journal article·2025-07Open access

Time-dependent model for in-situ concrete carbonation depth under combined effects of temperature and relative humidity

Ting Du, Yongjia Cai, Yipu Guo, Jinghao Chen, Sen Chen, Mofang Yuan, Fulin Qu

Abstract

Fluctuations in temperatures and relative humidity in the external environment significantly influence the carbonation depth in concrete structures, making it an essential topic when considering concrete durability . This study aims to predict and compare the carbonation depth of concrete under various temperature and relative humidity conditions through both experiment and modeling. The experimental results demonstrate an exponential relationship between carbonation depth and temperature at all ages of the concrete, showing a consistent increase, with rising temperature. Additionally, the carbonation depth of concrete exhibits a parabolic relationship with relative humidity, characterized by an initial increase followed by a subsequent decrease, forming a downward-opening curve. This relationship is well-corrected with the data. Moreover, sensitivity analysis reveals a noticeable variation in sensitivity factors related to temperature and relative humidity after a 28-day carbonation period, with the sensitivity factor for temperature being higher than that for relative humidity. Finally, by employing the Sensitivity Analysis and Least-Square Fitting (SA-LSF) method, a novel model is developed that incorporates both temperature and relative humidity as influential factors in predicting carbonation depth under diverse environmental conditions. The experimental results align well with the model’s predictions, confirming its ability to accurately forecast carbonation depth of concrete. These findings provide significant insights for practical applications, as the model can give valuable predictions for carbonation in concrete.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Concrete and Cement Materials Research · Concrete Properties and Behavior · Rock Mechanics and Modeling

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (62)

