journal article·2021-08-21Open access

High-Performance Flexible Transparent Electrodes Fabricated via Laser Nano-Welding of Silver Nanowires

Tao Wang, Yinzhou Yan, Liye Zhu, Qian Li, Jing He, Xiaoxia Zhang, Xi Li, Xiaohua Zhang, Yongman Pan, Yue Wang

Crystals· Volume 11· Issue 8

Abstract

Silver nanowires (Ag-NWs), which possess a high aspect ratio with superior electrical conductivity and transmittance, show great promise as flexible transparent electrodes (FTEs) for future electronics. Unfortunately, the fabrication of Ag-NW conductive networks with low conductivity and high transmittance is a major challenge due to the ohmic contact resistance between Ag-NWs. Here we report a facile method of fabricating high-performance Ag-NW electrodes on flexible substrates. A 532 nm nanosecond pulsed laser is employed to nano-weld the Ag-NW junctions through the energy confinement caused by localized surface plasmon resonance, reducing the sheet resistance and connecting the junctions with the substrate. Additionally, the thermal effect of the pulsed laser on organic substrates can be ignored due to the low energy input and high transparency of the substrate. The fabricated FTEs demonstrate a high transmittance (up to 85.9%) in the visible band, a low sheet resistance of 11.3 Ω/sq, high flexibility and strong durability. The applications of FTEs to 2D materials and LEDs are also explored. The present work points toward a promising new method for fabricating high-performance FTEs for future wearable electronic and optoelectronic devices.
Source: crossref · Quality: baseline

Research context

OpenAlex topics: Advanced Sensor and Energy Harvesting Materials · Nanomaterials and Printing Technologies · ZnO doping and properties

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Faculty of Science, Beijing University of Technology, Beijing 100124, China

Faculty of Materials and Manufacturing, Beijing University of Technology, Beijing 100124, China

Funding

Beijing Municipal Commission of Education · National Natural Science Foundation of China

References (44)

