journal article·2021-01-26

Facile and Scalable Electrospun Nanofiber-Based Alternative Current Electroluminescence (ACEL) Device

Wanasinghe Arachchige Dumith Madushanka Jayathilaka, Amutha Chinnappan, Dongxiao Ji, Rituparna Ghosh, Thang Q. Tran, Seeram Ramakrishna

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Abstract

Alternative current electroluminescence (ACEL) can be identified as an efficient light-emitting technique among a number of different light emission methods. Open-air fabrication capability of the ACEL technique outshines among a few other advantages, whereas electrospinning has been widely identified as a simple, open-air fabrication for nanosized fibers. Here, the authors have combined these two techniques together and fabricated an ACEL device with electrospinning for the first time. The role of electrospinning is highlighted as a scalable fabrication technique to achieve uniform dispersion of both phosphor (ZnS:Cu) and dielectric (BaTiO3) particles. With a greenish-blue luminescence (peak wavelength, 484 nm), the proposed device has achieved a maximum brightness value of 88.55 cd/m2 and a maximum current efficiency of 7.4 cd/A with only 1 kHz sinusoidal input signal. The uniformity of nanofiber mats was evaluated with SEM and EDS analyses, TEM was used as a corroboration. The crystal structures of the active materials were confirmed with X-ray diffraction (XRD) analysis as well. With the opportunities available in both electrospinning and optoelectronic field, this can initiate newer prospects including but not limited to backlighting and smooth light emitting panels in display technology, surface emitting devices in large-area luminescence applications, e.g., in advertising or architectural aspects, and even phototherapeutic applications as well.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Advanced Sensor and Energy Harvesting Materials · Conducting polymers and applications · Electrospun Nanofibers in Biomedical Applications

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Center for Nanotechnology and Sustainability, Department of Mechanical Engineering, National University of Singapore, 119260 Singapore

Funding

Singapore Institute of Manufacturing Technology · National University of Singapore · Lloyd's Register Foundation

References (44)

Show source-provided references
1. Armaroli N. · 2017
2. 10.3390/polym1101009810.3390/polym11010098 ↗
3. Yang, X.; Mutlugun, E.; Gao, Y.; Zhao, Y.; Tan, S. T.; Sun, X. W.; Demir, H. V. InHighly Flexible, Full-Color, Top-Emitting Quantum Dot Light-Emitting Diode Tapes, 2013 IEEE Photonics Conference; IEEE, 2013; Vol. 2, pp 151–152.10.1109/IPCon.2013.6656417 ↗
4. Winkler H. · 2014 · 4910.1002/9783527670147.ch3 ↗
5. Morkoç H. · 2013 · 3 · 20910.1002/9783527649006.ch7 ↗
6. 10.1016/j.mejo.2004.11.00810.1016/j.mejo.2004.11.008 ↗
7. Schubert E. F. · 200610.1017/CBO9780511790546 ↗
8. 10.1002/adom.20180115410.1002/adom.201801154 ↗
9. 10.1039/C9TC01267B10.1039/C9TC01267B ↗
10. Winscom C. J. · 2015 · 1
11. 10.1889/JSID19.11.79810.1889/JSID19.11.798 ↗
12. 10.1016/j.progpolymsci.2018.07.00210.1016/j.progpolymsci.2018.07.002 ↗
13. 10.1016/j.progpolymsci.2013.02.00110.1016/j.progpolymsci.2013.02.001 ↗
14. Coles S. R. · 2015 · 5710.1039/9781849735575-00057 ↗
15. 10.1021/acsami.6b1345310.1021/acsami.6b13453 ↗
16. 10.1021/nl062778+10.1021/nl062778+ ↗
17. 10.1111/jace.1445510.1111/jace.14455 ↗
18. 10.1021/nn201029c10.1021/nn201029c ↗
19. 10.1002/mame.20120027710.1002/mame.201200277 ↗
20. 10.1021/acs.macromol.5b0137710.1021/acs.macromol.5b01377 ↗
21. 10.1016/j.progpolymsci.2014.10.00110.1016/j.progpolymsci.2014.10.001 ↗
22. 10.1364/OE.24.02341910.1364/OE.24.023419 ↗
23. 10.1016/j.ssc.2016.11.01010.1016/j.ssc.2016.11.010 ↗
24. 10.1080/00150193.2017.134999310.1080/00150193.2017.1349993 ↗
25. 10.1016/j.ceramint.2016.07.20910.1016/j.ceramint.2016.07.209 ↗
26. 10.1002/adma.20030215110.1002/adma.200302151 ↗
27. 10.1039/C6NR09302G10.1039/C6NR09302G ↗
28. 10.1002/adma.20140268210.1002/adma.201402682 ↗
29. 10.1016/j.orgel.2014.08.06010.1016/j.orgel.2014.08.060 ↗
30. 10.1016/j.matpr.2017.04.00910.1016/j.matpr.2017.04.009 ↗
31. 10.1039/c3tc30767k10.1039/c3tc30767k ↗
32. 10.3390/ma302135310.3390/ma3021353 ↗
33. 10.1002/adma.20160208310.1002/adma.201602083 ↗
34. 10.1016/j.jallcom.2010.06.07410.1016/j.jallcom.2010.06.074 ↗
35. 10.1007/s10853-018-2540-910.1007/s10853-018-2540-9 ↗
36. 10.1063/1.493564510.1063/1.4935645 ↗
37. 10.1016/j.jssc.2008.05.03710.1016/j.jssc.2008.05.037 ↗
38. Li, Y.; Yang, W.; Gao, X.; Li, C.; Yu, S.; Sun, R. InEnhanced Dielectric Performance of PVDF Composites with Graphene-BaTiO3 Nanohybrids as Fillers, 2016 China Semiconductor Technology International Conference (CSTIC); IEEE, 2016; pp 1–3.10.1109/CSTIC.2016.7463940 ↗
39. 10.1364/OME.6.00287910.1364/OME.6.002879 ↗
40. 10.1039/C7RA01318C10.1039/C7RA01318C ↗
41. 10.1002/adma.20140548610.1002/adma.201405486 ↗
42. 10.3938/jkps.70.44210.3938/jkps.70.442 ↗
43. 10.1021/acsami.0c1013210.1021/acsami.0c10132 ↗
44. 10.1021/acsami.8b2213510.1021/acsami.8b22135 ↗