Adaptive helicity and chiral recognition in bright europium quadruple-stranded helicates induced by host-guest interaction
Source abstract
Abstract
Chiral information transfer is crucial to design new functions like, for instance, sensing through chiroptical probes in which the input is readout as a consequence of a chiral recognition event. Herein, we report lanthanide quadruple-stranded helicates [Ln2L4]2− that show a guest-to-host chirality transfer. As confirmed by X-ray diffraction (XRD) and density functional theory (DFT) calculations, these cages are present in solution as an equilibrating racemic mixture of left- and right-handed helicates. The helicates adapt their helical conformation by encapsulation of a chiral guest enabling also straightforward enantiomeric excess determination. Asymmetric induction is demonstrated by circular dichroism (CD) and circularly polarized luminescence (CPL), and a helicity inversion mechanism based on a Bailar twist is proposed and studied by DFT calculations. The presented research contributes to the design of helicates with a unique combination of confined cavities, adaptive chirality, and peculiar luminescent properties, finding applications toward the development of optical probes for selective chiral sensing via molecular recognition.
Source: openalex_inverted_index · Quality: baseline
Research context
OpenAlex topics: Lanthanide and Transition Metal Complexes · Supramolecular Chemistry and Complexes · Magnetism in coordination complexes
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
References (80)
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