Show source-provided references
1. Flexible, Transparent, and Conductive Ti3C2Tx MXene-Silver Nanowire Films with Smart Acoustic Sensitivity for High-Performance Electromagnetic Interference Shielding10.1021/acsnano.0c01635 ↗
2. Realizing Ultrahigh Mechanical Flexibility and >15% Efficiency of Flexible Organic Solar Cells via a “Welding” Flexible Transparent Electrode10.1002/adma.201908478 ↗
3. Improvements in the electroless deposition of Ag nanowires in hot ethylene glycol for resistive touchscreen device10.1016/j.materresbull.2018.06.030 ↗
4. Highly sensitive wearable strain sensor based on silver nanowires and nanoparticles10.1088/1361-6528/aabbba ↗
5. Highly flexible organic light-emitting diodes on patterned Ag nanowire network transparent electrodes10.1016/j.orgel.2019.05.035 ↗
6. Highly stabilized flexible transparent capacitive photodetector based on silver nanowire/graphene hybrid electrodes10.1038/s41598-021-88730-6 ↗
7. Wetting-Induced Fabrication of Graphene Hybrid with Conducting Polymers for High-Performance Flexible Transparent Electrodes10.1021/acsami.0c15734 ↗
8. Flexible and Transparent Graphene Electrode Architecture with Selective Defect Decoration for Organic Light-Emitting Diodes10.1002/adfm.201704435 ↗
9. Cryo-Transferred Ultrathin and Stretchable Epidermal Electrodes10.1002/smll.202000450 ↗
10. Embedding Silver Nanowires into a Hydroxypropyl Methyl Cellulose Film for Flexible Electrochromic Devices with High Electromechanical Stability10.1021/acsami.0c16066 ↗
11. Mechanically and thermally stable, transparent electrodes with silver nanowires encapsulated by atomic layer deposited aluminium oxide for organic optoelectronic devices10.1016/j.orgel.2019.105593 ↗
12. Facile preparation of flexible and highly stable graphene oxide-silver nanowire hybrid transparent conductive electrode10.1088/2053-1591/ab6262 ↗
13. A highly bendable transparent electrode for organic electrochromic devices10.1016/j.orgel.2018.12.015 ↗
14. Ultrahigh-performance transparent conductive films of carbon-welded isolated single-wall carbon nanotubes10.1126/sciadv.aap9264 ↗
15. Fabrication of Flexible Carbon Nanotube Network on Paper Substrate: Effect of Post Treatment Temperature on Electrodes10.1166/jno.2020.2896 ↗
16. Hybrid PEDOT:PSS to obtain high-performance Ag NW-based flexible transparent electrodes for transparent heaters10.1007/s10854-020-03351-5 ↗
17. Song, J., Ma, G., Qin, F., Hu, L., Luo, B., Liu, T., Yin, X., Su, Z., Zeng, Z., and Jiang, Y. (2020). High-Conductivity, Flexible and Transparent PEDOT:PSS Electrodes for High Performance Semi-Transparent Supercapacitors. Polymers, 12.10.3390/polym12020450 ↗
18. Facile fabrication of large-scale silver nanowire-PEDOT:PSS composite flexible transparent electrodes for flexible touch panels10.1088/2053-1591/ab20d5 ↗
19. Silver nanowire networks with preparations and applications: A review10.1007/s10854-020-04131-x ↗
20. Flexible Transparent Conductive Films with High Performance and Reliability Using Hybrid Structures of Continuous Metal Nanofiber Networks for Flexible Optoelectronics10.1021/acsami.7b04314 ↗
21. Seed-mediated synthesis of ultra-long copper nanowires and their application as transparent conducting electrodes10.1016/j.apsusc.2017.06.051 ↗
22. Smart, soft contact lens for wireless immunosensing of cortisol10.1126/sciadv.abb2891 ↗
23. A soft and transparent contact lens for the wireless quantitative monitoring of intraocular pressure10.1038/s41551-021-00719-8 ↗
24. Facile Approach to Fabricating Stretchable Organic Transistors with Laser-Patterned Ag Nanowire Electrodes10.1021/acsami.0c15339 ↗
25. Stretchable Transparent Conductive Films Based on Ag Nanowires for Flexible Circuits and Tension Sensors10.1021/acsanm.1c00217 ↗
26. Thermal annealing effects on silver nanowire networks10.1504/IJNT.2014.063788 ↗
27. Oh, J.S., Oh, J.S., and Yeom, G.Y. (2020). Invisible Silver Nanomesh Skin Electrode via Mechanical Press Welding. Nanomaterials, 10.10.3390/nano10040633 ↗
28. Capillary-Force-Induced Cold Welding in Silver-Nanowire-Based Flexible Transparent Electrodes10.1021/acs.nanolett.6b04613 ↗
29. Electrically sintered silver nanowire networks for use as transparent electrodes and heaters10.1088/2053-1591/ab47e0 ↗
30. Electron beam irradiated silver nanowires for a highly transparent heater10.1038/srep17716 ↗
31. Facile and Efficient Welding of Silver Nanowires Based on UVA-Induced Nanoscale Photothermal Process for Roll-to-Roll Manufacturing of High-Performance Transparent Conducting Films10.1002/admi.201801635 ↗
32. Hu, Y., Liang, C., Sun, X., Zheng, J., Duan, J.A., and Zhuang, X. (2019). Enhancement of the Conductivity and Uniformity of Silver Nanowire Flexible Transparent Conductive Films by Femtosecond Laser-Induced Nanowelding. Nanomaterials, 9.10.3390/nano9050673 ↗
33. Lee, P., Kwon, J., Lee, J., Lee, H., Suh, Y.D., Hong, S., and Yeo, J. (2017). Rapid and Effective Electrical Conductivity Improvement of the Ag NW-Based Conductor by Using the Laser-Induced Nano-Welding Process. Micromachines, 8.10.3390/mi8050164 ↗
34. Highly localized heat generation by femtosecond laser induced plasmon excitation in Ag nanowires10.1063/1.4790189 ↗
35. Crystalline Nanojoining Silver Nanowire Percolated Networks on Flexible Substrate10.1021/acsnano.5b03601 ↗
36. Quantitative Study of the Photothermal Properties of Metallic Nanowire Networks10.1021/acsnano.5b01673 ↗
37. Creating Well-Defined Hot Spots for Surface-Enhanced Raman Scattering by Single-Crystalline Noble Metal Nanowire Pairs10.1021/jp809391c ↗
38. Effect of crossing geometry on the plasmonic behavior of dielectric core/metal sheath nanowires10.1063/1.3094129 ↗
39. Broadband nano-focusing of light using kissing nanowires10.1088/1367-2630/12/9/093030 ↗
40. New figure of merit for transparent conductors10.1063/1.323240 ↗
41. Instantaneous and Repeatable Self-Healing of Fully Metallic Electrodes at Ambient Conditions10.1021/acsami.9b12417 ↗
42. Samy, O., Zeng, S., Birowosuto, M.D., and El Moutaouakil, A. (2021). A Review on MoS2 Properties, Synthesis, Sensing Applications and Challenges. Crystals, 11.10.3390/cryst11040355 ↗
43. Electrical control of optical properties of monolayer MoS210.1016/j.ssc.2012.11.010 ↗
44. Electric-field effect on photoluminescence of lead-halide perovskites10.1016/j.mattod.2019.01.003 ↗