journal article·2019-09Open access

Inferring radiation-induced microstructural evolution in single-crystal niobium through changes in thermal transport

Sara E. Ferry, Cody A. Dennett, Kevin B. Woller, Michael P. Short

Abstract

Abstract Ion beams enable accelerated radiation exposure experiments, but traditional destructive post-irradiation examination techniques remain time-consuming. Here, measurements of thermal diffusivity are used to monitor microstructural changes in single crystal niobium irradiated with Si3+ ions up to 1.9 dpa (5.1 × 1015 ions/cm2). Changes in thermal transport are correlated to defect generation and clustering through dose-microstructure relationships. These measurements are made using transient grating spectroscopy (TGS), a multi-modal, non-destructive, rapid characterization technique. This work demonstrates that in this low-dose point defect clustering regime, direct measurements of thermal properties are a powerful tool for understanding irradiation-induced microstructure evolution.
Source: openaire · Quality: candidate unverified · Source record ↗

Research context

OpenAlex topics: Ion-surface interactions and analysis · Fusion materials and technologies · Nuclear Materials and Properties

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (41)

Show source-provided references
1. Soneda · 2014
2. Irradiation response of delta ferrite in as-cast and thermally aged cast stainless steel10.1016/j.jnucmat.2015.08.006 ↗
3. Use of self-ion bombardment to study void swelling in advanced radiation-resistant alloys
4. Materials challenges in nuclear energy10.1016/j.actamat.2012.11.004 ↗
5. Mechanical property degradation in irradiated materials: a multiscale modeling approach10.1016/S0168-583X(01)00392-5 ↗
6. Emulation of reactor irradiation damage using ion beams10.1016/j.scriptamat.2014.06.003 ↗
7. Opportunities and limitations for ion beams in radiation effects studies: bridging critical gaps between charged particle and neutron irradiations10.1016/j.scriptamat.2017.06.041 ↗
8. Development of a nondestructive inspection method for irradiation-induced microstructural evolution of thick 304 stainless steel blocks10.1016/j.jnucmat.2013.02.036 ↗
9. Microstructure changes and thermal conductivity reduction in uo2 following 3.9 MeV He 2+ ion irradiation10.1016/j.jnucmat.2014.07.053 ↗
10. Measurement of thermal conductivity in proton irradiated silicon10.1016/j.nimb.2014.02.003 ↗
11. Thermal conductivity measurements via time-domain thermoreflectance for the characterization of radiation induced damage10.1557/jmr.2015.11 ↗
12. Evaluation of radiation damage using nonlinear ultrasound10.1063/1.3692086 ↗
13. Sensitivity of ultrasonic nonlinearity to irradiated, annealed, and re-irradiated microstructure changes in RPV steels10.1016/j.jnucmat.2014.01.038 ↗
14. Optical generation and characterization of acoustic waves in thin films: fundamentals and applications10.1146/annurev.matsci.30.1.117 ↗
15. Optical heterodyne detection of laser-induced gratings10.1364/OL.23.001319 ↗
16. Lattice swelling and modulus change in a helium-implanted tungsten alloy: X-ray micro-diffraction, surface acoustic wave measurements, and multiscale modelling10.1016/j.actamat.2015.01.055 ↗
17. Non-contact measurement of thermal diffusivity in ion-implanted nuclear materials10.1038/srep16042 ↗
18. Detecting self-ion irradiation-induced void swelling in pure copper using transient grating spectroscopy10.1016/j.actamat.2017.12.007 ↗
19. Bridging the gap to mesoscale radiation materials science with transient grating spectroscopy10.1103/PhysRevB.94.214106 ↗
20. Increase in elastic anisotropy of single crystal tungsten upon He-ion implantation measured with laser-generated surface acoustic waves10.1063/1.4964709 ↗
21. Real-time thermomechanical property monitoring during ion beam irradiation using in situ transient grating spectroscopy10.1016/j.nimb.2018.10.025 ↗
22. The effect of cold-work distortion on X-ray patterns10.1063/1.1699713 ↗
23. X-ray line broadening from filed aluminium and wolfram10.1016/0001-6160(53)90006-6 ↗
24. Broadening of X-ray diffraction lines of crystals containing dislocation distributions10.1002/crat.19760111108 ↗
25. Defect structure of epitaxial GaN films determined by transmission electron microscopy and triple-axis X-ray diffractometry10.1080/01418619808221225 ↗
26. The estimation of dislocation densities in metals from X-ray data10.1016/0001-6160(53)90106-0 ↗
27. Dislocation density calculation
28. Ferry · 2018
29. SRIM–the stopping and range of ions in matter (2010)10.1016/j.nimb.2010.02.091 ↗
30. Transient thermal gratings at surfaces for thermal characterization of bulk materials and thin films10.1007/BF01538190 ↗
31. Real-time thermomechanical property monitoring during ion beam irradiation using in situ transient grating spectroscopy10.1016/j.nimb.2018.10.025 ↗
32. Time-resolved, dual heterodyne phase collection transient grating spectroscopy10.1063/1.4983716 ↗
33. Thermal diffusivity determination using heterodyne phase insensitive transient grating spectroscopy10.1063/1.5026429 ↗
34. Phase-controlled, heterodyne laser-induced transient grating measurements of thermal transport properties in opaque material10.1063/1.3675467 ↗
35. Optical generation of long-lived surface vibrations in a periodic microstructure10.1063/1.3153956 ↗
36. Was · 2016
37. Electrical-resistivity model for polycrystalline films: the case of arbitrary reflection at external surfaces10.1103/PhysRevB.1.1382 ↗
38. Scattering of electrons at threading dislocations in GaN10.1063/1.366585 ↗
39. Effect of oxygen impurity on defect agglomeration and hardening of neutron-irradiated niobium10.1016/0001-6160(73)90058-8 ↗
40. Microstructural characterisation of proton irradiated niobium using X-ray diffraction technique
41. Comparison of swelling and irradiation creep behavior of FCC-austenitic and BCC-ferritic/martensitic alloys at high neutron exposure10.1016/S0022-3115(99)00225-1 ↗