journal article·2012-09-14

Characterization of amorphous zinc tin oxide semiconductors

Jaana S. Rajachidambaram, Shail Sanghavi, Ponnusamy Nachimuthu, Vaithiyalingam Shutthanandan, Tamas Varga, Brendan Flynn, Suntharampillai Thevuthasan, Gregory S. Herman

Journal of Materials Research· Volume 27· Issue 17
Publisher page

Abstract

Amorphous zinc tin oxide (ZTO) was investigated to determine the effect of deposition and postannealing conditions on film structure, composition, surface contamination, and thin-film transistor (TFT) performance. X-ray diffraction results indicated that the ZTO films remain amorphous even after annealing to 600 °C. Rutherford backscattering spectrometry indicated that the bulk Zn:Sn ratio of the sputter-deposited films were slightly tin rich compared to the composition of the ceramic sputter target. X-ray photoelectron spectroscopy indicated that residual surface contamination depended strongly on the sample postannealing conditions where water, carbonate, and hydroxyl species were adsorbed to the surface. Electrical characterization of ZTO TFTs indicated that the best devices had mobilities of 17 cm2/Vs, threshold voltages of −1.5 V, subthreshold slopes of 0.9 V/dec, turn-on voltages of −12 V, and on-to-off ratio of >107. Annealing ZTO in vacuum assisted in the removal of adsorbed species, which may reduce defects in the films and improve device performance.
Source: expertdata · Quality: candidate unverified · Source record ↗

Research context

OpenAlex topics: Thin-Film Transistor Technologies · Transition Metal Oxide Nanomaterials · ZnO doping and properties

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (52)

Show source-provided references
1. 10.1063/1.171201510.1063/1.1712015 ↗
2. 10.1016/j.jssc.2007.10.02310.1016/j.jssc.2007.10.023 ↗
3. 10.1007/s13391-011-1073-z10.1007/s13391-011-1073-z ↗
4. 10.1063/1.364304010.1063/1.3643040 ↗
5. 10.1021/la801105210.1021/la8011052 ↗
6. 10.1063/1.37368510.1063/1.373685 ↗
7. 10.1021/jp027554410.1021/jp0275544 ↗
8. 40. Freeware available at www.uksaf.org/xpspeak41.zip
9. 10.1016/j.matchar.2011.07.00610.1016/j.matchar.2011.07.006 ↗
10. 10.1016/j.matchemphys.2011.10.01310.1016/j.matchemphys.2011.10.013 ↗
11. 10.1016/j.jallcom.2004.08.05310.1016/j.jallcom.2004.08.053 ↗
12. 10.1016/j.apsusc.2007.03.03610.1016/j.apsusc.2007.03.036 ↗
13. 10.1016/j.apsusc.2011.04.05210.1016/j.apsusc.2011.04.052 ↗
14. 10.1063/1.148310410.1063/1.1483104 ↗
15. 10.1016/j.surfrep.2010.09.00110.1016/j.surfrep.2010.09.001 ↗
16. 10.1088/1468-6996/11/4/04430510.1088/1468-6996/11/4/044305 ↗
17. 10.1038/nmat256010.1038/nmat2560 ↗
18. 10.1021/jp803475g10.1021/jp803475g ↗
19. 10.1063/1.280693410.1063/1.2806934 ↗
20. 10.3938/jkps.54.54410.3938/jkps.54.544 ↗
21. 10.1063/1.282886210.1063/1.2828862 ↗
22. 10.1143/JJAP.44.L3410.1143/JJAP.44.L34 ↗
23. 10.1149/1.266658810.1149/1.2666588 ↗
24. 10.1088/0022-3727/42/3/03510610.1088/0022-3727/42/3/035106 ↗
25. 10.1063/1.184328610.1063/1.1843286 ↗
26. 10.1016/j.jnoncrysol.2006.01.07310.1016/j.jnoncrysol.2006.01.073 ↗
27. Mayer · 1997
28. 10.1016/0169-4332(94)90031-010.1016/0169-4332(94)90031-0 ↗
29. 10.1063/1.212089510.1063/1.2120895 ↗
30. Kluth · 2003 · 1800
31. 10.1021/ja100615r10.1021/ja100615r ↗
32. 10.1149/1.347460610.1149/1.3474606 ↗
33. 10.1016/j.sse.2006.03.00410.1016/j.sse.2006.03.004 ↗
34. Ink-jet-printed zinc–tin–oxide thin-film transistors and circuits with rapid thermal annealing process
35. 10.1038/nature0309010.1038/nature03090 ↗
36. 10.1143/JJAP.33.L169310.1143/JJAP.33.L1693 ↗
37. 10.1116/1.234520610.1116/1.2345206 ↗
38. 10.1016/S0925-4005(98)00135-X10.1016/S0925-4005(98)00135-X ↗
39. 10.1063/1.278396110.1063/1.2783961 ↗
40. 10.1116/1.212795410.1116/1.2127954 ↗
41. 10.1149/1.351660810.1149/1.3516608 ↗
42. 10.1038/nmat301110.1038/nmat3011 ↗
43. 10.1063/1.302071410.1063/1.3020714 ↗
44. 10.1109/TED.2008.201167910.1109/TED.2008.2011679 ↗
45. 10.2298/SOS0702153I10.2298/SOS0702153I ↗
46. 10.1116/1.283986010.1116/1.2839860 ↗
47. Preparation and characterization of transparent conducting Zn-Sn-O films deposited on organic substrates at low temperature
48. 10.1116/1.57959210.1116/1.579592 ↗
49. 10.1016/j.jallcom.2010.10.21210.1016/j.jallcom.2010.10.212 ↗
50. 10.1002/adma.20090245010.1002/adma.200902450 ↗
51. 10.1016/j.tsf.2007.10.05510.1016/j.tsf.2007.10.055 ↗
52. 10.1016/j.snb.2009.07.05610.1016/j.snb.2009.07.056 ↗