journal article·2021-08-15Open access

A Study on Solution-Processed Y2O3 Films Modified by Atomic Layer Deposition Al2O3 as Dielectrics in ZnO Thin Film Transistor

Haiyang Xu, Xingwei Ding, Jie Qi, Xuyong Yang, Jianhua Zhang

Coatings· Volume 11· Issue 8

Abstract

In this work, Y2O3–Al2O3 dielectrics were prepared and used in ZnO thin film transistor as gate insulators. The Y2O3 film prepared by the sol–gel method has many surface defects, resulting in a high density of interface states with the active layer in TFT, which then leads to poor stability of the devices. We modified it by atomic layer deposition (ALD) technology that deposited a thin Al2O3 film on the surface of a Y2O3 dielectric layer, and finally fabricated a TFT device with ZnO as the active layer by ALD. The electrical performance and bias stability of the ZnO TFT with a Y2O3–Al2O3 laminated dielectric layer were greatly improved, the subthreshold swing was reduced from 147 to 88 mV/decade, the on/off-state current ratio was increased from 4.24 × 106 to 4.16 × 108, and the threshold voltage shift was reduced from 1.4 to 0.7 V after a 5-V gate was is applied for 800 s.
Source: crossref · Quality: baseline

Research context

OpenAlex topics: Thin-Film Transistor Technologies · ZnO doping and properties · Semiconductor materials and devices

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Key Laboratory of Advanced Display and System Application, Ministry of Education, Shanghai University, Shanghai 200072, China

School of Mechatronics and Automation, Shanghai University, Shanghai 200072, China

Research and Development Department, Air Liquide Innovation Campus Shanghai, Shanghai 201108, China

Funding

National Natural Science Foundation of China

References (27)

Show source-provided references
1. Enhanced electrical properties of oxide semiconductor thin-film transistors with high conductivity thin layer insertion for the channel region10.1016/j.apsusc.2016.11.194 ↗
2. Recent progress in transparent oxide semiconductors: Materials and device application10.1016/j.tsf.2006.12.125 ↗
3. Metal oxides for optoelectronic applications10.1038/nmat4599 ↗
4. Metal oxide semiconductor thin-film transistors for flexible electronics10.1063/1.4953034 ↗
5. Material characteristics and applications of transparent amorphous oxide semiconductors10.1038/asiamat.2010.5 ↗
6. Wide-bandgap high-mobility ZnO thin-film transistors produced at room temperature10.1063/1.1790587 ↗
7. Bottom-gate zinc oxide thin-film transistors (ZnO TFTs) for AM-LCDs10.1109/TED.2008.2003330 ↗
8. Interface studies of N2 plasma-treated ZnSnO nanowire transistors using low-frequency noise measurements10.1088/0957-4484/24/30/305201 ↗
9. Enhanced Reliability of In–Ga–ZnO thin-film transistors through design of dual passivation layers10.1109/TED.2018.2836146 ↗
10. Bi-layer channel structure-based oxide thin-film transistors consisting of ZnO and Al-doped ZnO with different Al compositions and stacking sequences10.1007/s13391-014-4305-1 ↗
11. Effect of Hf alloy in ZrOx gate insulator for solution processed a-IZTO Thin Film Transistors
12. Solution-Processed Amorphous In–Zn–Sn Oxide Thin-film transistor performance improvement by solution-processed Y2O3 passivation10.1109/LED.2016.2528288 ↗
13. Solvent engineering for high-performance inorganic–organic hybrid perovskite solar cells10.1038/nmat4014 ↗
14. Past achievements and future challenges in the development of optically transparent electrodes10.1038/nphoton.2012.282 ↗
15. Flexible self-powered ZnO film UV sensor with a high response10.1021/acsami.9b09264 ↗
16. Improvement of bias-stability in amorphous-indium-gallium-zinc-oxide thin-film transistors by using solution-processed Y2O3 passivation10.1063/1.4892541 ↗
17. Evaluation of Y2O3 gate insulators for a-IGZO thin film transistors10.1016/j.tsf.2009.02.020 ↗
18. Enhanced light stability of InGaZnO thin-film transistors by atomic-layer-deposited Y2O3 with Ozone10.1021/acsami.7b14260 ↗
19. Controlled Zr doping for inkjet-printed ZTO TFTs10.1016/j.ceramint.2016.11.165 ↗
20. Half-volt operation of IGZO thin-film transistors enabled by ultrathin HfO2 gate dielectric10.1063/1.5037410 ↗
21. Water-induced scandium Oxide dielectric for low-operating voltage n- and p-type metal-oxide thin-film transistors10.1002/adfm.201502612 ↗
22. A solution-processed yttrium oxide gate insulator for high-performance all-solution-processed fully transparent thin film transistors10.1039/c2jm34162j ↗
23. Nitrogen-doped ZnO film fabricated via rapid low-temperature atomic layer deposition for high-performance ZnON transistors10.1109/TED.2018.2848275 ↗
24. Adamopoulos, G., Thomas, S., Bradley, D., McLachlan, M., and Anthopoulos, T. (2011). Low-voltage ZnO thin-film transistors based on Y2O3 and Al2O3 high-k dielectrics deposited by spray pyrolysis in air. Appl. Phys. Lett., 98.10.1063/1.3568893 ↗
25. Effect of double-layered Al2O3/SiO2 dielectric materials on In–Ga–Zn–O(IGZO)-based amorphous transparent thin film transistors10.1016/j.ceramint.2014.04.151 ↗
26. High-performance ZnO thin-film transistors on gate dielectrics grown by atomic layer deposition10.1063/1.2188379 ↗
27. High-Performance 1-V ZnO Thin-film transistors with ultrathin, ALD-processed ZrO2 gate dielectric10.1109/TED.2019.2924135 ↗