Show source-provided references
1. Variation of self-cleaning performance of nano-TiO2 modified mortar caused by carbonation: From hydrates to carbonates10.1016/j.cemconres.2022.106852 ↗
2. Impacts of climate change on optimal mixture design of blended concrete considering carbonation and chloride ingress10.1007/s11709-020-0608-5 ↗
3. Novel empirical model for predicting residual flexural capacity of corroded steel reinforced concrete beam10.1007/s11709-020-0637-0 ↗
4. Effect of microlimestone on properties of self-consolidating concrete with manufactured sand and mineral admixture10.1007/s11709-020-0678-4 ↗
5. Optimum proportion of fly ash or slag for resisting concrete deterioration due to carbonation and chloride ingress
6. Durability deterioration of concrete under marine environment from material to structure: A critical review
7. Multi-region lifetime assessment of reinforced concrete structures subjected to carbonation and climate change
8. Three-dimensional lattice modeling of concrete carbonation at meso-scale based on reconstructed coarse aggregates10.1016/j.conbuildmat.2018.10.052 ↗
9. The pore solution of blended cements: a review10.1617/s11527-015-0724-1 ↗
10. Investigation of the carbonation performance of cement-based materials under high temperatures10.1016/j.conbuildmat.2020.121634 ↗
11. Microstructure and phase assemblage of low-clinker cements during the early stages of carbonation10.1016/j.cemconres.2021.106643 ↗
12. A study on the change in frost resistance and pore structure of concrete containing blast furnace slag under the carbonation conditions10.1016/j.conbuildmat.2022.127295 ↗
13. Natural and accelerated CO2 binding kinetics in cement paste at different relative humidities10.1016/j.cemconres.2013.03.009 ↗
14. Effect of polyacrylamide on the carbonation behavior of cement paste10.1016/j.cemconres.2022.106756 ↗
15. Influence of carbonation on chloride binding of mortars made with simulated marine sand10.1016/j.conbuildmat.2021.124455 ↗
16. Predicting carbonation in early-aged cracked concrete10.1016/j.cemconres.2005.12.019 ↗
17. Alternative pH-indicators for determination of carbonation depth on cement-based concretes10.1016/j.cemconcomp.2020.103565 ↗
18. Effect of global climatic change on carbonation progress of concrete10.1016/j.atmosenv.2007.05.028 ↗
19. A review on effects of curing, sheltering, and CO2 concentration upon natural carbonation of concrete10.1016/j.conbuildmat.2016.09.056 ↗
20. Carbonation of cement paste: Understanding, challenges, and opportunities10.1016/j.conbuildmat.2016.04.138 ↗
21. Effects of carbonation on phase composition of Metakaolin-blended cement pastes10.1016/j.conbuildmat.2022.126639 ↗
22. Chloride-binding capacity of cement-GGBFS-nanosilica composites under seawater chloride-rich environment10.1016/j.conbuildmat.2022.127890 ↗
23. Effects of pipe diameter, curing age and exposure temperature on chloride diffusion of concrete with embedded PVC pipe
24. Anti-cracking and shrinkage performance of sustainable concrete incorporating high-volume natural pozzolans: A case design for high-speed railway concrete slab tracks
25. Carbonation performance of concrete with fly ash as fine aggregate after stress damage and high temperature exposure10.1016/j.conbuildmat.2020.118125 ↗
26. Analysis of an accelerated carbonation test with severe preconditioning10.1016/j.cemconres.2014.01.003 ↗
27. Carbonation in concrete infrastructure in the context of global climate change: Development of a service lifespan model10.1016/j.conbuildmat.2012.11.026 ↗
28. Properties investigation of recycled aggregates and concrete modified by accelerated carbonation through increased temperature10.1016/j.conbuildmat.2022.127813 ↗
29. Increasing efficiency of carbon dioxide sequestration through high temperature carbonation of cement-based materials10.1016/j.jclepro.2019.117980 ↗
30. Carbonation of hardened cement pastes: Influence of temperature10.1016/j.cemconres.2018.09.019 ↗
31. A carbonation prediction model for accelerated carbonation testing of concrete10.1680/macr.1994.46.168.191 ↗
32. The role of relative humidity and cement type on carbonation resistance of concrete10.1016/j.aej.2019.10.008 ↗
33. Effects of stress and high temperature on the carbonation resistance of fly ash concrete10.1016/j.conbuildmat.2017.02.039 ↗
34. An improved model calculating CO2 solubility in pure water and aqueous NaCl solutions from 273 to 533 K and from 0 to 2000 bar10.1016/S0009-2541(02)00263-2 ↗
35. Understanding the process of carbonation in concrete using numerical modeling10.3151/jact.19.1148 ↗
36. Wet-carbonation-based Mineral Extraction and CO2 Sequestration Using Concrete Waste Fines at a Low Temperature10.3151/jact.21.166 ↗
37. Permeability of sulfate ions in cementitious materials containing γ-Ca2SiO4 after autoclave curing and accelerated carbonation10.3151/jact.9.223 ↗
38. Carbon sequestration, performance optimization and environmental impact assessment of functional materials in cementitious composites10.1016/j.jcou.2024.102986 ↗
39. Fundamental modeling and experimental investigation of concrete carbonation
40. Durability of concrete—accelerated carbonation and weathering studies10.1016/S0360-1323(98)00042-0 ↗
41. Neutron diffraction for studying the influence of the relative humidity on the carbonation process of cement pastes
42. Strategies to accelerate CO2 sequestration of cement-based materials and their application prospects10.1016/j.conbuildmat.2021.125646 ↗
43. Carbonation model for fly ash concrete based on artificial neural network: Development and parametric analysis10.1016/j.conbuildmat.2020.121050 ↗
44. Time-dependent reliability analysis of recycled aggregate concrete cover cracking induced by reinforcement corrosion
45. A review on the modelling of carbonation of hardened and fresh cement-based materials10.1016/j.cemconcomp.2021.104315 ↗
46. Effect of supplementary cementing materials on concrete resistance against carbonation and chloride ingress10.1016/S0008-8846(99)00249-5 ↗
47. A reaction engineering approach to the problem of concrete carbonation10.1002/aic.690351008 ↗
48. Influence of environmental moisture and temperature on carbonation of mortar10.3151/crt1990.1.1_85 ↗
49. Carbonation depth model and carbonated acceleration rate of concrete under different environment10.1016/j.cemconcomp.2020.103736 ↗
50. Carbonation in concrete infrastructure in the context of global climate change–Part 1: Experimental results and model development10.1016/j.cemconcomp.2012.04.011 ↗
51. Carbonation of blended cement concretes after 12 years of natural exposure10.1016/j.conbuildmat.2020.122122 ↗
52. Accelerated carbonation testing of alkali-activated slag/metakaolin blended concretes: effect of exposure conditions10.1617/s11527-014-0289-4 ↗
53. Economic feasibility and sensitivity analysis of integrating industrial-scale mineral carbonation into mining operations10.1016/j.mineng.2012.07.007 ↗
54. Carbonation of the synthetic calcium silicate hydrate (CSH) under different concentrations of CO2: Chemical phases analysis and kinetics10.1016/j.jcou.2019.10.001 ↗
55. Development of hybrid models using metaheuristic optimization techniques to predict the carbonation depth of fly ash concrete10.1016/j.conbuildmat.2022.128483 ↗
56. Impact of the microstructure model on coupled simulation of drying and accelerated carbonation10.1016/j.cemconres.2017.11.008 ↗
57. A modified numerical model for predicting carbonation depth of concrete with stress damage10.1016/j.conbuildmat.2021.124389 ↗
58. Prediction of carbonation depth for recycled aggregate concrete using ANN hybridized with swarm intelligence algorithms10.1016/j.conbuildmat.2021.124382 ↗
59. An assessment on parameters affecting the carbonation of alkali-activated slag concrete10.1016/j.jclepro.2017.04.097 ↗
60. Predicting carbonation depth for concrete with organic film coatings combined with ageing effects10.1016/j.conbuildmat.2017.03.063 ↗
61. A model for predicting the carbonation depth of concrete containing low-calcium fly ash10.1016/j.conbuildmat.2008.02.019 ↗
62. Effects of urea on carbonation properties and microstructure of cementitious materials