deposited CuO thin film. Ceram Int 47:3626–363310.1016/j.ceramint.2020.09.211 ↗
27. Tripathi N, Rath S (2014) Effect of thermal annealing and swift heavy ion irradiation on the optical properties of indium oxide thin films. ECS J Solid State Sci Technol 3:P21–P2510.1149/2.002403jss ↗
28. Beena D, Lethy KJ, Vinodkumar R, Pillai VPM, Ganesan V, Phase DM, Sudheer SK (2009) Effect of substrate temperature on structural, optical and electrical properties of pulsed laser ablated nanostructured indium oxide films. Appl Surf Sci 255:8334–834210.1016/j.apsusc.2009.05.057 ↗
29. Dewan N, Sreenivas K, Gupta V (2008) Comparative study on TeO2 and TeO3 thin film for γ-ray sensor application. Sens Actuators A Phys 147:115–12010.1016/j.sna.2008.04.011 ↗
30. Girtan M, Folcher G (2003) Structural and optical properties of indium oxide thin films prepared by an ultrasonic spray CVD process. Surf Coat Technol 172:242–25010.1016/S0257-8972(03)00334-7 ↗
31. Arshak K, Korostynska O (2002) Gamma radiation dosimetry using Tellurium dioxide thin film structures. Sensors 2:347–35510.3390/s20800347 ↗
32. Hadia NMA, Mohamed HA (2013) Synthesis, structure and optical properties of single-crystalline In 2O3 nanowires. J Alloys Compd 547:63–6710.1016/j.jallcom.2012.08.116 ↗
33. Maity TK, Sharma SL (2008) Effect of gamma radiation on optical and electrical properties of tellurium dioxide thin films. Bull Mater Sci 31:841–84610.1007/s12034-008-0134-x ↗
34. Erhart P, Klein A, Egdell RG, Albe K (2007) Band structure of indium oxide: indirect versus direct band gap. Phys Rev B Condens Matter Mater 75:15320510.1103/PhysRevB.75.153205 ↗
35. Arshak K, Korostynska O (2004) Preliminary studies of properties of oxide thin/thick films for gamma radiation dosimetry. Mater Sci Eng B Solid-State Mater Adv Technol 107:224–23210.1016/j.mseb.2003.11.014 ↗
36. El-Nahass MM, Darwish AAA, El-Zaidia EFM, Bekheet AE (2013) Gamma irradiation effect on the structural and optical properties of nanostructured InSe thin films. J Non Cryst Solids 382:74–7810.1016/j.jnoncrysol.2013.10.012 ↗
37. Waikar MR, Raste PM, Sonker RK, Gupta V, Tomar M, Shirsat MD, Sonkawade RG (2020) Enhancement in NH3 sensing performance of ZnO thin-film via gamma-irradiation. J Alloys Compd 830:15464110.1016/j.jallcom.2020.154641 ↗
38. Göde F, Güneri E, Emen FM, Emir Kafadar V, Ünlü S (2014) Synthesis, structural, optical, electrical and thermoluminescence properties of chemically deposited PbS thin films. J Lumin 147:41–4810.1016/j.jlumin.2013.10.050 ↗
39. Prathap P, Subbaiah YPV, Devika M, Reddy KTR (2006) Optical properties of In2O3 films prepared by spray pyrolysis. Mater chem phys 100:375–37910.1016/j.matchemphys.2006.01.016 ↗
40. Abu EL-Fadl A, Hafiz MM, Wakaad MM, Aashour AS (2007) Influence of γ-radiation on the optical parameters of Ag10Te90 thin films. Radiat Phys Chem 76:61–6610.1016/j.radphyschem.2006.08.007 ↗
41. Craciun D, Socol G, Caër SL, Trinca LM, Galca AC, Pantelica D, Ionescu P, Craciun V (2016) Gamma irradiation effects on the properties of indium zinc oxide thin films. Thin Solid Films 614:2–610.1016/j.tsf.2016.04.041 ↗
42. Salim SR (2014) The Effect of irradiation on structural and optical characteristics of indium oxide thin films. Int J Sci Res 3:2004–2014
43. Aparna C, Kumara P, Mahesha MG, Karunakara N, Yashodhara I (2022) Structural, optical and sensitivity study of optimized indium oxide thin film for gamma sensing applications. Sens Actuators A Phys 345:11378510.1016/j.sna.2022.113785 ↗
44. Arshak K, Korostynska O, Henry J (2004) Thick film PN-junctions based on mixed oxides of indium and silicon as gamma radiation sensors. Microelectron Int 21:19–2710.1108/13565360410517085 ↗
45. Horowitz Y, Olko P (2004) The effects of ionisation density on the thermoluminescence response (efficiency) of LiF:Mg, Ti and LiF:Mg, Cu. P Radiat Prot Dosim 109:331–34810.1093/rpd/nch310 ↗
46. Maity TK, Sharma SL (2011) Effects of gamma irradiation on electrical, optical and structural properties of tellurium dioxide thin films. Indian J Pure Appl Phys 49:606–612
47. Aparna C, Shetty PK, Mahesha MG, Karunakara N (2022) Temperature dependence of optical and electrical properties of gamma-irradiated indium oxide thin film. Optik (Stuttg) 269:169881
48. Arshak K, Corcoran J, Korostynska O (2005) Gamma radiation sensing properties of TiO2, ZnO, CuO and CdO thick film pn-junctions. Sensors Actuators A Phys 123–124:194–19810.1016/j.sna.2005.01.014 ↗