journal article·2024-05-28

Epitaxial Rare-Earth-Doped Complex Oxide Thin Films for Infrared Applications

Mythili Surendran, Joshua R. Rollag, Christopher E. Stevens, Ching-Tai Fu, Harish Kumarasubramanian, Zhe Wang, Darrell G. Schlom, Ricky Gibson, Joshua R. Hendrickson, Jayakanth Ravichandran

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Abstract

Rare-earth dopants are one of the most extensively studied optical emission centers for a broad range of applications such as laser optoelectronics, sensing, lighting, and quantum information technologies due to their narrow optical line width and exceptional coherence properties. Epitaxial doped oxide thin films can serve as a promising and controlled host to investigate rare-earth dopants suitable for scalable quantum memories, on-chip lasers, and amplifiers. Here, we report high-quality epitaxial thin films of Tm-doped CaZrO 3 grown by pulsed laser deposition for infrared optoelectronic and quantum memory applications. We perform extensive structural and chemical characterization to probe the crystallinity of the films and the doping behavior. Low-temperature photoluminescence measurements show sharp radiative transitions in the short-wave infrared range of 1.75–2 μm.
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Research context

OpenAlex topics: Luminescence Properties of Advanced Materials · Transition Metal Oxide Nanomaterials · Solid State Laser Technologies

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Affiliations

Mork Family Department of Chemical Engineering and Materials Science, University of Southern California, 925 Bloom Walk, Los Angeles, California 90089, United States

Core Center of Excellence in Nano Imaging, University of Southern California, 1002 West Childs Way, MCB Building, Los Angeles, California 90089, United States

KBR Inc., 3725 Pentagon Blvd, Suite 210, Beavercreek, Ohio 45431, United States

Air Force Research Laboratory, Sensors Directorate, Wright-Patterson Air Force Base, 2241 Avionics Circle, Ohio 45433, United States

Ming Hsieh Department of Electrical and Computer Engineering, University of Southern California, 925 Bloom Walk, Los Angeles, California 90089, United States

Department of Materials Science and Engineering, Cornell University, Ithaca, New York 14853, United States

Kavli Institute at Cornell for Nanoscale Science, Ithaca, New York 14853, United States

Funding

Air Force Office of Scientific Research

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