journal article·2024-07Open access

Further hydration hardening behavior of CO2-cured sodium-doped calcium silicate compacts

Luyi Sun, Songhui Liu, Yuli Wang, Saisai Zhang, Jianping Zhu, Xuemao Guan, Caijun Shi

Abstract

To further enhance the mechanical properties of CO2-cured sodium-doped calcium silicate (Na2Ca2Si3O9) compacts and promote sustainable low-carbon materials, this study analyzed the subsequent hydration hardening behavior after initial carbonation curing. The compressive strength evolution, pore structure, phase composition, and microstructure were characterized through strength tests, 1H NMR, XRD, TGA, FTIR, and SEM analyses. The findings reveal that subjecting carbonated Na2Ca2Si3O9 compacts to further water-saturated hydration curing enhances their hardening performance. The compressive strength of the 28 d subsequent hydration-cured samples exhibited a remarkable increase compared to the carbonated counterparts. Microscopic examination elucidates that sufficient water facilitates continuous reactions between carbonation products and unreacted Na2Ca2Si3O9, generating more prismatic pirssonite(Na2Ca(CO3)2·2H2O), CaCO3, and (N)-C-S-H gels, leading to reduced porosity and superior compressive strength. The proposed mechanism offers insights into activating the subsequent hardening process of carbonated cementitious materials.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Concrete and Cement Materials Research · Magnesium Oxide Properties and Applications · Concrete Properties and Behavior

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

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